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in subjects: "Chlorides"

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Pion correlations as a function of atomic mass in heavy ion collisions

The method of two pion interferometry was used to obtain source-size and lifetime parameters for the pions produced in heavy ion collisions. The systems used were 1.70 {center dot} A GeV {sup 56}Fe + Fe, 1.82 {center dot} A GeV {sup 40}Ar + KCl and 1.54 {center dot} A GeV {sup 93}Nb + Nb, allowing for a search for dependences on the atomic number. Two acceptances (centered, in the lab., at {approximately} 0{degrees} and 45{degrees}) were used for each system, allowing a search for dependences o… more

Date: November 26, 1989

Creator: Chacon, A.D.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Alkali sorber (RABSAM), September 1, 1990--August 30, 1991

The objective of this work is to develop a regenerable activated-bauxite sorber alkali monitor that requires no high-temperature/high-pressure sampling line for the reliable in situ measurement of alkali-vapor concentration in the exhaust from the pressurized fluidized-bed combustion of coal. 11 refs., 2 figs., 1 tab.

Date: January 1, 1991

Creator: Lee, S. H. D. & Swift, M. W.

Item Type: Article

Partner: UNT Libraries Government Documents Department

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Exploring novel silicon-containing polymers---From preceramic polymers to conducting polymers with nonlinear optical properties

Several new types of silicon-containing preceramic polymers, i.e., poly(diorganosilacetylene) and poly(diorganosilvinylene) have been synthesized with molecular weights from 10,000 to 120,000. These polymers could be thermally converted to SiC with a moderate to high char yields. Ready solubility and good processability made these types of polymers attractive in their applications to ceramics. The thermal polymerization of diethynyldiphenyl-silane, which was reported in 1968 to afford poly(diph… more

Date: October 7, 1991

Creator: Pang, Yi.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Recovery of plutonium and americium from chloride salt wastes by solvent extraction

Plutonium and americium can be recovered from aqueous waste solutions containing a mixture of HCl and chloride salt wastes by the coupling of two solvent extraction systems: tributyl phosphate (TBP) in tetrachloroethylene (TCE) and octyl(phenyl)-N,N-diisobutylcarbamoylmethylphosphine oxide (CMPO) in TCE. In the flowsheet developed, the salt wastes are dissolved in HCl, the Pu(III) is oxidized to the IV state with NaClO/sub 2/ and recovered in the TBP-TCE cycle, and the Am is then removed from t… more

Date: January 1, 1987

Creator: Reichley-Yinger, L. & Vandegrift, G.F.

Item Type: Article

Partner: UNT Libraries Government Documents Department

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The bioenergetics of salt tolerance

The aim of this project was to try to understand the adaptive mechanisms that organisms develop in order to respond to a sudden transformation in their environment to a salt shock.'' To study this problem we used a fresh water oxygenic photosynthetic cyanobacterium known as Synecoccus 6311. This organism suffers injury after this sudden exposure to high concentrations of sodium chloride equivalent to or even higher than that in sea water. Yet they are able to re-establish their photosynthetic a… more

Date: January 1, 1991

Creator: Packer, L.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Magnetic measurements of the transuranium elements. Progress report, January 1-December 31, 1986

Magnetic measurements have been made on polycrystalline CfCl/sub 3/ in both a hexagonal and orthorhombic crystal form. The magnetic properties were studied as a function of crystal structure by converting the same sample back and forth from one form to the other. In a continuation of a study of the magnetic transition temperature as a function of actinide-actinide separation of the curium pnictide series we have undertaken magnetic measurements on curium bismuthide during this contract period. … more

Date: September 1, 1986

Creator: Nave, S.E.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Elastic and Plastic Strains and the Stress Corrosion Cracking of Austenitic Stainless Steels. Progress Report, April 30, 1977--December 30, 1977

