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Determination of the Azimuthal Asymmetry of Deuteron Photodisintegration in the Energy Region E{sub {gamma}} = 1.1 - 2.3 GeV

Description: Deuteron photodisintegration is a benchmark process for the investigation of the role of quarks and gluons in nuclei. Existing theoretical models of this process describe the available cross sections with the same degree of success. Therefore, spin-dependent observables are crucial for a better understanding of the underlying dynamical mechanisms. However, data on the induced polarization (P{sub y}), along with the polarization transfers (C{sub x'} and C{sub z'} ), have been shown to be insensitive to differences between theoretical models. On the other hand, the beam-spin asymmetry {Sigma} is predicted to have a large sensitivity and is expected to help in identifying the energy at which the transition from the hadronic to the quark-gluon picture of the deuteron takes place. Here, the work done to determine the experimental values of the beam-spin asymmetry in deuteron photodisintegration for photon energies between 1.1 – 2.3 GeV is presented. The data were taken with the CLAS at the Thomas Jefferson National Accelerator Facility during the g13 experiment. Photons with linear polarization of ~80% were produced using the coherent bremsstrahlung facility in Hall B. The work done by the author to calibrate a specific detector system, select deuteron photodisintegration events, study the degree of photon polarization, and finally determine the azimuthal asymmetry and any systematic uncertainties associate with it, is comprehensively explained. This work shows that the collected data provide the kinematic coverage and statistics to test the available QCD-based models. The results of this study show that the available theoretical models in their current state do not adequately predict the azimuthal asymmetry in the energy region 1.1 – 2.3 GeV.
Date: May 20, 2012
Creator: Zachariou, Nicholas
Partner: UNT Libraries Government Documents Department

Developing nanotechnology for biofuel and plant science applications

Description: This dissertation presents the research on the development of mesoporous silica based nanotechnology for applications in biofuels and plant science. Mesoporous silica nanoparticles (MSNs) have been the subject of great interest in the last two decades due to their unique properties of high surface area, tunable pore size and particle morphology. The robust nature of the silica framework is easily functionalized to make the MSNs a promising option for selective separations. Also, the independent channels that form the pores of MSN have been exploited in the use of particles as platforms for molecular delivery. Pore size and organic functionality are varied to identify the ideal adsorbent material for free fatty acids (FFAs). The resulting material is able to sequester FFAs with a high degree of selectivity from a simulated solution and microalgal oil. The recyclability and industrial implications are also explored. A continuation of the previous material, further tuning of MSN pore size was investigated. Particles with a smaller diameter selectively sequester polyunsaturated free fatty acids (PUFAs) over monounsaturated FFAs and saturated FFAs. The experimental results were verified with molecular modeling. Mesoporous silica nanoparticle materials with a pore diameter of 10 nm (MSN-10) were decorated with small gold nanoparticles. The resulting materials were shown to deliver proteins and DNA into plant cells using the biolistic method.
Date: June 20, 2012
Creator: Valenstein, Justin
Partner: UNT Libraries Government Documents Department

Hot electron dynamics in graphene

Description: Graphene, a two-dimensional (2D) honeycomb structure allotrope of carbon atoms, has a long history since the invention of the pencil [Petroski (1989)] and the linear dispersion band structure proposed by Wallace [Wal]; however, only after Novoselov et al. successively isolated graphene from graphite [Novoselov et al. (2004)], it has been studied intensively during the recent years. It draws so much attentions not only because of its potential application in future electronic devices but also because of its fundamental properties: its quasiparticles are governed by the two-dimensional Dirac equation, and exhibit a variety of phenomena such as the anomalous integer quantum Hall effect (IQHE) [Novoselov et al. (2005)] measured experimentally, a minimal conductivity at vanishing carrier concentration [Neto et al. (2009)], Kondo effect with magnetic element doping [Hentschel and Guinea (2007)], Klein tunneling in p-n junctions [Cheianov and Fal’ko (2006), Beenakker (2008)], Zitterbewegung [Katsnelson (2006)], and Schwinger pair production [Schwinger (1951); Dora and Moessner (2010)]. Although both electron-phonon coupling and photoconductivity in graphene also draws great attention [Yan et al. (2007); Satou et al. (2008); Hwang and Sarma (2008); Vasko and Ryzhii (2008); Mishchenko (2009)], the nonequilibrium behavior based on the combination of electronphonon coupling and Schwinger pair production is an intrinsic graphene property that has not been investigated. Our motivation for studying clean graphene at low temperature is based on the following effect: for a fixed electric field, below a sufficiently low temperature linear eletric transport breaks down and nonlinear transport dominates. The criteria of the strength of this field [Fritz et al. (2008)] is eE = T2/~vF (1.1) For T >√eE~vF the system is in linear transport regime while for T <√eE~vF the system is in nonlinear transport regime. From the scaling’s point of view, at the nonlinear transport regime the temperature T and electric field E are also ...
Date: October 20, 2011
Creator: Ling, Meng-Cheieh
Partner: UNT Libraries Government Documents Department

