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Hybrid heat exchange for the compression capture of CO2 from recirculated flue gas

Description: An approach proposed for removal of CO2 from flue gas cools and compresses a portion of a recirculated flue-gas stream, condensing its volatile materials for capture. Recirculating the flue gas concentrates SOx, H2O and CO2 while dramatically reducing N2 and NOx, enabling this approach, which uses readily available industrial components. A hybrid system of indirect and direct-contact heat exchange performs heat and mass transfer for pollutant removal and energy recovery. Computer modeling and experimentation combine to investigate the thermodynamics, heat and mass transfer, chemistry and engineering design of this integrated pollutant removal (IPR) system.
Date: January 1, 2004
Creator: Oryshchyn, Danylo B.; Ochs, Thomas L. & Summers, Cathy A.
Partner: UNT Libraries Government Documents Department

Integrated pollutant removal: modeling and experimentation

Description: Experimental and computational work at the Albany Research Center, USDOE is investigating an integrated pollutant removal (IPR) process which removes all pollutants from flue gas, including SOX, NOX, particulates, CO2, and Hg. In combination with flue gas recirculation, heat recovery, and oxy-fuel combustion, the process produces solid, gas, and liquid waste streams. The gas exhaust stream comprises O2 and N2. Liquid streams contain H2O, SOX, NOX, and CO2. Computer modeling and low to moderate pressure experimentation are defining system chemistry with respect to SOX and H2O as well as heat and mass transfer for the IPR process.
Date: January 1, 2005
Creator: Ochs, Thomas L.; Oryshchyn, Danylo B. & Summers, Cathy A.
Partner: UNT Libraries Government Documents Department

The effect of SO2 on mineral carbonation in batch tests

Description: CO2 sequestration is a key element of future emission-free fossil-fueled power plants. Other constituents of flue gas must also be captured and rendered innocuous. Contemporary power plants remove SOx from exit gases, but next-generation plants may simultaneously treat CO2, SOx, and other pollutants. Pioneering tests at the U.S. Department of Energy's Albany Research Center investigated the combined treatment of CO2 and SO2 in a mineral-carbonation process. SO2 was removed from the gas stream, and as a small fraction of the total volume of mineralizing gas, it did not inhibit the carbonation reaction. The results indicate that this approach to CO2 sequestration could be used to treat multiple pollutants.
Date: January 1, 2004
Creator: Summers, Cathy A.; Dahlin, David C. & Ochs, Thomas L.
Partner: UNT Libraries Government Documents Department

Pressure gradient passivation of carbonaceous material normally susceptible to spontaneous combustion

Description: This invention is a process for the passivation or deactivation with respect to oxygen of a carbonaceous material by the exposure of the carbonaceous material to an oxygenated gas in which the oxygenated gas pressure is increased from a first pressure to a second pressure and then the pressure is changed to a third pressure. Preferably a cyclic process which comprises exposing the carbonaceous material to the gas at low pressure and increasing the pressure to a second higher pressure and then returning the pressure to a lower pressure is used. The cycle is repeated at least twice wherein the higher pressure may be increased after a selected number of cycles.
Date: January 29, 2002
Creator: Ochs, Thomas L.; Sands, William D.; Schroeder, Karl; Summers, Cathy A. & Utz, Bruce R.
Partner: UNT Libraries Government Documents Department

Investigation of the liquid/vapor composition of compressed liquid CO2 with N2 and O2 in integrated pollutant removal systems for coal combustion

Description: Accurate prediction of the processes in Integrated Pollutant Removal (IPR) using compression and condensation of coal combustion products requires an understanding of the liquid/vapor ternary CO2/O2/N2 system. At conditions close to the critical point of CO2 the existing equations of state deviate from the sparse measured results available in the literature. Building on existing data and procedures, the USDOE/Albany Research Center has designed an apparatus for examining compositions in this region. The design of the apparatus and planned initial experiments are presented.
Date: January 1, 2005
Creator: Oryshchyn, Danylo B.; Ochs, Thomas L.; Summers, Cathy A.; Penner, Larry R. & Gerdemann, Stephen J.
Partner: UNT Libraries Government Documents Department

Pressure Gradient Passivation of Carbonaceous Material Normally Susceptible to Spontaneous Combustion

Description: This invention is a process for the passivation or deactivation with respect to oxygen of a carbonaceous material by the exposure of the carbonaceous material to an oxygenated gas in which the oxygenated gas pressure is increased from a first pressure to a second pressure and then the pressure is changed to a third pressure. Preferably a cyclic process which comprises exposing the carbonaceous material to the gas at low pressure and increasing the pressure to a second higher pressure and then returning the pressure to a lower pressure is used. The cycle is repeated at least twice wherein the higher pressure may be increased after a selected number of cycles.
Date: July 15, 1999
Creator: Ochs, Thomas L.; Sands, William D.; Schroeder, Karl; Summers, Cathy A. & Utz, Bruce R.
Partner: UNT Libraries Government Documents Department

Final Report to Jupiter Oxygen Corporation on CRADA Phase 1 Activities, January 1, 2004, through June 30, 2005