A newly developed test environment based on NaCl, Na/sub 2/SO/sub 4/, and HCl has provided some insight to several aspects of SCC in a transformable austenitic stainless steel. Current vs. time curves indicated the presence of the formation of a ''protective'' film which drastically reduced the anodic current leading to failure. This film, not indicated by the polarization curves, is subject to highly localized damage such as pitting. Thus, although it allows only very small corrosion currents,… more

Date: January 1, 1978

Creator: Troiano, A. R.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Nuclear magnetic resonance study of metallic scandium chlorides

The /sup 45/Sc nuclear magnetic resonance was studied in samples having the general composition CsSc/sub x/Cl/sub 3/ (0.67 less than or equal to x less than or equal to 1.0) in the CsCl-ScCl/sub 3/-Sc system. In particular the structure of CsScCl/sub 3/ suggests that it may be a one-dimensional conductor, and an attempt was therefore made to detect the occurrence of a metal-insulator transition of the type characteristic of one-dimensional conductors. Conventional crossed-coil (nuclear inductio… more

Date: April 1, 1978

Creator: McMullen, T.P.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Long-term leaching of irradiated spent fuel

Spent Light Water Reactor (LWR) fuel with burnups of 9, 28 and 54 MWd/kg U were leach tested at 25/sup 0/C in deionized water in a Paige apparatus. No discernible differences in leach rates were observed due to burnup. Additionally, the 28 MWd/kg U fuel was IAEA leach tested in five different leachants using the IAEA method. Deionized water gave the highest leach rates and a calcium chloride solution gave the lowest leach rates. An accelerated leaching period was observed during the Paige leach… more

Date: January 1, 1979

Creator: Katayama, Y. B. & Bradley, D. J.

Item Type: Article

Partner: UNT Libraries Government Documents Department

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Vapor phase spectroscopy of complex lanthanide halide--aluminum halide molecular species

The absorption spectrum of ErCl/sub 3/ (AlCl/sub 3/)/sub x/ vapor complex was measured and analyzed using the Judd-Ofelt theory. Structural correlations in other AlCl/sub 3/ vapor complexes and radiation emission are discussed. Fluorescence of TbCl/sub 3/ (AlCl/sub 3/)/sub x/ vapor complex and in the NdCl/sub 3/ (AlCl/sub 3/)/sub x/ system were studied. (DLC)

Date: January 1, 1977

Creator: Carnall, W T; Hessler, J P; Williams, C W & Hoekstra, H R

Item Type: Article

Partner: UNT Libraries Government Documents Department

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Removal of silica from Raft River geothermal water

Lack of sufficient quantities of clean surface or near-surface water at Raft River for cooling purposes dictates that cooled geothermal fluid, effluent from the Raft River 5 MW(e) Pilot Power Plant, must also be used as condenser coolant. Prior testing revealed that a water-treatment system would be required to reduce silica and calcium concentrations of the cooling fluid. The water-treatment system specified was to use dolomitic lime for both pH adjustment and source of magnesium. The dolomiti… more

Date: June 1, 1980

Creator: Suciu, D. F. & Miller, R. L.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Tilt-pour melt-caster for encapsulation of radioactive cesium

Use of the tilt-pour melt-caster makes distinct improvements in the cesium encapsulation process. Compared to the vacuum castings system now in use, the tilt-pour equipment requires no reliance on heat-traced transfer lines, less sealing pressure for capsule filling, is less corrosive to capsules and is easier to repair. From the results of the extensive development program, it is concluded that the tilt-pour melt-caster can be operated to meet the cesium encapsulation production and maintenanc… more

Date: January 1, 1977

Item Type: Article

Partner: UNT Libraries Government Documents Department

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Chemical Technology Division, Unit Operations Section Monthly Progress Report, May 1961

The experimental results on the oxidation of H from a He stream with CuO pellets were very close to the predicted behavior based on the mathematical model. Experimental measurements of uranyl sulfate loading rates on chloride equilibrated resin showed little variation with solution concentrations. A tentative flowsbeet was proposed for cost analysis of processing a Pebble Bed Reactor. A U-Zr plate was dissolved in nitrate-free Zirflex solution. An authentic TRIGA prototype was processed in engi… more