First principles analysis of lattice dynamics for Fe-based superconductors and entropically-stabilized phases

Description: Modern calculations are becoming an essential, complementary tool to inelastic x-ray scattering studies, where x-rays are scattered inelastically to resolve meV phonons. Calculations of the inelastic structure factor for any value of Q assist in both planning the experiment and analyzing the results. Moreover, differences between the measured data and theoretical calculations help identify important new physics driving the properties of novel correlated systems. We have used such calculations to better and more e#14;ciently measure the phonon dispersion and elastic constants of several iron pnictide superconductors. This dissertation describes calculations and measurements at room temperature in the tetragonal phase of CaFe{sub 2}As{sub 2} and LaFeAsO. In both cases, spin-polarized calculations imposing the antiferromagnetic order present in the low-temperature orthorhombic phase dramatically improves the agreement between theory and experiment. This is discussed in terms of the strong antiferromagnetic correlations that are known to persist in the tetragonal phase. In addition, we discuss a relatively new approach called self-consistent ab initio lattice dynamics (SCAILD), which goes beyond the harmonic approximation to include phonon-phonon interactions and produce a temperature-dependent phonon dispersion. We used this technique to study the HCP to BCC transition in beryllium.
Date: July 20, 2012
Creator: Hahn, Steven
Partner: UNT Libraries Government Documents Department

Unorthodox theoretical methods

Description: The use of the ReaxFF force field to correlate with NMR mobilities of amine catalytic substituents on a mesoporous silica nanosphere surface is considered. The interfacing of the ReaxFF force field within the Surface Integrated Molecular Orbital/Molecular Mechanics (SIMOMM) method, in order to replicate earlier SIMOMM published data and to compare with the ReaxFF data, is discussed. The development of a new correlation consistent Composite Approach (ccCA) is presented, which incorporates the completely renormalized coupled cluster method with singles, doubles and non-iterative triples corrections towards the determination of heats of formations and reaction pathways which contain biradical species.
Date: June 20, 2012
Creator: Nedd, Sean
Partner: UNT Libraries Government Documents Department

Biomolecular Assembly of Gold Nanocrystals

Description: Over the past ten years, methods have been developed to construct discrete nanostructures using nanocrystals and biomolecules. While these frequently consist of gold nanocrystals and DNA, semiconductor nanocrystals as well as antibodies and enzymes have also been used. One example of discrete nanostructures is dimers of gold nanocrystals linked together with complementary DNA. This type of nanostructure is also known as a nanocrystal molecule. Discrete nanostructures of this kind have a number of potential applications, from highly parallel self-assembly of electronics components and rapid read-out of DNA computations to biological imaging and a variety of bioassays. My research focused in three main areas. The first area, the refinement of electrophoresis as a purification and characterization method, included application of agarose gel electrophoresis to the purification of discrete gold nanocrystal/DNA conjugates and nanocrystal molecules, as well as development of a more detailed understanding of the hydrodynamic behavior of these materials in gels. The second area, the development of methods for quantitative analysis of transmission electron microscope data, used computer programs written to find pair correlations as well as higher order correlations. With these programs, it is possible to reliably locate and measure nanocrystal molecules in TEM images. The final area of research explored the use of DNA ligase in the formation of nanocrystal molecules. Synthesis of dimers of gold particles linked with a single strand of DNA possible through the use of DNA ligase opens the possibility for amplification of nanostructures in a manner similar to polymerase chain reaction. These three areas are discussed in the context of the work in the Alivisatos group, as well as the field as a whole.
Date: May 20, 2005
Creator: Micheel, Christine Marya
Partner: UNT Libraries Government Documents Department


