Studies of Novel Quantum Phenomena in Ruthenates

PDF Version Also Available for Download.

Description

Strongly correlated oxides have been the subject of intense study in contemporary condensed matter physics, and perovskite ruthenates (Sr,Ca)n+1RunO3n+1 have become a new focus in this field. One of important characteristics of ruthenates is that both lattice and orbital degrees of freedom are active and are strongly coupled to charge and spin degrees of freedom. Such a complex interplay of multiple degrees of freedom causes the properties of ruthenates to exhibit a gigantic response to external stimuli under certain circumstances. Magnetic field, pressure, and chemical composition all have been demonstrated to be effective in inducing electronic/magnetic phase transitions in ruthenates. ... continued below

Physical Description

4 images; 582 KB; 11 pages

Creation Information

Mao, Zhiqiang April 8, 2011.

Context

This report is part of the collection entitled: Office of Scientific & Technical Information Technical Reports and was provided by UNT Libraries Government Documents Department to Digital Library, a digital repository hosted by the UNT Libraries. More information about this report can be viewed below.

Who

People and organizations associated with either the creation of this report or its content.

Author

Sponsor

Publisher

Provided By

UNT Libraries Government Documents Department

Serving as both a federal and a state depository library, the UNT Libraries Government Documents Department maintains millions of items in a variety of formats. The department is a member of the FDLP Content Partnerships Program and an Affiliated Archive of the National Archives.

Contact Us

What

Descriptive information to help identify this report. Follow the links below to find similar items on the Digital Library.

Description

Strongly correlated oxides have been the subject of intense study in contemporary condensed matter physics, and perovskite ruthenates (Sr,Ca)n+1RunO3n+1 have become a new focus in this field. One of important characteristics of ruthenates is that both lattice and orbital degrees of freedom are active and are strongly coupled to charge and spin degrees of freedom. Such a complex interplay of multiple degrees of freedom causes the properties of ruthenates to exhibit a gigantic response to external stimuli under certain circumstances. Magnetic field, pressure, and chemical composition all have been demonstrated to be effective in inducing electronic/magnetic phase transitions in ruthenates. Therefore, ruthenates are ideal candidates for searching for novel quantum phenomena through controlling external parameters. The objective of this project is to search for novel quantum phenomena in ruthenate materials using high-quality single crystals grown by the floating-zone technique, and investigate the underlying physics. The following summarizes our accomplishments. We have focused on trilayered Sr4Ru3O10 and bilayered (Ca1-xSrx)3Ru2O7. We have succeeded in growing high-quality single crystals of these materials using the floating-zone technique and performed systematic studies on their electronic and magnetic properties through a variety of measurements, including resistivity, Hall coefficient, angle-resolved magnetoresistivity, Hall probe microscopy, and specific heat. We have also studied microscopic magnetic properties for some of these materials using neutron scattering in collaboration with Los Alamos National Laboratory. We have observed a number of unusual exotic quantum phenomena through these studies, such as an orbital selective metamagnetic transition, bulk spin valve effect, and a heavy-mass nearly ferromagnetic state with a surprisingly large Wilson ratio. Our work has also revealed underlying physics of these exotic phenomena. Exotic phenomena of correlated electron has been among central topics of contempary condensed matter physics. Ultrfast phase transitions accompanied by switching of conductivity or magnetization in stronly correlated materials are believed to be promising in developing next generation of transistors. Our work on layered ruthenates has remarkably advanced our understanding of how the exotic phenomena of correlated electrons is governed by the complex interplay between charge, spin, lattice and orbital degrees of freedom. In addition to studies on ruthenates, we have also expanded our research to the emerging field of Fe-based superconductors, focusing on the iron chalcogenide Fe1+y(Te1-xSex) superconductor system. We first studied the superconductivity of this alloy system following the discovery of superconductivity in FeSe using polycrystalline samples. Later, we successfuly grew high-quality single crystals of these materials. Using these single crystals, we have determined the magnetic structure of the parent compound Fe1+yTe, observed spin resonance of superconducting state in optimally doped samples, and established a phase diagram. Our work has produced an important impact in this burgeoning field. The PI presented an invited talk on this topic at APS March meeting in 2010. We have published 19 papers in these two areas (one in Nature materials, five in Physical Review Letters, and nine in Physical Review B) and submitted two (see the list of publications attached below).

Physical Description

4 images; 582 KB; 11 pages

Language

Item Type

Identifier

Unique identifying numbers for this report in the Digital Library or other systems.

  • Report No.: DOE/07ER46358-3
  • Grant Number: FG02-07ER46358
  • DOI: 10.2172/1010920 | External Link
  • Office of Scientific & Technical Information Report Number: 1010920
  • Archival Resource Key: ark:/67531/metadc832624

Collections

This report is part of the following collection of related materials.

Office of Scientific & Technical Information Technical Reports

Reports, articles and other documents harvested from the Office of Scientific and Technical Information.

Office of Scientific and Technical Information (OSTI) is the Department of Energy (DOE) office that collects, preserves, and disseminates DOE-sponsored research and development (R&D) results that are the outcomes of R&D projects or other funded activities at DOE labs and facilities nationwide and grantees at universities and other institutions.

What responsibilities do I have when using this report?

When

Dates and time periods associated with this report.

Creation Date

  • April 8, 2011

Added to The UNT Digital Library

  • May 19, 2016, 3:16 p.m.

Description Last Updated

  • Aug. 3, 2016, 6:03 p.m.

Usage Statistics

When was this report last used?

Yesterday: 0
Past 30 days: 0
Total Uses: 2

Interact With This Report

Here are some suggestions for what to do next.

Start Reading

PDF Version Also Available for Download.

International Image Interoperability Framework

IIF Logo

We support the IIIF Presentation API

Mao, Zhiqiang. Studies of Novel Quantum Phenomena in Ruthenates, report, April 8, 2011; United States. (digital.library.unt.edu/ark:/67531/metadc832624/: accessed September 20, 2018), University of North Texas Libraries, Digital Library, digital.library.unt.edu; crediting UNT Libraries Government Documents Department.