Partitioning between sediment and porewater of radiocesium from Chernobyl fallout
Description
As part of a joint USA/USSR Environmental Agreement to determine the distribution and concentration of Chernobyl radioactivity in the northwest Black Sea area, the sediment from eight stations was collected and analyzed to assess the ability of sediment from the northwest Black Sea to adsorb radiocesium. Two methods were used to determine partitioning between liquid and solid phases; batch tests and porewater separation. In the batch test, Cs-137 tracer was added to mixtures of sediment and bottom water, with contact solutions ranging from 85 Bq/ml to 1760 Bq/ml. The distribution ratios (R{sub D}) for individual batch tests ranged from 390 … continued below
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32 pages
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- United States. Department of Energy. DOE; USDOE, Washington, DC (United States)
- United States. Environmental Protection Agency. EPA; Environmental Protection Agency, Washington, DC (United States)
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Brookhaven National Laboratory
Place of Publication: Upton, New York
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Description
As part of a joint USA/USSR Environmental Agreement to determine the distribution and concentration of Chernobyl radioactivity in the northwest Black Sea area, the sediment from eight stations was collected and analyzed to assess the ability of sediment from the northwest Black Sea to adsorb radiocesium. Two methods were used to determine partitioning between liquid and solid phases; batch tests and porewater separation. In the batch test, Cs-137 tracer was added to mixtures of sediment and bottom water, with contact solutions ranging from 85 Bq/ml to 1760 Bq/ml. The distribution ratios (R{sub D}) for individual batch tests ranged from 390 to 1770 ml/g. Isotherms were linear for all cores and R{sub D} values calculated from the slopes of the isotherms ranged from 660 to 1660 ml/g. A second approach was used to determine the partitioning of Cs-137 between the porewater and the sediment under more natural conditions. The top 2 cm of two cores were sectioned and the sediment and the porewater were separated. In both samples the sediment contained significant amounts of Cs-137 and Cs-134 indicating the presence of fallout from the Chernobyl reactor accident. There was no cesium activity observed in the porewater at a minimum detectable level of 0,008 Bq/ml. 32 refs., 5 figs., 7 tabs.
Physical Description
32 pages
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OSTI; NTIS; INIS; GPO Dep.
Subjects
Keywords
- Accidents
- Alkali Metal Isotopes
- Beta Decay Radioisotopes
- Beta-Minus Decay Radioisotopes
- Black Sea
- Cesium 134
- Cesium 137
- Cesium Isotopes
- Chernobylsk-4 Reactor
- Ecological Concentration
- Electron Capture Radioisotopes
- Enriched Uranium Reactors
- Environmental Transport
- Fallout
- Graphite Moderated Reactors
- Hazards
- Health Hazards
- Hours Living Radioisotopes
- Hydrogen Compounds
- Intermediate Mass Nuclei
- Internal Conversion Radioisotopes
- Isomeric Transi
- Isotopes
- Lwgr Type Reactors
- Mass Transfer
- Nuclei
- Odd-Even Nuclei
- Oxygen Compounds
- Power Reactors
- Radiation Hazards
- Radioactivity
- Radioecological Concentration
- Radioisotopes
- Radionuclide Migration
- Reactor Accidents
- Reactors
- Seas
- Sediments
- Surface Waters
- Thermal Reactors
- Water
- Water Cooled Reactors
- Years Living Radioisotopes 220900* -- Nuclear Reactor Technology-- Reactor Safety
STI Subject Categories
- 22 General Studies Of Nuclear Reactors
- 54 Environmental Sciences
- 540130 -- Environment, Atmospheric-- Radioactive Materials Monitoring & Transport-- (1990-)
- 540230 -- Environment, Terrestrial-- Radioactive Materials Monitoring & Transport-- (1990-)
- 540330 -- Environment, Aquatic-- Radioactive Materials Monitoring & Transport-- (1990-)
Source
- 1. international ocean pollution symposium, Magaquez (Puerto Rico), 28 Apr 1991
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- Other: DE91015653
- Report No.: BNL-46348
- Report No.: CONF-9104279--1
- Grant Number: AC02-76CH00016
- Office of Scientific & Technical Information Report Number: 5702750
- Archival Resource Key: ark:/67531/metadc1084944
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- April 23, 1991
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- Feb. 10, 2018, 10:06 p.m.
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- Jan. 14, 2020, 6:21 p.m.
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Fuhrmann, M.; Pietrzak, R. (Brookhaven National Lab., Upton, NY (USA)); Neiheisel, J. & Dyer, R. (Environmental Protection Agency, Washington, DC (USA)). Partitioning between sediment and porewater of radiocesium from Chernobyl fallout, article, April 23, 1991; Upton, New York. (https://digital.library.unt.edu/ark:/67531/metadc1084944/: accessed May 14, 2024), University of North Texas Libraries, UNT Digital Library, https://digital.library.unt.edu; crediting UNT Libraries Government Documents Department.