Description: Ion exchange column elution methods for the separation of americium and curium using tartrate and lactate solutions have been developed which are superior to citrate elutions. Tartrate elutions are suitable for slow separations and lactate elutions are satisfactory for general use where rapid separations are required. Fission and spallation products were isolated from Pu{sup 239} targets which had been bombarded with alpha particles of 21 to 37 Mev energy. Fission yield curves as well as fission and spallation excitation functions are presented and discussed in terms of odd-even and Z{sup 2}/A effects. The high cross sections observed for the (a, 2n) and (a, p2n) reactions were surprising results from this investigation. In the course of the Pu{sup 239} bombardments, studies of the decay schemes of Am{sup 240}, Cm{sup 240}, and Cm{sup 241} were undertaken. Decay energy and half-1ife information on all of the transmercury nuclides has been collected and systematized. Trends on the energy surface for alpha energies, beta energies, nucleon binding energies, and Bohr-Wheeler parameters are presented. These energy systematics have led to a complete tabulation of the masses of the isotopes of the elements above mercury. Predictions of nuclear properties are included for some isotopes of elements 99 through 103.
Date: April 20, 1954
Creator: Glass, Richard Alois
Partner: UNT Libraries Government Documents Department

An Analysis Framework Addressing the Scale and Legibility of Large Scientific Data Sets

Description: Much of the previous work in the large data visualization area has solely focused on handling the scale of the data. This task is clearly a great challenge and necessary, but it is not sufficient. Applying standard visualization techniques to large scale data sets often creates complicated pictures where meaningful trends are lost. A second challenge, then, is to also provide algorithms that simplify what an analyst must understand, using either visual or quantitative means. This challenge can be summarized as improving the legibility or reducing the complexity of massive data sets. Fully meeting both of these challenges is the work of many, many PhD dissertations. In this dissertation, we describe some new techniques to address both the scale and legibility challenges, in hope of contributing to the larger solution. In addition to our assumption of simultaneously addressing both scale and legibility, we add an additional requirement that the solutions considered fit well within an interoperable framework for diverse algorithms, because a large suite of algorithms is often necessary to fully understand complex data sets. For scale, we present a general architecture for handling large data, as well as details of a contract-based system for integrating advanced optimizations into a data flow network design. We also describe techniques for volume rendering and performing comparisons at the extreme scale. For legibility, we present several techniques. Most noteworthy are equivalence class functions, a technique to drive visualizations using statistical methods, and line-scan based techniques for characterizing shape.
Date: November 20, 2006
Creator: Childs, H R
Partner: UNT Libraries Government Documents Department

Production, Characterization, and Acceleration of Optical Microbunches

Description: Optical microbunches with a spacing of 800 nm have been produced for laser acceleration research. The microbunches are produced using a inverse Free-Electron-Laser (IFEL) followed by a dispersive chicane. The microbunched electron beam is characterized by coherent optical transition radiation (COTR) with good agreement to the analytic theory for bunch formation. In a second experiment the bunches are accelerated in a second stage to achieve for the first time direct net acceleration of electrons traveling in a vacuum with visible light. This dissertation presents the theory of microbunch formation and characterization of the microbunches. It also presents the design of the experimental hardware from magnetostatic and particle tracking simulations, to fabrication and measurement of the undulator and chicane magnets. Finally, the dissertation discusses three experiments aimed at demonstrating the IFEL interaction, microbunch production, and the net acceleration of the microbunched beam. At the close of the dissertation, a separate but related research effort on the tight focusing of electrons for coupling into optical scale, Photonic Bandgap, structures is presented. This includes the design and fabrication of a strong focusing permanent magnet quadrupole triplet and an outline of an initial experiment using the triplet to observe wakefields generated by an electron beam passing through an optical scale accelerator.
Date: June 20, 2008
Creator: Sears, Christopher M.S. & /SLAC, /Stanford U.
Partner: UNT Libraries Government Documents Department

