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RF Gun Photocathode Research at SLAC

Description: LCLS is presently operating with a third copper photocathode in the original rf gun, with a quantum efficiency (QE) of {approx}1 x 10{sup -4} and projected emittance {gamma}{var_epsilon}{sub x,y} = 0.45 {micro}m at 250 pC bunch charge. The spare LCLS gun is installed in the SLAC Accelerator Structure Test Area (ASTA), fully processed to high rf power. As part of a wider photocathode R and D program, a UV laser system and additional gun diagnostics are being installed at ASTA to measure QE, QE lifetime, and electron beam emittance under a variety of operating conditions. The near-term goals are to test and verify the spare photocathode production/installation sequence, including transfer from the final holding chamber to the rf gun. Mid- and longer-term goals include development of a rigorous understanding of plasma and laser-assisted surface conditioning and investigation of new, high-QE photocathode materials. In parallel, an x-ray photoemission spectroscopy station is nearing completion, to analyze Cu photocathode surface chemistry. In this paper we review the status and anticipated operating parameters of ASTA and the spectroscopy test chamber.
Date: May 16, 2012
Creator: Jongewaard, E.; Akre, R.; Brachmann, A.; Corbett, J.; Gilevich, S.; Grouev, K. et al.
Partner: UNT Libraries Government Documents Department

Insights on the Cuprate High Energy Anomaly Observed in ARPES

Description: Recently, angle-resolved photoemission spectroscopy has been used to highlight an anomalously large band renormalization at high binding energies in cuprate superconductors: the high energy 'waterfall' or high energy anomaly (HEA). The anomaly is present for both hole- and electron-doped cuprates as well as the half-filled parent insulators with different energy scales arising on either side of the phase diagram. While photoemission matrix elements clearly play a role in changing the aesthetic appearance of the band dispersion, i.e. creating a 'waterfall'-like appearance, they provide an inadequate description for the physics that underlies the strong band renormalization giving rise to the HEA. Model calculations of the single-band Hubbard Hamiltonian showcase the role played by correlations in the formation of the HEA and uncover significant differences in the HEA energy scale for hole- and electron-doped cuprates. In addition, this approach properly captures the transfer of spectral weight accompanying doping in a correlated material and provides a unifying description of the HEA across both sides of the cuprate phase diagram. We find that the anomaly demarcates a transition, or cross-over, from a quasiparticle band at low binding energies near the Fermi level to valence bands at higher binding energy, assumed to be of strong oxygen character.
Date: August 16, 2011
Creator: Moritz, Brian
Partner: UNT Libraries Government Documents Department

ARPES study of the evolution of band structure and charge density wave properties in RTe3 ( R=Y , La, Ce, Sm, Gd, Tb, and Dy)

Description: We present a detailed angle-resolved photoemission spectroscopy (ARPES) investigation of the RTe3 family, which sets this system as an ideal"textbook" example for the formation of a nesting driven charge density wave (CDW). This family indeed exhibits the full range of phenomena that can be associated to CDWinstabilities, from the opening of large gaps on the best nested parts of Fermi surface (up to 0.4 eV), to the existence of residual metallic pockets. ARPES is the best suited technique to characterize these features, thanks to its unique ability to resolve the electronic structure in k space. An additional advantage of RTe3 is that theband structure can be very accurately described by a simple two dimensional tight-binding (TB) model, which allows one to understand and easily reproduce many characteristics of the CDW. In this paper, we first establish the main features of the electronic structure by comparing our ARPES measurements with the linear muffin-tinorbital band calculations. We use this to define the validity and limits of the TB model. We then present a complete description of the CDW properties and of their strong evolution as a function of R. Using simple models, we are able to reproduce perfectly the evolution of gaps in k space, the evolution of the CDW wave vector with R, and the shape of the residual metallic pockets. Finally, we give an estimation of the CDWinteraction parameters and find that the change in the electronic density of states n (EF), due to lattice expansion when different R ions are inserted, has the correct order of magnitude to explain the evolution of the CDW properties.
Date: January 16, 2008
Creator: Hussain, Zahid; Brouet, Veronique; Yang, Wanli; Zhou, Xingjiang; Hussain, Zahid; Moore, R.G. et al.
Partner: UNT Libraries Government Documents Department

Investigations of the electronic structure and superconductivity in newly predicted metallic crystalline carbon

Description: This project investigated the electronic, structural, and optical properties of fullerene-based materials under high pressure/temperature conditions. It involved: (1) Raman spectroscopy and X-ray diffraction measurements on C-60 fullerenes compressed in diamond anvil cell, (2) synthesis of C-60 thin films and determination of their electronic structure by photoemission spectroscopy, and (3) investigations of the adsorption of water molecules into single-walled carbon nanotubes.
Date: August 16, 2007
Creator: Sharma, Suresh C
Partner: UNT Libraries Government Documents Department

Crystal Growth And Characterization of the Model High-Temperature Superconductor HgBa{sub 2}CuO{sub 4+{delta}}

