Final LDRD report : nanoscale mechanisms in advanced aging of materials during storage of spent %22high burnup%22 nuclear fuel.

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We present the results of a three-year LDRD project focused on understanding microstructural evolution and related property changes in Zr-based nuclear cladding materials towards the development of high fidelity predictive simulations for long term dry storage. Experiments and modeling efforts have focused on the effects of hydride formation and accumulation of irradiation defects. Key results include: determination of the influence of composition and defect structures on hydride formation; measurement of the electrochemical property differences between hydride and parent material for understanding and predicting corrosion resistance; in situ environmental transmission electron microscope observation of hydride formation; development of a predictive simulation ... continued below

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51 p.

Creation Information

Clark, Blythe G.; Rajasekhara, Shreyas; Enos, David George; Dingreville, Remi Philippe Michel; Doyle, Barney Lee; Hattar, Khalid Mikhiel et al. September 1, 2013.

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  • Sandia National Laboratories
    Publisher Info: Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)
    Place of Publication: Albuquerque, New Mexico

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Description

We present the results of a three-year LDRD project focused on understanding microstructural evolution and related property changes in Zr-based nuclear cladding materials towards the development of high fidelity predictive simulations for long term dry storage. Experiments and modeling efforts have focused on the effects of hydride formation and accumulation of irradiation defects. Key results include: determination of the influence of composition and defect structures on hydride formation; measurement of the electrochemical property differences between hydride and parent material for understanding and predicting corrosion resistance; in situ environmental transmission electron microscope observation of hydride formation; development of a predictive simulation for mechanical property changes as a function of irradiation dose; novel test method development for microtensile testing of ionirradiated material to simulate the effect of neutron irradiation on mechanical properties; and successful demonstration of an Idaho National Labs-based sample preparation and shipping method for subsequent Sandia-based analysis of post-reactor cladding.

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51 p.

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  • Report No.: SAND2013-8084
  • Grant Number: AC04-94AL85000
  • Office of Scientific & Technical Information Report Number: 1096269
  • Archival Resource Key: ark:/67531/metadc828502

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Office of Scientific & Technical Information Technical Reports

Reports, articles and other documents harvested from the Office of Scientific and Technical Information.

Office of Scientific and Technical Information (OSTI) is the Department of Energy (DOE) office that collects, preserves, and disseminates DOE-sponsored research and development (R&D) results that are the outcomes of R&D projects or other funded activities at DOE labs and facilities nationwide and grantees at universities and other institutions.

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  • September 1, 2013

Added to The UNT Digital Library

  • May 19, 2016, 9:45 a.m.

Description Last Updated

  • June 17, 2016, 3:13 p.m.

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Clark, Blythe G.; Rajasekhara, Shreyas; Enos, David George; Dingreville, Remi Philippe Michel; Doyle, Barney Lee; Hattar, Khalid Mikhiel et al. Final LDRD report : nanoscale mechanisms in advanced aging of materials during storage of spent %22high burnup%22 nuclear fuel., report, September 1, 2013; Albuquerque, New Mexico. (digital.library.unt.edu/ark:/67531/metadc828502/: accessed October 20, 2017), University of North Texas Libraries, Digital Library, digital.library.unt.edu; crediting UNT Libraries Government Documents Department.