Identification and temporal behavior of radical intermediates formed during the combustion and pyrolysis of gaseous fuels: Kinetic pathways to soot formation. Final performance report, July 1, 1997 - September 30, 2000

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A shock tube coupled to a time-of-flight mass spectrometer has been employed to analyze the dynamic behavior of reactants, products, and intermediates in those reaction systems which are most pertinent to understanding the chemistry attendant to the soot formation process. The measurement of the decay rates of the reactants, the rate of formation of intermediates and products have been used to determine rate constants over a wide temperature range. Recent examples include the pyrolyses of allene, propyne, pyrazine, pyrimidine, pyridine, acetylene, furan, cyclopentadiene, and methylcyclopentadiene.

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12 p.

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Kern, Ralph D. September 30, 2000.

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A shock tube coupled to a time-of-flight mass spectrometer has been employed to analyze the dynamic behavior of reactants, products, and intermediates in those reaction systems which are most pertinent to understanding the chemistry attendant to the soot formation process. The measurement of the decay rates of the reactants, the rate of formation of intermediates and products have been used to determine rate constants over a wide temperature range. Recent examples include the pyrolyses of allene, propyne, pyrazine, pyrimidine, pyridine, acetylene, furan, cyclopentadiene, and methylcyclopentadiene.

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12 p.

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OSTI as DE00809793

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Medium: P; Size: 12 pages

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  • September 30, 2000

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  • Oct. 18, 2015, 6:40 p.m.

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Thumbnail image of item number 1 in: 'Identification and temporal behavior of radical intermediates formed during the combustion and pyrolysis of gaseous fuels: Kinetic pathways to soot formation. Final performance report, July 1, 1997 - September 30, 2000'.
Thumbnail image of item number 2 in: 'Identification and temporal behavior of radical intermediates formed during the combustion and pyrolysis of gaseous fuels: Kinetic pathways to soot formation. Final performance report, July 1, 1997 - September 30, 2000'.
Thumbnail image of item number 3 in: 'Identification and temporal behavior of radical intermediates formed during the combustion and pyrolysis of gaseous fuels: Kinetic pathways to soot formation. Final performance report, July 1, 1997 - September 30, 2000'.
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Kern, Ralph D. Identification and temporal behavior of radical intermediates formed during the combustion and pyrolysis of gaseous fuels: Kinetic pathways to soot formation. Final performance report, July 1, 1997 - September 30, 2000, report, September 30, 2000; United States. (https://digital.library.unt.edu/ark:/67531/metadc733995/: accessed October 5, 2026), University of North Texas Libraries, UNT Digital Library, https://digital.library.unt.edu; crediting UNT Libraries Government Documents Department.

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