Steady-state and transient catalytic oxidation and coupling of methane

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This project addresses the conversion of methane from natural gas into ethane, ethylene and higher hydrocarbons. Our research explores the mechanistic and practical implications of carrying out the methane oxidative coupling reaction in reactor designs other than conventional packed-beds with co-fed reactants. These alternate reactor designs are needed to prevent the full oxidation of methane, which limits C{sub 2}, yields in methane oxidative coupling reactions. The research strategy focuses on preventing contact between the 0{sub 2} reactant required for favorable overall thermodynamics and the C{sub 2+} products of methane coupling. The behavior of various reactor designs are simulated using detailed ... continued below

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11 p.

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Iglesia, E.; Perry, D.L. & Heinemann, H. June 1, 1995.

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Description

This project addresses the conversion of methane from natural gas into ethane, ethylene and higher hydrocarbons. Our research explores the mechanistic and practical implications of carrying out the methane oxidative coupling reaction in reactor designs other than conventional packed-beds with co-fed reactants. These alternate reactor designs are needed to prevent the full oxidation of methane, which limits C{sub 2}, yields in methane oxidative coupling reactions. The research strategy focuses on preventing contact between the 0{sub 2} reactant required for favorable overall thermodynamics and the C{sub 2+} products of methane coupling. The behavior of various reactor designs are simulated using detailed kinetic transport models. These simulations have suggested that the best way to prevent high C0{sub 2} yields is to separate the oxygen and hydrocarbon streams altogether. As a result, the project has focused on the experimental demonstration of proton transport membrane reactors for the selective conversion of methane into higher hydrocarbons.

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11 p.

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OSTI as DE95012321

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  • Natural gas research, development and demonstration contractors review meeting, Baton Rouge, LA (United States), 4-6 Apr 1995

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  • Other: DE95012321
  • Report No.: DOE/MC--00098-95/C0463
  • Report No.: CONF-950494--21
  • Grant Number: AC03-76SF00098
  • Office of Scientific & Technical Information Report Number: 69433
  • Archival Resource Key: ark:/67531/metadc711568

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Office of Scientific & Technical Information Technical Reports

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  • June 1, 1995

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  • Sept. 12, 2015, 6:31 a.m.

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  • April 5, 2016, 10:49 a.m.

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Iglesia, E.; Perry, D.L. & Heinemann, H. Steady-state and transient catalytic oxidation and coupling of methane, article, June 1, 1995; California. (digital.library.unt.edu/ark:/67531/metadc711568/: accessed November 17, 2018), University of North Texas Libraries, Digital Library, digital.library.unt.edu; crediting UNT Libraries Government Documents Department.