Description: In January of 2004, a Cooperative Research and Development Agreement was signed with the Jupiter Oxygen Corporation; its term extends from January 2004 to January 1, 2009. The statement of work is attached as Appendix A. Under Phase I of this agreement, ARC was to provide technical expertise to develop computer models of existing power plants relative to retrofitting with oxy-fuel combustion; help design experiments to verify models and analyze data from experiments; help produce designs at larger scales; help design a new technology oxy-fuel power plant; and co-author technical papers on this work for presentation at appropriate conferences.
Date: June 30, 2005
Creator: Summers, Cathy A.; Oryshchyn, Danylo B.; Ochs, Thomas L. & Turner, Paul C.
Partner: UNT Libraries Government Documents Department

The potential for clean energy production using oxy-fuel combustion and integrated pollutant removal

Description: Effective remediation of flue gas produced by an oxy-fuel coal combustion process has been proven at bench scale in the course of cooperative research between USDOE’s Albany Research Center (ARC) and Jupiter Oxygen Corporation. All combustion gas pollutants were captured, including CO2 which was compressed to a liquefied state suitable for sequestration. Current laboratory-scale research and the future of combined oxy-fuel/IPR systems are discussed.
Date: May 1, 2005
Creator: Ochs, Thomas L.; Oryshchyn, Danylo B.; Weber, Thomas (Jupiter Oxygen Corporation, Schiller Park, IL 60176). & Summers, Cathy A.
Partner: UNT Libraries Government Documents Department

Developments in integrated pollutant removal for low-emission oxy-fuel combustion

Description: A complete coal combustion and flue gas treatment scheme was designed, constructed, and operated at bench scale as a product of cooperative research between US DOE’s Albany Research Center (ARC) and Jupiter Oxygen Corporation. The combustion gas generated using this oxy-fuel coal combustion process was effectively captured using an integrated pollutant removal (IPR) process. Supporting laboratory-scale research focuses on elements of IPR such as extraction of particulates, SO2, and mercury, and on the character of the liquid and vapor phase compositions for the CO2 - N2 - O2 mixture at the temperature and pressure conditions found at the end of the process. Future pilot-scale work will be necessary to generate economic and engineering data that will apply to full-scale oxy-fuel/IPR systems.
Date: September 1, 2005
Creator: Gerdemann, Stephen J.; Summers, Cathy A.; Oryshchyn, Danylo B.; Patrick, Brian (Jupiter Oxygen Corp.) & Ochs, Thomas L.
Partner: UNT Libraries Government Documents Department

The next generation of oxy-fuel boiler systems

Description: Research in the area of oxy-fuel combustion which is being pioneered by Jupiter Oxygen Corporation combined with boiler research conducted by the USDOE/Albany Research Center has been applied to designing the next generation of oxy-fuel combustion systems. The new systems will enhance control of boiler systems during turn-down and improve response time while improving boiler efficiency. These next generation boiler systems produce a combustion product that has been shown to be well suited for integrated pollutant removal. These systems have the promise of reducing boiler foot-print and boiler construction costs. The modularity of the system opens the possibility of using this design for replacement of boilers for retrofit on existing systems.
Date: January 1, 2005
Creator: Ochs, Thomas L.; Gross, Alex (Jupiter Oxygen Corp.); Patrick, Brian (Jupiter Oxygen Corp.); Oryshchyn, Danylo B.; Summers, Cathy A. & Turner, Paul C.
Partner: UNT Libraries Government Documents Department

Proof of concept for integrating oxy-fuel combustion and the removal of all pollutants from a coal fired flame

Description: The USDOE/Albany Research Center and Jupiter Oxygen Corporation, working together under a Cooperative Research and Development Agreement, have demonstrated proof-of-concept for the integration of Jupiter’s oxy-fuel combustion and an integrated system for the removal of all stack pollutants, including CO2, from a coal-fired flame. The components were developed using existing process technology with the addition of a new oxy-coal combustion nozzle. The results of the test showed that the system can capture SOx, NOx, particulates, and even mercury as a part of the process of producing liquefied CO2 for sequestration. This is part of an ongoing research project to explore alternative methods for CO2 capture that will be applicable to both retrofit and new plant construction.
Date: January 1, 2005
Creator: Ochs, Thomas L.; Patrick, Brian (Jupiter Oxygen Corp.); Oryshchyn, Danylo B.; Gross, Alex (Jupiter Oxygen Corp.); Summers, Cathy A.; Simmons, William (CoalTeck LLC) et al.
Partner: UNT Libraries Government Documents Department

Oxy-fuel combustion systems for pollution free coal fired power generation

Description: Jupiter Oxygen's patented oxy-fuel combustion systems1 are capable of economically generating power from coal with ultra-low emissions and increased boiler efficiency. Jupiter's system uses pure oxygen as the combustion agent, excluding air and thus nitrogen, concentrating CO2 and pollutants for efficient capture with near zero NOx production, reducing exhaust mass flow, and increasing radiant heat transfer. Flue-gas recirculation rates can be varied to add flexibility to new boiler designs using this technology. Computer modeling and thermal analysis have identified important design considerations in retrofit applications.
Date: January 1, 2004
Creator: Ochs, Thomas L.; Oryshchyn, Danylo B.; Gross, Dietrich (Jupiter Oxygen Corp.); Patrick, Brian (Jupiter Oxygen Corp.); Gross, Alex (Jupiter Oxygen Corp.); Dogan, Cindy et al.
Partner: UNT Libraries Government Documents Department