Description: Since the discovery of high-transition-temperature (T{sub c}) superconductivity in La{sub 2-x}Ba{sub x}CuO{sub 4} in 1986, the study of the lamellar copper oxides has remained at the forefront of condensed matter physics. Apart from their unusually high values of T{sub c}, these materials also exhibit a variety of complex phenomena and phases. This rich behavior is a consequence of the lamellar crystal structures, formed of copper-oxygen sheets separated by charge reservoir layers, and of the strong electron-electron correlations in the copper-oxygen sheets. After two decades of intensive research, which has stimulated many valuable new insights into correlated electron systems in general, there remains a lack of consensus regarding the correct theory for high-T{sub c} superconductivity. The ultimate technological goal of room-temperature superconductivity might only be attained after the development of a deeper understanding of the mercury-based compounds HgBa{sub 2}Ca{sub n-1}Cu{sub n}OI{sub 2n+2+{delta}}, which currently exhibit the highest T{sub c}values. One very important issue in this regard is the role of electronic versus chemical and structural inhomogeneities in these materials, and the associated need to separate material-specific properties from those that are essential to superconductivity. Unfortunately, there has been remarkably little scientific work on the mercury-based compounds because sizable crystals have not been available; quantitative measurements of any kind would be invaluable benchmarks for testing the theories of high-T{sub c} superconductivity. The compounds HgBa{sub 2}Ca{sub n-1}Cu{sub n}OI{sub 2n+2+{delta}} can be viewed as model systems not only because of their record high-T{sub c} values, but also because of their high-symmetry crystal structures. Of particular interest is the simplest member of this materials family, HgBa{sub 2}CuO{sub 4+{delta}} (Hg1201), which possesses only one copper-oxygen sheet per unit cell (n = 1), as shown schematically in Figure 1a. The largest crystals obtained by previous growth methods do not exceed 1 mm{sup 3}, and hence are insufficient ...
Date: March 16, 2007
Creator: Zhao, Xudong; Yu, Guichuan; Cho, Yong-Chan; Chabot-Couture, Guillaume; Barisic, Neven; Bourges, Philippe et al.
Partner: UNT Libraries Government Documents Department

Switching a magnetic vortex by interlayer coupling in epitaxially grown Co/Cu/Py/Cu(001) trilayer disks

Description: Epitaxial Py/Cu/Co/Cu(001) trilayers were patterned into micron sized disks and imaged using element-specific photoemission electron microscopy. By varying the Cu spacer layer thickness, we study how the coupling between the two magnetic layers influences the formation of magnetic vortex states. We find that while the Py and Co disks form magnetic vortex domains when the interlayer coupling is ferromagnetic, the magnetic vortex domains of the Py and Co disks break into anti-parallel aligned multidomains when the interlayer coupling is antiferromagnetic. We explain this result in terms of magnetic flux closure between the Py and Co layers for the antiferromagnetic coupling case.
Date: July 16, 2010
Creator: Wu, J.; Carlton, D.; Oelker, E.; Park, J. S.; Jin, E.; Arenholz, E. et al.
Partner: UNT Libraries Government Documents Department

Activation Layer Stabilization of High Polarization Photocathodes in Sub-Optimal RF Gun Environments

Description: Specific activation recipes for bulk, 100 nm thick MBE grown and high polarization III-V photocathode material have been developed which mitigate the effects of exposure to background gasses. Lifetime data using four representative gasses were acquired for bulk GaAs, 100 nm unstrained GaAs and strained superlattice GaAs/GaAsP, all activated both with Cs and then Cs and Li (bi-alkali). Each photoemitter showed marked resilience improvement when activated using the bi-alkali recipe compared to the standard single alkali recipe. A dual alkali activation system at SLAC was constructed, baked and commissioned with the purpose of performing spin-polarization measurements on electrons emitted from the bi-alkali activated surfaces. An end station at SSRL was configured with the required sources for energy resolved photoemission measurements on the bi-alkali activated and CO2 dosed surfaces. The bi-alkali recipes were successfully implemented at SLAC/SSRL. Measurements at SLAC of the photoelectron spin-polarization from the modified activation surface showed no sign of a change in value compared to the standard activated material, i.e., no ill effects. Analysis of photoemission data indicates that the addition of Li to the activation layer results in a multi-layer structure. The presence of Li in the activation layer also acts as an inhibitor to CO2 absorption, hence better lifetimes in worse vacuum were achieved. The bi-alkali activation has been tested on O2 activated GaAs for comparison with NF3 activated surfaces. Comparable resilience to CO2 exposure was achieved for the O2 activated surface. An RF PECVD amorphous silicon growth system was modified to allow high temperature heat cleaning of GaAs substrates prior to film deposition. Growth versus thickness data were collected. Very thin amorphous silicon germanium layers were optimized to exhibit good behavior as an electron emitter. Growth of the amorphous silicon germanium films on the above substrates was fine tuned with respect to time and ...
Date: November 16, 2010
Creator: Mulhollan, Gregory A.
Partner: UNT Libraries Government Documents Department

DEVELOPMENT OF NEXT-GENERATION DETECTORS AND INSTRUMENTATION FOR PHOTOELECTRON SPECTROSCOPY, DIFFRACTION AND HOLOGRAPHY

Description: We have developed a new multichannel detector for use in photoelectron spectroscopy (as well as other types of high-count-rate spectroscopy) that will operate at rates of up to 1 GHz. Such detectors are crucial to the full utilization of the high-brightness radiation generated by third-generation synchrotron radiation sources. In addition, new software and hardware has been developed to permit rapidly and accurately scanning photoelectron spectra that will be accumulated in as little as a 200 micros. A versatile next-generation sample goniometer permitting equally rapid scanning of specimen angles or photon energies for angle-resolved photoemission studies, photoelectron diffraction, and photoelectron holography measurements, and cooling to below 10K has also been designed and constructed. These capabilities have been incorporated into a unique photoelectron spectrometer/diffractometer at the Advanced Light Source of the Lawrence Berkeley National Laboratory; this experimental system includes ultrahigh energy resolution, in situ rotation, variable polarization, and optional spin detection. This overall system is now being used in studies of a variety of problems including magnetic metals and oxides; metal/metal, metal/metal oxide, and metal-oxide/metal-oxide multilayers; and systems exhibiting giant and colossal magnetoresistance.
Date: October 16, 2005
Creator: Charles S. Fadley, Principal Investigator
Partner: UNT Libraries Government Documents Department