An Alternative Model for Electron Correlation in Pu
Description:
Using a density functional theory based approach that treats the 5f electrons relativistically, a Pu electronic structure with zero net magnetic moment is obtained, where the 5f orbital and 5f spin moments cancel each other. By combining the spin and orbital specific densities of states with state, spin and polarization specific transition moments, it is possible to reconstruct the experimentally observed photoemission spectra from Pu. Extrapolating to a spin-resolving Fano configuration, it is…
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Date:
October 23, 2007
Creator:
Yu, S.; Tobin, J. & Soderlind, P.
Partner:
UNT Libraries Government Documents Department