Date: December 26, 1961

Creator: Whatley, M. E.; Haas, P. A.; Horton, R. W.; Ryon, A. D.; Suddath, J. C. & Watson, C. D.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Low-cost solar array project. Task I. Silicon material. Investigation of the hydrogenation of SiCl/sub 4/

Reaction kinetic measurements on the hydrochlorination of SiCl/sub 4/ and m.g. silicon metal were last reported as a function of reaction temperature, reactor pressure, H/sub 2//SiCl/sub 4/ ratio and silicon metal particle size distribution, 3 SiCl/sub 4/ + 2 H/sub 2/ + Si reversible 4 SiHCl/sub 3/. The effect of impurities in the m.g. silicon metal on the rate of this reaction has been investigated in this quarter. The m.g. silicon was replaced with high purity, electronic grade silicon metal … more

Date: October 7, 1980

Creator: Mui, J. Y. P. & Seyferth, D.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Efficient forward conversion in a Raman generator

Stimulated Raman scattering of an XeCl laser at 308 nm in a high pressure H/sub 2/ cell shows anomalously high conversion into first Stokes (S1) when a pumping geometry with a Fresnel number near unity is used. Specifically a quantum efficiency of 88% is obtained into S1. Comparison with a plane-wave model indicates that a theory including diffraction and 4-wave mixing may be necessary to understand the anomalous holdoff of the second Stokes component. 10 references.

Date: January 1, 1984

Creator: Carlsten, J.L.; Telle, J.M. & Wenzel, R.G.

Item Type: Article

Partner: UNT Libraries Government Documents Department

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The GALLEX Project

The GALLEX collaboration aims at the detection of solar neutrinos in a radiochemical experiment employing 30 tons of Gallium in form of concentrated aqueous Gallium-chloride solution. The detector is primarily sensitive to the otherwise inaccessible pp-neutrinos. Details of the experiment have been repeatedly described before. Here we report the present status of implementation in the Laboratori Nazionali del Gran Sasso (Italy). So far, 12.2 tons of Gallium are at hand. The present status of de… more

Date: January 1, 1989

Creator: Kirsten, T. (Max-Planck-Institut fuer Kernphysik, Heidelberg (Germany, F.R.))

Item Type: Article

Partner: UNT Libraries Government Documents Department

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EXTRACTION OF NEPTUNIUM FROM ACIDIC SOLUTIONS BY ORGANIC NITROGEN AND PHOSPHORUS COMPOUNDS

Neptunium distribution coefficients from acid nitrate, chloride, and sulfate solutions by several organic nitiogen and phosphorus compounds were measured as functions of several extraction variables, including neptunium valence, acid and salt concentration, and reagent concentration. Extractability by all the reagents varied in the order Np(IV)> Np(VI)>> Np(V). Except for primary amines, all reagents extracted Np(IV) much more strongly from nitrate than sulfate solutions. Among organonitrogen c… more

Date: October 19, 1961

Creator: Weaver, B.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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MAP3S precipitation chemistry network. Third periodic summary report, July 1978-December 1979

The MAP3S Precipitation Chemistry Network consists of eight collection sites in the northeastern United States. Precipitation event samples are collected by cooperating site operators, using specially developed sampling equipment. In this, the third periodic summary report, are listed field and concentration data for the period July 1, 1978 to December 31, 1979. Over three years' samples have been collected at most of the sites, which went into operation between September 1976 and October 1978.… more

Date: May 1, 1980

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Recovery of platinum from concentrated sodium chloride brine by electrodeposition on vitreous carbon

The voltammetric characteristics of Pt(II) and Pt(IV) have been examined at a vitreous carbon electrode in slightly acidic 3M (approx. 15 wt %) NaCl solutions. Pt(IV) is reduced to Pt(II) at approx. 0 V and Pt(II) is reduced to Pt(0) at approx. -0.5 V vs Ag-AgCl. The rate of deposition of platinum metal at -0.5 V is very low on bare carbon, but increases as the coverage of platinum increases. The potential at which hydrogen is evolved in this medium is approx. -0.85 V. A technique has been test… more

