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THE LIFETIME OF AEROSOL DROPLETS IN AMBIENT AIR: CONSIDERATION OF THE EFFECTS OF SURFACTANTS AND CHEMICAL REACTIONS

Description: The relatively long lifetime of droplets in atmospheric haze and fog in comparison to similar droplets of pure water is attributed to the presence of a monolayer of surfactant film and to the accumulation of soluble salts from chemical reactions. The lifetime of these droplets is a significant factor in the evaluation of the role of heterogeneous aqueous chemical reactions occurring in the troposphere. A new formulation is given which includes both these processes. As an example, the catalytic oxidation of SO{sub 2} in the presence of liquid water droplets is investigated.
Date: September 1, 1980
Creator: Toossi, R. & Novakov, T.
Partner: UNT Libraries Government Documents Department

CHARACTERISTICS OF RANGE HOODS IN CALIFORNIA HOMES DATA COLLECTED FROM A REAL ESTATE WEB SITE

Description: Venting range hoods are important residential ventilation components that remove pollutants generated by cooking activities and natural gas cooking burners. To address the lack of data on range hood installations in California, we conducted a survey by examining photographs of homes for sale or rent listed on a popular real estate web site. The survey was conducted in November 2010 and April–May 2011. Posted photos of the homes were reviewed to determine if a hood was installed, the type of hood, and two installation details that can impact performance, namely the height above the cooktop and the degree to which the hood covers the cooktop burners. We additionally collected information about the homes, including asking price for purchase or rent, type of building (e.g. detached house, townhouse or apartment), building age, floor area, and cooktop fuel type. Listings were first sampled to focus on homes built since 2005, then randomly sampled to include varied prices and locations around the state. Data were obtained for 1002 homes built between 1865 and 2011 (median year built 1989). Homes for sale varied in asking price from $16,000 to $16,500,000 (median $353,000) and homes for rent varied from $500 to $25,000 (median $2125) per month. Approximately 74% of the sample had natural gas cooktops. In this sample, natural gas cooktops were more prevalent in more expensive homes than in less expensive homes. Across the entire sample, 7.4 % appeared to have no hood installed, 33% had a short hood, 13% had a deep hood and 47% had a microwave over the range. The percentage of these hoods that vent to the outdoors could not be determined. Hood type was related to coverage of the cooktop. For deep hoods, 76% appeared to cover most or all of the cooktop burners. For short hoods, 70% covered ...
Date: September 2, 2011
Creator: Klug, Victoria; Singer, Brett; Bedrosian, Tod & DCruz, Chris
Partner: UNT Libraries Government Documents Department

SOOT IN THE ARCTIC

Description: Substantial concentrations of graphitic carbon and its associated large optical absorption coefficient are observed in the Arctic. The graphitic content shows a dramatic increase from late fall to early spring, reaching levels that can be comparable to those found in urban environments.
Date: October 1, 1980
Creator: Rosen, H.; Novakov, T. & Bodhaine, B. A.
Partner: UNT Libraries Government Documents Department

THE ROLE OF SOOT PARTICLES AND NO{sub x} IN THE OXIDATION OF SO{sub 2} IN AQUEOUS SOLUTION: KINETICS, MECHANISM, AND IMPACT ON SULFATE AEROSOL FORMATION

Description: We have identified two previously unrecognized processes which could play an important role in terms of acid rain and sulfate aerosol formation: 1) the oxidation of SO{sub 2} in water droplets containing soot particles, and 2) the oxidation of SO{sub 2} by NO{sub x} in water droplets. The results of our investigation on these two systems are outlined.
Date: November 1, 1980
Creator: Chang, S.G.; Brodzinsky, R.; Oblath, S.; Markowitz, S.; Toossi, R. & Novakov, T.
Partner: UNT Libraries Government Documents Department

