REFORMULATION OF COAL-DERIVED TRANSPORTATION FUELS: SELECTIVE OXIDATION OF CARBON MONOXIDE ON METAL FOAM CATALYSTS Page: 4 of 74
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Table of Contents
Table of Contents iii
List of Graphical Materials v
1.1 Preferential Oxidation 1
1.2 Literature Review 2
1.3 Metal Foam Support 3
2. Executive Summary 4
3.1 Catalyst Preparation (Metal Foams, Ceramic Monoliths,
Provided by PFCT) 6
3.2 Catalyst Preparation (NCSU) 6
3.3 Catalyst Preparation (Clemson) 7
3.4 Reactor System (NCSU) 7
3.5 Reaction System (Clemson) 8
3.6 Testing Conditions (NCSU) 8
3.7 Reaction Measurements (Clemson) 9
3.8 Catalyst Characterization (Clemson) 10
3.9 Isotopic-Transient Kinetic Analysis (ITKA) 10
4. Results and Discussion
4.1 Catalyst Screening 11
4.2 Reverse Water Gas Shift Reaction 12
4.3 Comparison of Metal Foam and Ceramic Monolith
4.3.1 Pt-Fe catalyst (No Pretreatment, Metal Foam) 14
4.3.2 Pt-Fe catalyst (No Pretreatment, Foam/Monolith) 15
4.3.3 Pt-Fe catalyst (Pretreatment, Foam/Monolith) 15
4.3.4 Pt-Fe catalyst (Transients, Foam/Monolith) 16
4.4 Effect of Operating Conditions
4.4.1 02/CO Ratio 17
4.4.2 Space Velocity / Linear Velocity 18
4.5 Testing of "Identical" Individual Pieces (Ceramic Monolith
and Metal Foam) 21
4.6 Metal Monolith and Ceramic Foam 21
4.7 ICP/BET (NCSU) 22
4.8 BET Surface Area (Clemson) 22
4.9 X-ray Powder Diffusion 22
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Chin, Mr. Paul; Sun, Dr. Xiaolei; Roberts, Professor George W.; Spivey, Professor James J.; Sirijarhuphan, Mr. Amornmart; Dr. James G. Goodwin, Jr. et al. REFORMULATION OF COAL-DERIVED TRANSPORTATION FUELS: SELECTIVE OXIDATION OF CARBON MONOXIDE ON METAL FOAM CATALYSTS, report, December 31, 2002; United States. (digital.library.unt.edu/ark:/67531/metadc737502/m1/4/: accessed November 17, 2018), University of North Texas Libraries, Digital Library, digital.library.unt.edu; crediting UNT Libraries Government Documents Department.