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Ir/PuO/sub 2/ compatibility: transfer of impurities from plutonium dioxide to iridium metal during high temperature aging

Description: Plutonium oxide fuel pellets for powering radioisotopic thermoelectric generators for NASA space vehicles are encapsulated in iridium which has been grain-boundary-stabilized with thorium and aluminum. After aging for 6 months at 1310/sup 0/C under vacuum, enhanced grain growth is observed in the near-surface grains of the iridium next to the PuO/sub 2/. Examination of the grain boundaries by AES and SIMS shows a depletion of thorium and aluminum. Iron, chromium, and nickel from the fuel were f… more
Date: January 1, 1984
Creator: Taylor, D. H.; Christie, W. H. & Pavone, D.
Partner: UNT Libraries Government Documents Department
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Space nuclear safety program. Progress report, August 1983

Description: This technical monthly report covers studies related to the use of /sup 238/PuO/sub 2/ in radioisotope power systems carried out for the Office of Special Nuclear Projects of the US Department of Energy by Los Alamos National Laboratory. Most of the studies discussed here are ongoing. Results and conclusions described may change as the work continues.
Date: January 1, 1984
Creator: Bronisz, S. E.
Partner: UNT Libraries Government Documents Department
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Plutonium release from pressed plutonium oxide fuel pellets in aquatic environments

Description: Plutonium oxide pellets (80% /sup 238/Pu, 40 g each) were exposed to fresh water and sea water at two temperatures for 3 y in enclosed glass chambers. The concentrations of plutonium observed in the waters increased linearly with time throughout the experiment. However, the observed release rates were inversely dependent on temperature and salinity, ranging from 160 ..mu..Ci/day for cold fresh water to 1.4 ..mu..Ci/day for warm sea water. The total releases, including the chamber residues, show… more
Date: December 1, 1983
Creator: Patterson, J. H.; Steinkruger, F. J.; Matlack, G. M.; Heaton, R. C.; Coffelt, K. P. & Herrera, B.
Partner: UNT Libraries Government Documents Department
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Space nuclear safety program. Progress report, July 1983

Description: This technical monthly report covers studies related to the use of /sup 238/PuO/sub 2/ in radioisotope power systems carried out for the Office of Special Nuclear Projects of the US Department of Energy by Los Alamos National Laboratory. Most of the studies discussed here are ongoing. Results and conclusions described may change as the work continues.
Date: November 1, 1983
Creator: Bronisz, S. E.
Partner: UNT Libraries Government Documents Department
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Space Nuclear-Safety Program progress report, February 1983

Description: This technical monthly report covers studies related to the use of /sup 238/PuO/sub 2/ in radioisotope power systems carried out for the Office of Special Nuclear Projects of the US Department of Energy by Los Alamos National Laboratory. Most of the studies discussed here are ongoing. Results and conclusions may change as the work continues.
Date: August 1, 1983
Creator: Bronisz, S. E.
Partner: UNT Libraries Government Documents Department
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General-Purpose Heat Source development: Safety Verification Test Program. Bullet/fragment test series

Description: The radioisotope thermoelectric generator (RTG) that will provide power for space missions contains 18 General-Purpose Heat Source (GPHS) modules. Each module contains four /sup 238/PuO/sub 2/-fueled clads and generates 250 W/sub (t)/. Because a launch-pad or post-launch explosion is always possible, we need to determine the ability of GPHS fueled clads within a module to survive fragment impact. The bullet/fragment test series, part of the Safety Verification Test Plan, was designed to provide… more
Date: May 1, 1985
Creator: George, T.G.; Tate, R.E. & Axler, K.M.
Partner: UNT Libraries Government Documents Department
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General-Purpose Heat Source Development: safety test program. Postimpact evaluation, Design Iteration Test 4