Water in the 21st Century

Description: This research project focused on sustainability issues in the southwest U.S. with an emphasis on water and energy. The efforts were directed through the UNLV Urban Sustainability Office with the funding used to develop a sustainability strategic plan; conduct extensive community outreach in the greater metropolitan area; provide seed money for multidisciplinary research teams to conduct studies in the areas of ecological, socio-cultural, and economic sustainability leading to community-based solutions; and to provide service-learning opportunities for UNLV graduate and undergraduate students. The research advanced understanding of urban and regional water issues with a particular focus on climate change and climate variability in the southwest. In addition, various events were held to promote discussion on energy, water, and sustainability discussions in the community. The impact of this research was broad dissemination of research through 13 peer-reviewed publications, learning opportunities for countless students as a result of class room equipment upgrades (see report for upgrade details), and new research funding for further advancement of these research efforts.
Date: February 8, 2013
Creator: Piechota, Thomas C
Partner: UNT Libraries Government Documents Department

Final Report-Confirmatory Survey Results for the ABB Combustion Engineering Site, Windsor, Connecticut; Revision 1 (DCN 5158-SR-02-1) (Docket No. 030-03754; RFTA No. 12-003)

Description: The objectives of the confirmatory activities were to provide independent contractor field data reviews and to generate independent radiological data for use by the NRC in evaluating the adequacy and accuracy of the contractor�s procedures and FSS results. ORAU reviewed ABB CE�s decommissioning plan, final status survey plan, and the applicable soil DCGLs, which were developed based on an NRC-approved radiation dose assessment. The surveys included gamma surface scans, gamma direct measurements, and soil sampling.
Date: January 28, 2013
Creator: ADAMS, WADE C
Partner: UNT Libraries Government Documents Department

INDEPENDENT CONFIRMATORY SURVEY SUMMARY AND RESULTS FOR THE FORD NUCLEAR REACTOR, ANN ARBOR, MICHIGAN

Description: At the NRC�s request, ORAU conducted confirmatory surveys of the FNR during the period of December 4 through 6, 2012. The survey activities included visual inspections and measurement and sampling activities. Confirmatory activities also included the review and assessment of UM�s project documentation and methodologies. Surface scans identified elevated activity in two areas. The first area was on a wall outside of Room 3103 and the second area was in the southwest section on the first floor. The first area was remediated to background levels. However, the second area was due to gamma shine from a neighboring source storage area. A retrospective analysis of UM�s FSS data shows that for the SUs investigated by the ORAU survey team, UM met the survey requirements set forth in the FSSP. The total mean surface activity values were directly compared with the mean total surface activity reported by UM. Mean surface activity values determined by UM were within two standard deviations of the mean determined by ORAU. Additionally, all surface activity values were less than the corresponding gross beta DCGLW. Laboratory analysis of the soil showed that COC concentrations were less than the respective DCGLW values. For the inter-lab comparison, the DER was above 3 for only one sample. However, since the sum of fractions for each of the soil samples was below 1, thus none of the samples would fail to meet release guidelines. Based on the findings of the side-by-side direct measurements, and after discussion with the NRC and ORAU, UM decided to use a more appropriate source efficiency in their direct measurement calculations and changed their source efficiency from 0.37 to 0.25.
Date: July 25, 2013
Creator: ALTIC, NICK A
Partner: UNT Libraries Government Documents Department

INTERIM REPORT--INDEPENDENT VERIFICATION SURVEY OF SECTION 3, SURVEY UNITS 1, 4 AND 5 EXCAVATED SURFACES, WHITTAKER CORPORATION, REYNOLDS INDUSTRIAL PARK, TRANSFER, PENNSYLVANIA DCN: 5002-SR-04-0"

Description: At Pennsylvania Department of Environmental Protection's request, ORAU's IEAV program conducted verification surveys on the excavated surfaces of Section 3, SUs 1, 4, and 5 at the Whittaker site on March 13 and 14, 2013. The survey activities included visual inspections, gamma radiation surface scans, gamma activity measurements, and soil sampling activities. Verification activities also included the review and assessment of the licensee�s project documentation and methodologies. Surface scans identified four areas of elevated direct gamma radiation distinguishable from background; one area within SUs 1 and 4 and two areas within SU5. One area within SU5 was remediated by removing a golf ball size piece of slag while ORAU staff was onsite. With the exception of the golf ball size piece of slag within SU5, a review of the ESL Section 3 EXS data packages for SUs 1, 4, and 5 indicated that these locations of elevated gamma radiation were also identified by the ESL gamma scans and that ESL personnel performed additional investigations and soil sampling within these areas. The investigative results indicated that the areas met the release criteria.
Date: April 18, 2013
Creator: ADAMS, WADE C
Partner: UNT Libraries Government Documents Department