Genotyping and Bioforensics of Ricinus communis

Description: The castor bean plant (Ricinus communis) is a member of the family Euphorbiaceae. In spite of its common name, the castor plant is not a true bean (i.e., leguminous plants belonging to the family, Fabaceae). Ricinus communis is native to tropical Africa, but because the plant was recognized for its production of oil with many desirable properties, it has been introduced and cultivated in warm temperate regions throughout the world (Armstrong 1999 and Brown 2005). Castor bean plants have also been valued by gardeners as an ornamental plant and, historically, as a natural rodenticide. Today, escaped plants grow like weeds throughout much of the southwestern United States, and castor seeds are even widely available to the public for order through the Internet. In this study, multiple loci of chloroplast noncoding sequence data and a few nuclear noncoding regions were examined to identify DNA polymorphisms present among representatives from a geographically diverse panel of Ricinus communis cultivated varieties. The primary objectives for this research were (1) to successfully cultivate castor plants and extract sufficient yields of high quality DNA from an assortment of castor cultivated varieties, (2) to use PCR and sequencing to screen available universal oligos against a small panel of castor cultivars, (3) to identify DNA polymorphisms within the amplified regions, and (4) to evaluate these DNA polymorphisms as appropriate candidates for assay development (see Figure 1). Additional goals were to design, test and optimize assays targeting any DNA polymorphisms that were discovered and to rapidly screen many castor cultivars to determine the amount of diversity present at that particular locus. Ultimately, the goal of this study was to construct a phylogeographic tree representing the genetic relationships present among Ricinus communis cultivars from diverse geographic regions. These research objectives were designed to test the hypothesis that cultivated varieties of ...
Date: November 20, 2006
Creator: Hinckley, A C
Partner: UNT Libraries Government Documents Department

Masters Thesis- Criticality Alarm System Design Guide with Accompanying Alarm System Development for the Radioisotope Production Laboratory in Richland, Washington

Description: A detailed instructional manual was created to guide criticality safety engineers through the process of designing a criticality alarm system (CAS) for Department of Energy (DOE) hazard class 1 and 2 facilities. Regulatory and technical requirements were both addressed. A list of design tasks and technical subtasks are thoroughly analyzed to provide concise direction for how to complete the analysis. An example of the application of the design methodology, the Criticality Alarm System developed for the Radioisotope Production Laboratory (RPL) of Richland, Washington is also included. The analysis for RPL utilizes the Monte Carlo code MCNP5 for establishing detector coverage in the facility. Significant improvements to the existing CAS were made that increase the reliability, transparency, and coverage of the system.
Date: December 20, 2009
Creator: Greenfield, Bryce A.
Partner: UNT Libraries Government Documents Department

Search for Lepton Flavour Violating Decays Tau -> l Ks with the BABAR Detector

Description: We present the search for the lepton flavour violating decay {tau} {yields} lK{sup 0}{sub s} with the BaBar experiment data. This process and many other lepton flavour violating {tau} decays, like {tau} {yields} {mu}{gamma} and {tau} {yields} lll, are one of the most promising channel to search for evidence of new physics. According to the Standard Model and the neutrino mixing parameters, branching fractions are estimated well below 10{sup -14}, but many models of new physics allow for branching fractions values close to the present experimental sensitivity. This analysis is based on a data sample of 469fb{sup -1} collected by BABAR detector at the PEP-II storage ring from 1999 to 2007, equivalent to 431 millions of {tau} pairs. the BABAR experiment, initially designed for studying CP violation in B mesons, has demonstrated to be one of the most suitable environments for studying {tau} decays. The tracking system, the calorimeter and the particle identification of BABAR, together with the knowledge of the {tau} initial energy, allow an extremely powerful rejection of background events that, for this analysis, is better than 10{sup -9}. Being {tau} {yields} lK{sup 0}{sub s} a decay mode without neutrinos, the signal {tau} decay can be fully reconstructed. Kinematical constraints are used in a fit that provides a decay tree reconstruction with a high resolution. For this analysis MC simulated events play a decisive role for estimating the signal efficiency and study the residual background. High statistics MC sample are produced simulating detector conditions for different periods of data collection, in order to reduce any discrepancies with the data. When discrepancies can not be removed, we perform studies to compute a correction factor or an estimation of systematic errors that need to be included in the final measurement. A significant improvement of the current result can be reached ...
Date: March 20, 2009
Creator: Cenci, Riccardo
Partner: UNT Libraries Government Documents Department

