Photoinitiated electron transfer in multichromophoric species: Synthetic tetrads and pentads

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This research project involves the design, synthesis and study of molecules which mimic many of the important aspects of photosynthetic electron and energy transfer. The knowledge gained from the study of synthetic model systems which abstract features of the natural photosynthetic apparatus can be used to design artificial photosynthetic systems which employ the basic physics and chemistry of photosynthesis to help meet mankind's energy needs. More specifically, the proposed models are designed to mimic the following aspects of natural photosynthetic multistep electron transfer: electron donation from a tetrapyrrole excited singlet state, electron transfer between tetrapyrroles, electron transfer from tetrapyrroles to … continued below

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19 pages

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Gust, J.D. Jr. & Moore, T.A. April 12, 1988.

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Description

This research project involves the design, synthesis and study of molecules which mimic many of the important aspects of photosynthetic electron and energy transfer. The knowledge gained from the study of synthetic model systems which abstract features of the natural photosynthetic apparatus can be used to design artificial photosynthetic systems which employ the basic physics and chemistry of photosynthesis to help meet mankind's energy needs. More specifically, the proposed models are designed to mimic the following aspects of natural photosynthetic multistep electron transfer: electron donation from a tetrapyrrole excited singlet state, electron transfer between tetrapyrroles, electron transfer from tetrapyrroles to quinones, and electron transfer between quinones with different redox properties.

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19 pages

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OSTI; NTIS; GPO Dep.

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Office of Scientific & Technical Information Technical Reports

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  • April 12, 1988

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  • Feb. 10, 2018, 10:06 p.m.

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  • Sept. 9, 2020, 5:37 p.m.

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Gust, J.D. Jr. & Moore, T.A. Photoinitiated electron transfer in multichromophoric species: Synthetic tetrads and pentads, report, April 12, 1988; Tempe, Arizona. (https://digital.library.unt.edu/ark:/67531/metadc1084502/: accessed July 16, 2024), University of North Texas Libraries, UNT Digital Library, https://digital.library.unt.edu; crediting UNT Libraries Government Documents Department.

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