Aerosol Optical Depth Value-Added Product Report

Description: This document describes the process applied to retrieve aerosol optical depth (AOD) from multifilter rotating shadowband radiometers (MFRSR) and normal incidence multifilter radiometers (NIMFR) operated at the ARM Climate Research Facility’s ground-based facilities.
Date: March 17, 2013
Creator: Koontz, A; Hodges, G; Barnard, J; Flynn, C & Michalsky, J
Partner: UNT Libraries Government Documents Department

Organic Aerosol Component (OACOMP) Value-Added Product Report

Description: Significantly improved returns in their aerosol chemistry data can be achieved via the development of a value-added product (VAP) of deriving OA components, called Organic Aerosol Components (OACOMP). OACOMP is primarily based on multivariate analysis of the measured organic mass spectral matrix. The key outputs of OACOMP are the concentration time series and the mass spectra of OA factors that are associated with distinct sources, formation and evolution processes, and physicochemical properties.
Date: August 23, 2013
Creator: Fast, J; Zhang, Q; Tilp, A; Shippert, T; Parworth, C & Mei, F
Partner: UNT Libraries Government Documents Department

Next generation aerosol-cloud microphysics for advanced high-resolution climate predictions

Description: The three top-level project goals are: -We proposed to develop, test, and run a new, physically based, scale-independent microphysical scheme for those cloud processes that most strongly affect greenhouse gas scenarios, i.e. warm cloud microphysics. In particular, we propsed to address cloud droplet activation, autoconversion, and accretion. -The new, unified scheme was proposed to be derived and tested using the University of Hawaii's IPRC Regional Atmospheric Model (iRAM). -The impact of the new parameterizations on climate change scenarios will be studied. In particular, the sensitivity of cloud response to climate forcing from increased greenhouse gas concentrations will be assessed.
Date: January 14, 2013
Creator: Bennartz, Ralf; Hamilton, Kevin P; Phillips, Vaughan T.J.; Wang, Yuqing & Brenguier, Jean-Louis
Partner: UNT Libraries Government Documents Department

"CONFIRMATORY SURVEY RESULTS FOR THE ABB COMBUSTION ENGINEERING SITE WINDSOR, CONNECTICUT DCN 5158-SR-02-2

Description: The objectives of the confirmatory activities were to provide independent contractor field data reviews and to generate independent radiological data for use by the NRC in evaluating the adequacy and accuracy of the contractor�s procedures and FSS results. ORAU reviewed ABB CE�s decommissioning plan, final status survey plan, and the applicable soil DCGLs, which were developed based on an NRC-approved radiation dose assessment. The surveys include gamma surface scans, gamma direct measurements, and soil sampling.
Date: March 25, 2013
Creator: ADAMS, WADE C
Partner: UNT Libraries Government Documents Department