Fast Ignition Experimental and Theoretical Studies

Description: We are becoming dependent on energy more today than we were a century ago, and with increasing world population and booming economies, sooner or later our energy sources will be exhausted. Moreover, our economy and welfare strongly depends on foreign oil and in the shadow of political uncertainties, there is an urgent need for a reliable, safe, and cheap energy source. Thermonuclear fusion, if achieved, is that source of energy which not only will satisfy our demand for today but also for centuries to come. Today, there are two major approaches to achieve fusion: magnetic confinement fusion (MFE) and inertial confinement fusion (ICF). This dissertation explores the inertial confinement fusion using the fast ignition concept. Unlike the conventional approach where the same laser is used for compression and ignition, in fast ignition separate laser beams are used. This dissertation addresses three very important topics to fast ignition inertial confinement fusion. These are laser-to-electron coupling efficiency, laser-generated electron beam transport, and the associated isochoric heating. First, an integrated fast ignition experiment is carried out with 0.9 kJ of energy in the compression beam and 70 J in the ignition beam. Measurements of absolute K{sub {alpha}} yield from the imploded core revealed that about 17% of the laser energy is coupled to the suprathermal electrons. Modeling of the transport of these electrons and the associated isochoric heating, with the previously determined laser-to-electron conversion efficiency, showed a maximum target temperature of 166 eV at the front where the electron flux is higher and the density is lower. The contribution of the potential, induced by charge separation, in opposing the motion of the electrons was moderate. Second, temperature sensitivity of Cu K{sub {alpha}} imaging efficiency using a spherical Bragg reflecting crystal is investigated. It was found that due to the shifting and broadening of ...
Date: October 20, 2006
Creator: Akli, K
Partner: UNT Libraries Government Documents Department

Nanolithographic Fabrication and Heterogeneous Reaction Studies ofTwo-Dimensional Platinum Model Catalyst Systems

Description: In order to better understand the fundamental components that govern catalytic activity, two-dimensional model platinum nanocatalyst arrays have been designed and fabricated. These catalysts arrays are meant to model the interplay of the metal and support important to industrial heterogeneous catalytic reactions. Photolithography and sub-lithographic techniques such as electron beam lithography, size reduction lithography and nanoimprint lithography have been employed to create these platinum nanoarrays. Both in-situ and ex-situ surface science techniques and catalytic reaction measurements were used to correlate the structural parameters of the system to catalytic activity.
Date: May 20, 2006
Creator: Contreras, A.M.
Partner: UNT Libraries Government Documents Department

Cobalt Nanocrystals as Starting Materials for Shape Modificationand Assembly Formation

Description: Surfactant-coated cobalt nanocrystals can be prepared with areasonable degree of control over particle size and shape using athermolytic route. The small crystallite size, enhanced reactivity andtunable interparticle interactions enable use of this material asstarting material for demonstration of achievement of novel structuresusing extremely simple solution-based approaches. In particular,formation of hollow cobalt sulfide nanocrystals upon chemicalmodification and emergence of long-range orientational order upondrying-mediated assembly of cobalt nanocrystals is reportedhere.Colloidal preparation of Co nanocrystals has been well-studied.Here, we emphasize general principles and crystallographic/morphologicalcharacterization of disk-shaped hcp-Co nanocrystals. Use of surfactantmolecules enables achievement of multiple morphologies in one syntheticsystem.Formation of hollow structures upon in-solution sulfidation of Conanocrystals is presented and discussed. A Kirkendall-type effect,involving dominant outward mass transport during formation of the ionicshell material explains the results naturally. It is expected that thisphenomenon will generalize extensively to formation of hollow structuresof an enormous variety of compositions. Detailed study of particlemorphology as a function of reaction conditions suggest phenomena likelyto be generally relevant to use of this approach. A short report ofcrystallographic co-alignment into vortex-like structures is alsoprovided. Our current best picture of this process involves an interplayof packing and magnetic interactions between facetedparticles.
Date: December 20, 2005
Creator: Erdonmez, Can Kerem
Partner: UNT Libraries Government Documents Department