Description: The General-Purpose Heat Source (GPHS) provides power for space missions by transmitting the heat of /sup 238/Pu decay to thermoelectric elements. Because of the inevitable return of certain aborted missions, the heat source must be designed and constructed to survive both re-entry and Earth impact. The Design Iteration Test (DIT) series is part of an ongoing test program. The fourth test (DIT-4) was designed to evaluate the effect on impact behavior of changing the procedure used at the Mound … more
Date: December 1, 1984
Creator: George, T.G. & Schonfeld, F.W.
Partner: UNT Libraries Government Documents Department
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Improvements in manufacture of iridium alloy materials

Description: Iridium alloys are used as fuel-cladding material in radioisotope thermoelectric generators (RTGs). Hardware produced at the Oak Ridge National Laboratory (ORNL) has been used in Voyager 1 and 2, Galileo, and Ulysses spacecraft. This hardware was fabricated from small, 500-g drop-cast ingots. Porosity in these ingots and the resulting defects in the rolled sheets caused rejection of about 30% of the product. An improved manufacturing process was developed with the goal of substantially reducing… more
Date: January 1, 1992
Creator: Ohriner, E. K.
Partner: UNT Libraries Government Documents Department
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Space nuclear safety program. Progress report, December 1982

Description: This technical monthly report covers studies related to the use of /sup 238/PuO/sub 2/ in radioisotope power systems carried out for the Office of Special Nuclear Projects of the US Department of Energy by Los Alamos National Laboratory. Most of the studies discussed here are ongoing. Results and conclusions described may change as the work continues.
Date: June 1, 1983
Creator: Bronisz, S. E.
Partner: UNT Libraries Government Documents Department
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Safety analysis for the Galileo Light-Weight Radioisotope Heater Unit

Description: The Light-Weight Radioisotope Heater Unit (LWRHU) will be used on the NASA Galileo Mission to provide thermal energy to the various systems on the orbiter and probe that are adversely affected by the low temperature a spacecraft encounters during a long interplanetary mission. Using these plutonia-fueled sources in 1-W increments permits employment of a single design and provides the spacecraft user the option of how many to use and where to position them to satisfy the proper thermal environme… more
Date: January 1, 1990
Creator: Johnson, E. W.
Partner: UNT Libraries Government Documents Department
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Space nuclear safety and fuels program. Progress report, September 1981

Description: This technical monthly report covers studies related to the use of /sup 238/PuO/sub 2/ in radioisotope power systems carried ot for the Office of Coordination and Special Projects of the US Department of Energy by Los Alamos National Laboratory. Most of the studies discussed here are ongoing. Results and conclusions described may change as the work continues. Published reference of the results cited in this report should not be made without the explicit permission of the person in charge of the… more
Date: February 1, 1982
Creator: Bronisz, S. E.
Partner: UNT Libraries Government Documents Department
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Environmental and radiological safety studies: interaction of /sup 238/PuO/sub 2/ heat sources with terrestrial and aquatic environments. Progress report, July 1-September 30, 1982

Description: Although existing radioisotope thermoelectric generator designs have proved more than adequately safe, more information is continually sought about the heat sources to improve their safety. The work here includes studies of the effects on the heat sources of terrestrial and aquatic environments and also of the effects of the heat sources on various simulated environments. This progress report presents recent data from environmental chamber and aquatic experiments and gives the present status of… more
Date: December 1, 1982
Creator: Matlack, G. M.; Patterson, J. H. & Stalnaker, N. D.
Partner: UNT Libraries Government Documents Department
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General-Purpose Heat Source safety verification test series: SVT-1 through SVT-6

Description: The General-Purpose Heat Source (GPHS) is a modular heat source that will supply energy for Radioisotope Thermoelectric Generators (RTGs) in space missions. The Safety Verification Tests (SVTs) are performed to assess the plutonia containment capability of heat source modules subjected to certain accident environments. This interim report described the GPHS module configuration, the test environment, and the response of the module components following simulated reentry and solid Earth impact. T… more
Date: June 1, 1985
Creator: Pavone, D.; George, T.G. & Frantz, C. E.
Partner: UNT Libraries Government Documents Department
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High-temperature compatibility study of iridium (DOP-26 alloy) with graphite and plutonia