"INDEPENDENT CONFIRMATORY SURVEY SUMMARY AND RESULTS FOR THE FORD NUCLEAR REACTOR, REVISION 1, ANN ARBOR, MICHIGAN

Description: At the NRC�s request, ORAU conducted confirmatory surveys of the FNR during the period of December 4 through 6, 2012. The survey activities included visual inspections and measurement and sampling activities. Confirmatory activities also included the review and assessment of UM�s project documentation and methodologies. Surface scans identified elevated activity in two areas. The first area was on a wall outside of Room 3103 and the second area was in the southwest section on the first floor. The first area was remediated to background levels. However, the second area was due to gamma shine from a neighboring source storage area. A retrospective analysis of UM�s FSS data shows that for the SUs investigated by the ORAU survey team, UM met the survey requirements set forth in the FSSP. The total mean surface activity values were directly compared with the mean total surface activity reported by UM. Mean surface activity values determined by UM were within two standard deviations of the mean determined by ORAU. Additionally, all surface activity values were less than the corresponding gross beta DCGL{sub W}. Laboratory analysis of the soil showed that COC concentrations were less than the respective DCGL{sub W} values. For the inter-lab comparison, the DER was above 3 for only one sample. However, since the sum of fractions for each of the soil samples was below 1, thus none of the samples would fail to meet release guidelines. Based on the findings of the side-by-side direct measurements, and after discussion with the NRC and ORAU, UM decided to use a more appropriate source efficiency in their direct measurement calculations and changed their source efficiency from 0.37 to 0.25.
Date: August 1, 2013
Creator: ALTIC, NICK A
Partner: UNT Libraries Government Documents Department

ARM Climate Research Facility Quarterly Value-Added Product Report Fourth Quarter: July 1–September 30, 2012

Description: The purpose of this report is to provide a concise status update for value-added products (VAP) implemented by the Atmospheric Radiation Measurement (ARM) Climate Research Facility. The report is divided into the following sections: (1) new VAPs for which development has begun, (2) progress on existing VAPs, (3) future VAPs that have been recently approved, (4) other work that leads to a VAP, and (5) top requested VAPs from the archive.
Date: November 13, 2012
Creator: Sivaraman, C.
Partner: UNT Libraries Government Documents Department

ARM Standards Policy Committee Report

Description: Data and metadata standards promote the consistent recording of information and are necessary to ensure the stability and high quality of Atmospheric Radiation Measurement (ARM) Climate Research Facility data products for scientific users. Standards also enable automated routines to be developed to examine data, which leads to more efficient operations and assessment of data quality. Although ARM Infrastructure agrees on the utility of data and metadata standards, there is significant confusion over the existing standards and the process for allowing the release of new data products with exceptions to the standards. The ARM Standards Policy Committee was initiated in March 2012 to develop a set of policies and best practices for ARM data and metadata standards.
Date: September 19, 2012
Creator: Cialella, A; Jensen, M; Koontz, A; McFarlane, S; McCoy, R; Monroe, J et al.
Partner: UNT Libraries Government Documents Department

Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report October 1–December 31, 2012

Description: Individual datastreams from instrumentation at the Atmospheric Radiation Measurement (ARM) Climate Research Facility fixed and mobile research sites are collected and routed to the Data Management Facility (DMF) for processing in near-real-time. Instrument and processed data are then delivered approximately daily to the ARM Data Archive, where they are made freely available to the research community. For each instrument, we calculate the ratio of the actual number of processed data records received daily at the Data Archive to the expected number of data records. The results are tabulated by (1) individual datastream, site, and month for the current year and (2) site and fiscal year dating back to 1998.
Date: January 11, 2013
Creator: Voyles, JW
Partner: UNT Libraries Government Documents Department

GAMMA DETECTOR RESPONSE/SOIL CONCENTRATION CORRELATION STUDY AT THE AAR MANUFACTURING, INC. SITE, LIVONIA, MICHIGAN

Description: At the NRC�s request, ORAU conducted surveys of the AAR Manufacturing site during the period of September 25 through September 27, 2012. The survey activities included walkover surveys and sampling activities. Once the survey team was onsite, the NRC personnel decided to forgo survey activities in the �New Addition� and the pickling area. Areas of the planned study boundary were inaccessible due to overgrowth/large pieces of concrete covering the soil surface; therefore, the study boundary was redefined. Gamma walkover scans of the site boundary and �front yard� identified multiple areas of elevated gamma radiation. As a result, two judgmental samples were collected. Sample results were above thorium background levels The answer to the PSQ relating to the relationship between thorium concentration in soil and NaI instrument response is �Yes.� NaI instrument response can be used as a predictor of Th-232 concentration in the 0 to 1 m layer. An R2 value of 0.79 was determined for the surface soil relationship, thus satisfying the DQOs. Moreover, the regression was cross-checked by comparing the predicted Th-232 soil core concentration to the average Th-232 concentration (Section 5.3.2). Based on the cross-check, the regression equation provides a reasonable estimate for the Th-232 concentration at the judgmental locations. Consideration must be given when applying this equation to other soil areas of the site. If the contamination was heterogeneously distributed, and not distributed in a discrete layer as it was in the study area, then using the regression equation to predict Th-232 concentration would not be applicable.
Date: March 22, 2013
Creator: ALTIC, NICK A
Partner: UNT Libraries Government Documents Department

