Spin Properties of Transition-Metallorganic Self-Assembled Molecules Page: 35 of 47
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(a)
.0
.0
-4 (b)
4
0 1
-4 (C)
-4
1x10-5 2x10-
t (s)1.00 -
0.00
-1.00U)
1x109
0
5x101 d0
(f) 1x10 0
0
-1x105
0 2x10 4x106
t (s)Figure 17: Transient relative conductance change due to longitudinal and transverse
spin relaxation in N@C60. Panel (a) describes the free relaxation of Sz after a r-pulse,
and panels (b) and (c) plot the corresponding evolution of Ag/go with spin-flip hopping
forbidden (A = 0) and spin-flip hopping allowed (A1 = A2 = 0.05), respectively. Panels
(d) describes the damped precession of transverse spin components, S, (red line) and Sy
(green line) after a r/2-pulse followed by an on-resonance microwave Hl = H1 (cos wote, +
sin wotey). Panels (e) and (f) plot the corresponding Ag/go as a function of time with
A = 0 and Al = A2 = 0.05, respectively. T = lOT2 = 10-5 s. Other parameters are the
same as in Fig. 16.34
(d) _
J-
- -d
- (e) -0
VJN -1
2x1(
0
d1 x10
2x1(
0
d 1x10
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Yu, Zhi Gang. Spin Properties of Transition-Metallorganic Self-Assembled Molecules, report, June 30, 2010; United States. (https://digital.library.unt.edu/ark:/67531/metadc1014357/m1/35/: accessed July 16, 2024), University of North Texas Libraries, UNT Digital Library, https://digital.library.unt.edu; crediting UNT Libraries Government Documents Department.