Description: This report outlines the materials compatibility tests conducted on DOP-26 iridium alloy and carbon. The carbon used was in the form of woven graphite as present in the impact shell used to encase plutonia in nuclear heat sources. In addition, compatibility tests of the DOP-26 alloy with plutonia are described. The reactivity observed in both systems is discussed. 4 refs., 6 figs.
Date: December 1, 1987
Creator: Axler, K.M. & Eash, D.T.
Partner: UNT Libraries Government Documents Department
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Light-Weight Radioisotope Heater Unit Safety Analysis Report (LWRHU-SAR). Volume I. A. Introduction and executive summary. B. Reference Design Document (RDD)

Description: The orbiter and probe portions of the NASA Galileo spacecraft contain components which require auxiliary heat during the mission. To meet these needs, the Department of Energy's (DOE's) Office of Special Nuclear Projects (OSNP) has sponsored the design, fabrication, and testing of a one-watt encapsulated plutonium dioxide-fueled thermal heater named the Light-Weight Radioisotope Heater Unit (LWRHU). This report addresses the radiological risks which might be encountered by people both at the la… more
Date: October 1, 1985
Creator: Johnson, E. W.
Partner: UNT Libraries Government Documents Department
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Space nuclear safety program. Progress report, January 1984

Description: This technical monthly report covers studies related to the use of /sup 238/PuO/sub 2/ in radioisotope power systems carried out for the Office of Special Nuclear Projects of the US Department of Energy by Los Alamos National Laboratory. Most of the studies discussed here are ongoing. Results and conclusions described may change as the work continues.
Date: July 1, 1984
Creator: Bronisz, S. E.
Partner: UNT Libraries Government Documents Department
open access

Space Nuclear Safety Program. Progress report, November 1983

Description: This technical monthly report covers studies related to the use of /sup 238/PuO/sub 2/ in radioisotope power systems carried out for the Office of Special Nuclear Projects of the US Department of Energy by Los Alamos National Laboratory. Topics discussed include: safety-verification impact tests; explosion test; fragment test; leaking fueled clads; effects of fresh water and seawater or PuO/sub 2/ pellets; and impact tests of 5 watt radioisotope thermoelectric generator.
Date: June 1, 1984
Creator: Bronisz, S. E.
Partner: UNT Libraries Government Documents Department
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Space Nuclear Space Program. Progress report, December 1983

Description: This technical monthly report covers studies related to the use of /sup 238/PuO/sub 2/ in radioisotope power systems carried out for the Office of Special Nuclear Projects of the US Department of Energy by Los Alamos National Laboratory. Results from safety-verification tests including impact tests are presented.
Date: June 1, 1984
Creator: Bronisz, S. E.
Partner: UNT Libraries Government Documents Department
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Helium release from radioisotope heat sources

Description: Diffusion of helium in /sup 238/PuO/sub 2/ fuel was characterized as a function of the heating rate and the fuel microstructure. The samples were thermally ramped in an induction furnace and the helium release rates measured with an automated mass spectrometer. The diffusion constants and activation energies were obtained from the data using a simple diffusion model. The release rates of helium were correlated with the fuel microstructure by metallographic examination of fuel samples. The relea… more
Date: May 1, 1984
Creator: Peterson, D.E.; Early, J.W.; Starzynski, J.S. & Land, C.C.
Partner: UNT Libraries Government Documents Department
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General-purpose heat source development: Extended series test program SRB fragment/fuselage tests

Description: General-Purpose Heat Source radioisotope thermoelectric generators (GPHS-RTGs) will provide electrical power for the NASA Galileo and European Space Agency (ESA) Ulysses missions. Each GPHS-RTG comprises two major components: GPHS modules, which provide thermal energy, and a thermoelectric converter, which converts the thermal energy into electrical power. Each of the 18 GPHS modules in a GPHS-RTG contains four /sup 238/PuO/sub 2/-fueled capsules. LANL conducted a series of safety verification … more
Date: June 1, 1989
Creator: Cull, T.A.
Partner: UNT Libraries Government Documents Department
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