Production Mechanism, Number Concentration, Size Distribution, Chemical Composition, and Optical Properties of Sea Spray Aerosols Workshop, Summer 2012

Description: The objective of this workshop was to address the most urgent open science questions for improved quantification of sea spray aerosol-radiation-climate interactions. Sea spray emission and its influence on global climate remains one of the most uncertain components of the aerosol-radiation-climate problem, but has received less attention than other aerosol processes (e.g. production of terrestrial secondary organic aerosols). Thus, the special emphasis was placed on the production flux of sea spray aerosol particles, their number concentration and chemical composition and properties.
Date: October 21, 2013
Creator: Meskhidze, Nicholas
Partner: UNT Libraries Government Documents Department

COMPARISON OF RESULTS FOR QUARTER 3 SURFACE WATER SPLIT SAMPLES COLLECTED AT THE NUCLEAR FUEL SERVICES SITE, ERWIN, TENNESSEE

Description: Oak Ridge Associated Universities (ORAU), under the Oak Ridge Institute for Science and Education (ORISE) contract, collected split surface water samples with Nuclear Fuel Services (NFS) representatives on March 20, 2013. Representatives from the U.S. Nuclear Regulatory Commission and the Tennessee Department of Environment and Conservation were also in attendance. Samples were collected at four surface water stations, as required in the approved Request for Technical Assistance number 11-018. These stations included Nolichucky River upstream (NRU), Nolichucky River downstream (NRD), Martin Creek upstream (MCU), and Martin Creek downstream (MCD). Both ORAU and NFS performed gross alpha and gross beta analyses, and Table 1 presents the comparison of results using the duplicate error ratio (DER), also known as the normalized absolute difference. A DER {<=} 3 indicates that at a 99% confidence interval, split sample results do not differ significantly when compared to their respective one standard deviation (sigma) uncertainty (ANSI N42.22). The NFS split sample report does not specify the confidence level of reported uncertainties (NFS 2013). Therefore, standard two sigma reporting is assumed and uncertainty values were divided by 1.96. In conclusion, most DER values were less than 3 and results are consistent with low (e.g., background) concentrations. The gross beta result for sample 5198W0012 was the exception. The ORAU result of 9.23 {+-} 0.73 pCi/L from location MCD is well above NFS�s result of -0.567 {+-} 0.63 pCi/L (non-detected). NFS�s data package included a detected result for U-233/234, but no other uranium or plutonium detection, and nothing that would suggest the presence of beta-emitting radionuclides. The ORAU laboratory reanalyzed sample 5198W0012 using the remaining portion of the sample volume and a result of 11.3 {+-} 1.1 pCi/L was determined. As directed, the laboratory also counted the filtrate using gamma spectrometry analysis and identified only naturally occurring or ubiquitous ...
Date: May 28, 2013
Partner: UNT Libraries Government Documents Department

