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Carbon Dioxide Capture From Flue Gas Using Dry Regenerable Sorbents Quarterly Technical Progress Report: April-June 2003

Description: This report describes research conducted between April 1, 2003 and June 30, 2003 on the use of dry regenerable sorbents for concentration of carbon dioxide from flue gas. Grade 1 sodium bicarbonate performed similarly to grade 5 sodium bicarbonate in fixed bed testing in that activity improved after the first carbonation cycle and did not decline over the course of 5 cycles. Thermogravimetric analysis indicated that sodium bicarbonate sorbents produced by calcination of sodium bicarbonate are s… more
Date: August 1, 2003
Creator: Green, David A.; Turk, Brian S.; Portzer, Jeffrey W.; Gupta, Raghubir P.; McMichael, William J.; Liang, Ya et al.
Partner: UNT Libraries Government Documents Department
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Carbon Dioxide Capture From Flue Gas Using Dry Regenerable Sorbents Quarterly Technical Progress Report: April-June 2004

Description: This report describes research conducted between April 1, 2004 and June 30, 2004 on the preparation and use of dry regenerable sorbents for removal of carbon dioxide from flue gas. Support materials and supported sorbents were prepared by spray drying. Sorbents consisting of 20 to 50% sodium carbonate on a ceramic support were prepared by spray drying in batches of approximately 300 grams. The supported sorbents exhibited greater carbon dioxide capture rates than unsupported calcined sodium bic… more
Date: July 1, 2004
Creator: Green, David A.; Turk, Brian S.; Portzer, Jeffrey W.; Gupta, Raghubir P.; McMichael, William J. & Nelson, Thomas
Partner: UNT Libraries Government Documents Department
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Carbon Dioxide Capture From Flue Gas Using Dry Regenerable Sorbents Quarterly Technical Progress Report: January-March 2004

Description: This report describes research conducted between January 1, 2004 and March 31, 2004 on the use of dry regenerable sorbents for removal of carbon dioxide from flue gas. RTI has produced laboratory scale batches (approximately 300 grams) of supported sorbents (composed of 20 to 40% sodium carbonate) with high surface area and acceptable activity. Initial rates of weight gain of the supported sorbents when exposed to a simulated flue gas exceeded that of 100% calcined sodium bicarbonate. One of th… more
Date: April 1, 2004
Creator: Green, David A.; Turk, Brian S.; Portzer, Jeffrey W.; Gupta, Raghubir P.; McMichael, William J. & Nelson, Thomas
Partner: UNT Libraries Government Documents Department
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Carbon Dioxide Capture From Flue Gas Using Dry Regenerable Sorbents Quarterly Technical Progress Report: January-March 2005

Description: This report describes research conducted between January 1, 2005 and March 31, 2005 on the use of dry regenerable sorbents for removal of carbon dioxide from flue gas. Engineered sorbents composed of sodium carbonate on a ceramic support were tested in a laboratory fluidized bed reactor system and found to be capable of essentially complete removal of carbon dioxide at 60 C in a short residence time. Upon breakthrough the sorbents can be thermally regenerated to recover essentially all of the a… more
Date: April 1, 2005
Creator: Green, David A.; Nelson, Thomas; Turk, Brian S.; Portzer, Jeffrey W. & Gupta, Raghubir P.
Partner: UNT Libraries Government Documents Department
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Carbon Dioxide Capture From Flue Gas Using Dry Regenerable Sorbents Quarterly Technical Progress Report: July-September 2002

Description: The objective of this project is to develop a simple and inexpensive process to separate CO{sub 2} as an essentially pure stream from a fossil fuel combustion system using a regenerable sorbent. The sorbents being investigated in this project are primarily alkali carbonates, and particularly sodium carbonate and potassium carbonate, which are converted to bicarbonates through reaction with carbon dioxide and water vapor. Bicarbonates are regenerated to carbonates when heated, producing a nearly… more
Date: October 1, 2002
Creator: Green, David A.; Turk, Brian S.; Portzer, Jeffrey W.; P.Gupta, Raghubir; McMichael, William J.; Liang, Ya et al.
Partner: UNT Libraries Government Documents Department
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Carbon Dioxide Capture From Flue Gas Using Dry Regenerable Sorbents Quarterly Technical Progress Report: July-September 2004

Description: Laboratory studies were conducted to investigate dry, regenerable, alkali carbonate-based sorbents for the capture of CO{sub 2} from power plant flue gas. Electrobalance, fixed-bed and fluid-bed reactors were used to examine both the CO{sub 2} capture and sorbent regeneration phases of the process. Sodium carbonate-based sorbents (calcined sodium bicarbonate and calcined trona) were the primary focus of the testing. Supported sodium carbonate and potassium carbonate sorbents were also tested. S… more
Date: November 1, 2004
Creator: Green, David A.; Turk, Brian S.; Portzer, Jeffrey W.; Gupta, Raghubir P.; McMichael, William J. & Nelson, Thomas
Partner: UNT Libraries Government Documents Department
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Carbon Dioxide Capture From Flue Gas Using Dry Regenerable Sorbents Quarterly Technical Progress Report: October-December 2002

Description: The objective of this project is to develop a simple and inexpensive process to separate CO{sub 2} as an essentially pure stream from a fossil fuel combustion system using a regenerable sorbent. The sorbents being investigated in this project are primarily alkali carbonates, and particularly sodium carbonate and potassium carbonate, which are converted to bicarbonates or intermediate salts through reaction with carbon dioxide and water vapor. Bicarbonates are regenerated to carbonates when heat… more
Date: January 1, 2003
Creator: Green, David A.; Turk, Brian S.; Portzer, Jeffrey W.; Gupta, Raghubir P.; McMichael, William J.; Liang, Ya et al.
Partner: UNT Libraries Government Documents Department
open access

Carbon Dioxide Capture From Flue Gas Using Dry Regenerable Sorbents Quarterly Technical Progress Report: October-December 2004

Description: This report describes research conducted between October 1, 2004 and December 31, 2004 on the use of dry regenerable sorbents for removal of carbon dioxide from flue gas. Two supported sorbents were tested in a bench scale fluidized bed reactor system. The sorbents were prepared by impregnation of sodium carbonate on to an inert support at a commercial catalyst manufacturing facility. One sorbent, tested through five cycles of carbon dioxide sorption in an atmosphere of 3% water vapor and 0.8 t… more
Date: January 1, 2005
Creator: Green, David A.; Turk, Brian S.; Portzer, Jeffrey W.; Nelson, Thomas & Gupta, Raghubir P.
Partner: UNT Libraries Government Documents Department
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