Direct Conversion of Methane to Methanol in a Non-Isothermal Catalytic Membrane Reactor

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The direct partial oxidation of CH{sub 4} to CH{sub 3}OH has been studied in a non-permselective, non-isothermal catalytic membrane reactor system. A cooling tube introduced coaxially inside a tubular membrane reactor quenches the product stream rapidly so that further oxidation of CH{sub 3}OH is inhibited. Selectivity for CH{sub 3}OH formation is significantly higher with quenching than in experiments without quenching. For CH{sub 4} conversion of 4% to 7% CH{sub 3}OH selectivity is 40% to 50% with quenching and 25% to 35% without quenching.

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8 p.

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Noble, R. D. & Falconer, J. L. December 31, 1993.

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This article is part of the collection entitled: Office of Scientific & Technical Information Technical Reports and was provided by the UNT Libraries Government Documents Department to the UNT Digital Library, a digital repository hosted by the UNT Libraries. It has been viewed 12 times. More information about this article can be viewed below.

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The direct partial oxidation of CH{sub 4} to CH{sub 3}OH has been studied in a non-permselective, non-isothermal catalytic membrane reactor system. A cooling tube introduced coaxially inside a tubular membrane reactor quenches the product stream rapidly so that further oxidation of CH{sub 3}OH is inhibited. Selectivity for CH{sub 3}OH formation is significantly higher with quenching than in experiments without quenching. For CH{sub 4} conversion of 4% to 7% CH{sub 3}OH selectivity is 40% to 50% with quenching and 25% to 35% without quenching.

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8 p.

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OSTI as DE94006023; Paper copy available at OSTI: phone, 865-576-8401, or email, reports@adonis.osti.gov

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  • Fuels technology contractors` review meeting,Morgantown, WV (United States),16-18 Nov 1993

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  • Other: DE94006023
  • Report No.: DOE/MC/27115--94/C0284
  • Report No.: CONF-931156--13
  • Grant Number: FG21-90MC27115
  • Office of Scientific & Technical Information Report Number: 10120166
  • Archival Resource Key: ark:/67531/metadc1276479

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  • December 31, 1993

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  • Oct. 12, 2018, 6:44 a.m.

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  • Jan. 15, 2021, 5:43 p.m.

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Noble, R. D. & Falconer, J. L. Direct Conversion of Methane to Methanol in a Non-Isothermal Catalytic Membrane Reactor, article, December 31, 1993; Boulder, Colorado. (https://digital.library.unt.edu/ark:/67531/metadc1276479/: accessed July 15, 2024), University of North Texas Libraries, UNT Digital Library, https://digital.library.unt.edu; crediting UNT Libraries Government Documents Department.

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