COMPARISON OF RESULTS FOR QUARTER 4 SURFACE WATER SPLIT SAMPLES COLLECTED AT THE NUCLEAR FUELS SERVICES SITE, ERWIN, TN

Description: Oak Ridge Associated Universities (ORAU), under the Oak Ridge Institute for Science and Education (ORISE) contract, collected split surface water samples with Nuclear Fuel Services (NFS) representatives on June 12, 2013. Representatives from the U.S. Nuclear Regulatory Commission (NRC) and the Tennessee Department of Environment and Conservation were also in attendance. Samples were collected at four surface water stations, as required in the approved Request for Technical Assistance number 11-018. These stations included Nolichucky River upstream (NRU), Nolichucky River downstream (NRD), Martin Creek upstream (MCU), and Martin Creek downstream (MCD). Both ORAU and NFS performed gross alpha and gross beta analyses, and Table 1 presents the comparison of results using the duplicate error ratio (DER), also known as the normalized absolute difference. A DER ≤ 3 indicates at a 99% confidence interval that split sample results do not differ significantly when compared to their respective one standard deviation (sigma) uncertainty (ANSI N42.22). The NFS split sample report specifies 95% confidence level of reported uncertainties (NFS 2013). Therefore, standard two sigma reporting values were divided by 1.96. In conclusion, most DER values were less than 3 and results are consistent with low (e.g., background) concentrations. The gross beta result for sample 5198W0014 was the exception. The ORAU gross beta result of 6.30 � 0.65 pCi/L from location NRD is well above NFS�s non-detected result of 1.56 � 0.59 pCi/L. NFS�s data package includes no detected result for any radionuclide at location NRD. At NRC�s request, ORAU performed gamma spectroscopic analysis of sample 5198W0014 to identify analytes contributing to the relatively elevated gross beta results. This analysis identified detected amounts of naturally-occurring constituents, most notably Ac-228 from the thorium decay series, and does not suggest the presence of site-related contamination.
Date: August 15, 2013
Partner: UNT Libraries Government Documents Department

COMPARISON OF RESULTS FOR QUARTER 2 SURFACE WATER SPLIT SAMPLES COLLECTED AT THE NUCLEAR FUEL SERVICES SITE, ERWIN, TENNESSEE

Description: Oak Ridge Associated Universities (ORAU), under the Oak Ridge Institute for Science and Education (ORISE) contract, collected split surface water samples with Nuclear Fuel Services (NFS) representatives on November 15, 2012. Representatives from the U.S. Nuclear Regulatory Commission and Tennessee Department of Environment and Conservation were also in attendance. Samples were collected at four surface water stations, as required in the approved Request for Technical Assistance number 11-018. These stations included Nolichucky River upstream (NRU), Nolichucky River downstream (NRD), Martin Creek upstream (MCU), and Martin Creek downstream (MCD). Both ORAU and NFS performed gross alpha and gross beta analyses, and the results are compared using the duplicate error ratio (DER), also known as the normalized absolute difference. A DER {<=} 3 indicates that, at a 99% confidence interval, split sample results do not differ significantly when compared to their respective one standard deviation (sigma) uncertainty (ANSI N42.22). The NFS split sample report does not specify the confidence level of reported uncertainties (NFS 2012). Therefore, standard two sigma reporting is assumed and uncertainty values were divided by 1.96. In conclusion, all DER values were less than 3 and results are consistent with low (e.g., background) concentrations.
Date: January 21, 2013
Partner: UNT Libraries Government Documents Department

Meteorological services annual data report for 2012

Description: This document presents the meteorological data collected at Brookhaven National Laboratory (BNL) by Meteorological Services (Met Services) for the calendar year 2012. The purpose is to publicize the data sets available to emergency personnel, researchers and facility operations. Met services has been collecting data at BNL since 1949. Data from 1994 to the present is available in digital format. Data is presented in monthly plots of one-minute data. This allows the reader the ability to peruse the data for trends or anomalies that may be of interest to them. Full data sets are available to BNL personnel and to a limited degree outside researchers. The full data sets allow plotting the data on expanded time scales to obtain greater details (e.g., daily solar variability, inversions, etc.).
Date: February 1, 2013
Creator: J., Heiser & Smith, S.
Partner: UNT Libraries Government Documents Department

1999 Gordon Research Conference on Atmospheric Chemistry

Description: The Gordon Research Conference (GRC) on Atmospheric Chemistry was held at Salve Regina University in Newport, Rhode Island, June 13-18, 1999. The conference was well attended with 151 participants. The attendees represented the spectrum of endeavor in this field coming from academia, industry, and government laboratories, both US and foreign scientists, senior researchers, young investigators, and students.
Date: August 1, 2000
Creator: Storm, C.
Partner: UNT Libraries Government Documents Department