Dynamical Study of Guest-Host Orientational Interaction in LiquidCrystalline Materials

Description: Guest-host interaction has long been a subject of interest in many disciplines. Emphasis is often on how a small amount of guest substance could significantly affect the properties of a host material. This thesis describe our work in studying a guest-host effect where dye-doping of liquid crystalline materials greatly enhances the optical Kerr nonlinearity of the material. The dye molecules, upon excitation and via intermolecular interaction, provides an extra torque to reorient the host molecules, leading to the enhanced optical Kerr nonlinearity. We carried out a comprehensive study on the dynamics of the photoexcited dye-doped liquid crystalline medium. Using various experimental techniques, we separately characterized the dynamical responses of the relevant molecular species present in the medium following photo-excitation, and thus were able to follow the transient process in which photo-excitation of the dye molecules exert through guest-host interaction a net torque on the host LC material, leading to the observed enhanced molecular reorientation. We also observed for the first time the enhanced reorientation in a pure liquid crystal system, where the guest population is created through photoexcitation of the host molecules themselves. Experimental results agree quantitatively with the time-dependent theory based on a mean-field model of the guest-host interaction.
Date: December 20, 2005
Creator: Truong, Thai Viet
Partner: UNT Libraries Government Documents Department


Description: The nuclear radiations of nuclides: U{sup 233}, Pu{sup 239}, Bk{sup 243}, Bk{sup 244}, Bk{sup 245}, Bk{sup 246}, Bk{sup 249}, Cf{sup 249}, and Fm{sup 255} were investigated with high-resolution spectrometers. The {alpha}-particle spectra of all nuclides except Bk{sup 249} were measured with 6 mm diameter surface-barrier detectors. Bk{sup 249} {alpha}-particles were analyzed with a double-focusing magnetic spectrograph. The {gamma}-singles were examined with the recently developed Ge(Li) and Si(Li) detectors coupled with very-low noise 'internal FET' preamplifiers. Weak alpha groups were observed in coincidence with {gamma}-rays, detected with a NaI(Tl) scintillation spectrometer. To improve the over-all coincidence efficiency a new coincidence apparatus was designed and built. This instrument consisted of a cooled 4.5 cm diameter semiconductor detector for {alpha}-particle detection and a 3 cm diameter by 2.7 cm long Ge(Li) detector for {gamma}-ray analysis. The Ge(Li) detector could also be replaced with a NaI(Tl) detector. Cf{sup 249} conversion electrons were measured with a cooled Si(Li) detector coupled with an internal FET preamplifier. On the basis of the present work and previous information, energy-level diagrams of the daughter nuclei have been constructed. The levels have been grouped into rotational bands built on Nilsson single-particle states. Because of identification of several rotational members of the bands, definite Nilsson quantum number assignments have been made in most cases. The alpha intensity calculations of Poggenburg were found quite helpful in making these assignments. A strong Coriolis effect was observed in the Am{sup 245} levels populated by the alpha groups of Bk{sup 249}. Calculations were made with Nilsson wave-functions, and these were found to agree with the experimental results. The Coriolis interaction was found important in almost all cases; the effect was very noticeable in the level spacings between the rotational members of the bands. High-lying bands in Cm{sup 245} (at 644 keV) and cf{sup 251} (at ...
Date: September 20, 1966
Creator: Ahmad, Irshad
Partner: UNT Libraries Government Documents Department

Linking Automated Data Analysis and Visualization with Applications in Developmental Biology and High-Energy Physics