Date: January 1, 1984

Creator: Harrar, J.E. & Stephens, F.B.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Excited state absorption measurements of Sm sup 2+ in CaF sub 2 , SrF sub 2 , and SrCl sub 2

We measured the pump-probe spectrum of the Sm{sup 2+} ion in three materials: CaF{sub 2}, SrF{sub 2}, and SrCl{sub 2}. The onset of the observed prominent excited-state absorption band is consistent with an electrostatic model for impurity levels in a solid-state material. 15 refs., 4 figs., 1 tab.

Date: April 1, 1991

Creator: Lawson, J. K.; Lee, H. W. H.; Payne, S. A. (Lawrence Livermore National Lab., CA (United States)) & Boatner, L. A. (Oak Ridge National Lab., TN (United States))

Item Type: Article

Partner: UNT Libraries Government Documents Department

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Potential geothermal resources in Hawaii: a preliminary regional survey. Phase I, final report

A regional geothermal resource assessment has been conducted for the major islands in the Hawaiian chain. The assessment was made through the compilation and evaluation of the readily accessible geological, geochemical, and geophysical data for the Hawaiian Archipelago that have been acquired during the last two decades. The geologic criteria used in the identification of possible geothermal reservoirs were age and location of most recent volcanism on the island and the geologic structure of ea… more

Date: June 1, 1979

Creator: Thomas, D.; Cox, M.; Erlandson, D. & Kajiwara, L.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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Basic studies of a gas-jet-coupled ion source for on-line isotope separation

A hollow-cathode ion source was used in a gas-jet-coupled configuration to produce ion beams of fission products transported to it from a /sup 252/Cf fission source. Solid aerosols of NaCl and Ag were used effectively as activity carriers in the gas-jet system. Flat-plate skimmers provided an effective coupling of the ion source to the gas jet. Ge(Li) spectrometric measurements of the activity deposited on an ion-beam collector relative to that deposited on a pre-skimmer collector were used to … more

Date: January 1, 1980

Creator: Anderl, R. A.; Novick, V. J. & Greenwood, R. C.

Item Type: Article

Partner: UNT Libraries Government Documents Department

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Physicochemical basis of the Na-K-Ca geothermometer

Regular changes in solution composition were observed experimentally during granite reaction with dilute NaCl (+CaCl/sub 2/) solutions; these changes closely follow the empirical Na-K-Ca geothermometer relationship. Initial minerals forming the granite (quartz, plagioclase, K-feldspar, and biotite) were etched by the reactions. Alteration phases formed include calcium-zeolite at <300/sup 0/C, feldspar overgrowths at >300/sup 0/C, and minor amounts of clay and calcsilicate at all temperatures. A… more

Date: August 1, 1986

Creator: Janecky, D. R.; Charles, R. W.; Bayhurst, Gregory K. & Benjamin, T. M.

Item Type: Report

Partner: UNT Libraries Government Documents Department

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SALT PHASE CHLORINATION OF REACTOR FUELS. III. CATALYZED DISSOLUTION OF URANIUM DIOXIDE IN LEAD CHLORIDE-CHLORIDE SYSTEMS

The rapid dissolution of uranium dioxide is described, wherein copper is added to molten lead chloride at 550 deg C. and chlorine is passed through the melt. The integral dissolution of zirconium-clad uranium dioxide fuels is also described. The dissolution rate of uranium dioxide is directly proportional to the concentration of cuprous chloride if an excess of chlorine is used; the value for the rate constant is approximately 100 mg (UO/sub 2/) cm/sup -2/ min/sup -1/ (CuCl molality). The urani… more

Date: February 1, 1962

Creator: Vander Wall, E. M.; Bauer, D. L. & Hahn, H. T.

Item Type: Report

Partner: UNT Libraries Government Documents Department