Plutonium Assay in Soil at the BRC Threshold

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The Atomic Weapons Establishment (AWE) at Aldermaston has investigated the performance of low and high-resolution gamma-ray detectors for plutonium (Pu) assay in soil at the UK Below Regulatory Concern (BRC) threshold (0.4 Bq/g above the natural background activity level). The goal was a rapid and economical technique for sorting large volumes of lightly contaminated soils into above and BRC fractions. The strategy involved utilizing the relatively high yield 60 keV emission from Am-241 ingrowth (Pu-241 daughter) and known isotopic ratios. This paper covers the determination of detector response factors for an Am-241 source positioned at various locations within a circular ... continued below

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6 pages

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Miller, T. February 25, 2003.

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Description

The Atomic Weapons Establishment (AWE) at Aldermaston has investigated the performance of low and high-resolution gamma-ray detectors for plutonium (Pu) assay in soil at the UK Below Regulatory Concern (BRC) threshold (0.4 Bq/g above the natural background activity level). The goal was a rapid and economical technique for sorting large volumes of lightly contaminated soils into above and BRC fractions. The strategy involved utilizing the relatively high yield 60 keV emission from Am-241 ingrowth (Pu-241 daughter) and known isotopic ratios. This paper covers the determination of detector response factors for an Am-241 source positioned at various locations within a circular tray of soil. These factors were weighted, according to the relative volumes that they represent, in order to derive a uniform response factor and quantify the systematic error for non-uniform activity distributions. Detection limits and random errors were also derived from the counting data. The high-resolution detector was shown to have the best detection levels and lowest systematic and random errors. However, uncertainties for non-uniform distributions of contamination were relatively large. Hence, analyzing soils at the BRC threshold would only be feasible if contamination was well distributed throughout the soil sample being monitored. Fortunately, contaminated land at AWE is generally homogeneous and so the technique has wide applicability.

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6 pages

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  • Waste Management 2003 Symposium, Tucson, AZ (US), 02/23/2003--02/27/2003

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  • Report No.: none
  • Office of Scientific & Technical Information Report Number: 827183
  • Archival Resource Key: ark:/67531/metadc782541

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Office of Scientific & Technical Information Technical Reports

Reports, articles and other documents harvested from the Office of Scientific and Technical Information.

Office of Scientific and Technical Information (OSTI) is the Department of Energy (DOE) office that collects, preserves, and disseminates DOE-sponsored research and development (R&D) results that are the outcomes of R&D projects or other funded activities at DOE labs and facilities nationwide and grantees at universities and other institutions.

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  • February 25, 2003

Added to The UNT Digital Library

  • Dec. 3, 2015, 9:30 a.m.

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  • April 27, 2016, 1:38 p.m.

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Miller, T. Plutonium Assay in Soil at the BRC Threshold, article, February 25, 2003; Tucson, Arizona. (digital.library.unt.edu/ark:/67531/metadc782541/: accessed December 13, 2017), University of North Texas Libraries, Digital Library, digital.library.unt.edu; crediting UNT Libraries Government Documents Department.