Description: Knowledge discovery from large and complex collections of today's scientific datasets is a challenging task. With the ability to measure and simulate more processes at increasingly finer spatial and temporal scales, the increasing number of data dimensions and data objects is presenting tremendous challenges for data analysis and effective data exploration methods and tools. Researchers are overwhelmed with data and standard tools are often insufficient to enable effective data analysis and knowledge discovery. The main objective of this thesis is to provide important new capabilities to accelerate scientific knowledge discovery form large, complex, and multivariate scientific data. The research covered in this thesis addresses these scientific challenges using a combination of scientific visualization, information visualization, automated data analysis, and other enabling technologies, such as efficient data management. The effectiveness of the proposed analysis methods is demonstrated via applications in two distinct scientific research fields, namely developmental biology and high-energy physics.Advances in microscopy, image analysis, and embryo registration enable for the first time measurement of gene expression at cellular resolution for entire organisms. Analysis of high-dimensional spatial gene expression datasets is a challenging task. By integrating data clustering and visualization, analysis of complex, time-varying, spatial gene expression patterns and their formation becomes possible. The analysis framework MATLAB and the visualization have been integrated, making advanced analysis tools accessible to biologist and enabling bioinformatic researchers to directly integrate their analysis with the visualization. Laser wakefield particle accelerators (LWFAs) promise to be a new compact source of high-energy particles and radiation, with wide applications ranging from medicine to physics. To gain insight into the complex physical processes of particle acceleration, physicists model LWFAs computationally. The datasets produced by LWFA simulations are (i) extremely large, (ii) of varying spatial and temporal resolution, (iii) heterogeneous, and (iv) high-dimensional, making analysis and knowledge discovery from complex ...
Date: November 20, 2009
Creator: Ruebel, Oliver
Partner: UNT Libraries Government Documents Department

A search for $ZH\rightarrow \mu\mu b \bar{b}$ production at the Tevatron

Description: The Standard Model describes with a very good accuracy all interactions of the, so far, known elementary particles. However the Higgs mechanism, which gives rise to the observed mass of these particles, has not yet been confirmed. The Higgs particle has not yet been observed, and the observation or exclusion is an important test of the Standard Model. The Standard Model does not predict the mass of the Higgs particle, however it does impose some limits on the range in which this mass can lie. In direct searches a Higgs with a mass smaller than 114.4 GeV and within 162 GeV and 166 GeV has been excluded at 95% CL at the LEP and the Tevatron colliders. The analysis presented in this thesis is aimed to search for the ZH → μμb$\bar{b}$ events in 3.1 fb<sup>-1</sup> of data collected with the DØ detector in p$\bar{p}$ collisions at √s = 1.96 TeV.
Date: April 20, 2010
Creator: Ancu, Lucian-Stefan
Partner: UNT Libraries Government Documents Department

Building Structural Complexity in Semiconductor Nanocrystals through Chemical Transformations

Description: Methods are presented for synthesizing nanocrystal heterostructures comprised of two semiconductor materials epitaxially attached within individual nanostructures. The chemical transformation of cation exchange, where the cations within the lattice of an ionic nanocrystal are replaced with a different metal ion species, is used to alter the chemical composition at specific regions ofa nanocrystal. Partial cation exchange was performed in cadmium sulfide (CdS) nanorods of well-defined size and shape to examine the spatial organization of materials within the resulting nanocrystal heterostructures. The selectivity for cation exchange to take place at different facets of the nanocrystal plays an important role in determining the resulting morphology of the binary heterostructure. The exchange of copper (I) (Cu+) cations in CdS nanorods occurs preferentially at the ends of the nanorods. Theoretical modeling of epitaxial attachments between different facets of CdS and Cu2S indicate that the selectivity for cation exchange at the ends of the nanorods is a result of the low formation energy of the interfaces produced. During silver (I) (Ag+) cation exchange in CdS nanorods, non-selective nucleation of silver sulfide (Ag2S), followed by partial phase segregation leads to significant changes in the spatial arrangement of CdS and Ag2S regions at the exchange reaction proceeds through the nanocrystal. A well-ordered striped pattern of alternating CdS and Ag2S segments is found at intermediate fractions of exchange. The forces mediating this spontaneous process are a combination of Ostwald ripening to reduce the interfacial area along with a strain-induced repulsive interaction between Ag2S segments. To elucidate why Cu+ and Ag+ cation exchange with CdS nanorods produce different morphologies, models for epitaxial attachments between various facets of CdS with Cu2S or Ag2S lattices were used to calculate interface formation energies. The formation energies indicate the favorability for interface nucleation at different facets of the nanorod and the stability of ...
Date: May 20, 2009
Creator: Sadtler, Bryce F.
Partner: UNT Libraries Government Documents Department

Extreme ultraviolet lithography: A few more pieces of the puzzle

Description: The work described in this dissertation has improved three essential components of extreme ultraviolet (EUV) lithography: exposure tools, photoresist, and metrology. Exposure tools. A field-averaging illumination stage is presented that enables nonuniform, high-coherence sources to be used in applications where highly uniform illumination is required. In an EUV implementation, it is shown that the illuminator achieves a 6.5% peak-to-valley intensity variation across the entire design field of view. In addition, a design for a stand-alone EUV printing tool capable of delivering 15 nm half-pitch sinusoidal fringes with available sources, gratings and nano-positioning stages is presented. It is shown that the proposed design delivers a near zero line-edge-rougness (LER) aerial image, something extremely attractive for the application of resist testing. Photoresist. Two new methods of quantifying the deprotection blur of EUV photoresists are described and experimentally demonstrated. The deprotection blur, LER, and sensitivity parameters of several EUV photoresists are quantified simultaneously as base weight percent, photoacid generator (PAG) weight percent, and post-exposure bake (PEB) temperature are varied. Two surprising results are found: (1) changing base weight percent does not significantly affect the deprotection blur of EUV photoresist, and (2) increasing PAG weight percent can simultaneously reduce LER and E-size in EUV photoresist. The latter result motivates the development of an EUV exposure statistics model that includes the effects of photon shot noise, the PAG spatial distribution, and the changing of the PAG distribution during the exposure. In addition, a shot noise + deprotection blur model is used to show that as deprotection blur becomes large relative to the size of the printed feature, LER reduction from improved counting statistics becomes dominated by an increase in LER due to reduced deprotection contrast. Metrology. Finally, this dissertation describes MOSAIC, a new wavefront metrology that enables complete wavefront recovery from print or aerial image ...
Date: May 20, 2009
Creator: Anderson, Christopher N.
Partner: UNT Libraries Government Documents Department

The Development of the Electrically Controlled High Power RF Switch and Its Application to Active RF Pulse Compression Systems

Description: In the past decades, there has been increasing interest in pulsed high power RF sources for building high-gradient high-energy particle accelerators. Passive RF pulse compression systems have been used in many applications to match the available RF sources to the loads requiring higher RF power but a shorter pulse. Theoretically, an active RF pulse compression system has the advantage of higher efficiency and compactness over the passive system. However, the key component for such a system an element capable of switching hundreds of megawatts of RF power in a short time compared to the compressed pulse width is still an open problem. In this dissertation, we present a switch module composed of an active window based on the bulk effects in semiconductor, a circular waveguide three-port network and a movable short plane, with the capability to adjust the S-parameters before and after switching. The RF properties of the switch module were analyzed. We give the scaling laws of the multiple-element switch systems, which allow the expansion of the system to a higher power level. We present a novel overmoded design for the circular waveguide three-port network and the associated circular-to-rectangular mode-converter. We also detail the design and synthesis process of this novel mode-converter. We demonstrate an electrically controlled ultra-fast high power X-band RF active window built with PIN diodes on high resistivity silicon. The window is capable of handling multi-megawatt RF power and can switch in 2-300ns with a 1000A current driver. A low power active pulse compression experiment was carried out with the switch module and a 375ns resonant delay line, obtaining 8 times compression gain with a compression ratio of 20.
Date: March 20, 2009
Creator: Guo, Jiquan
Partner: UNT Libraries Government Documents Department