Experimental studies in high temperature aqueous chemistry at Oak Ridge National Laboratory

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Experimental research is conducted and models developed in a long- standing program at Oak Ridge on aqueous chemistry at high temperatures of broad classes of electrolytes emphasizing thermodynamics of reaction equilibria and excess thermodynamic properties of electrolytes. Experimental methods, their capabilities, data analysis, and results are summarized. Relevance of the work to problems in power plants, natural and industrial processes as well as basic solution chemistry and geochemistry are given. Progress in potentiometry, electrical conductivity, flow calorimetry, and isopiestic research is described. Future in this field demands greater precision in measurements and significant gains in our understanding of the solvation ... continued below

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12 p.

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Mesmer, R.E.; Palmer, D.A.; Simonson, J.M.; Holmes, H.F.; Ho, P.C.; Wesolowski, D.J. et al. January 1, 1996.

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Description

Experimental research is conducted and models developed in a long- standing program at Oak Ridge on aqueous chemistry at high temperatures of broad classes of electrolytes emphasizing thermodynamics of reaction equilibria and excess thermodynamic properties of electrolytes. Experimental methods, their capabilities, data analysis, and results are summarized. Relevance of the work to problems in power plants, natural and industrial processes as well as basic solution chemistry and geochemistry are given. Progress in potentiometry, electrical conductivity, flow calorimetry, and isopiestic research is described. Future in this field demands greater precision in measurements and significant gains in our understanding of the solvation phenomena especially in the vicinity and beyond the critical point for water. The communities who do research on scattering, spectroscopy, and computer simulations can help guide these efforts through studies at extreme conditions.

Physical Description

12 p.

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OSTI as DE96014607

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  • 7. international symposium on solubility phenomena, Leoben (Austria), 22-25 Jul 1996

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  • Other: DE96014607
  • Report No.: CONF-960727--1
  • Grant Number: AC05-96OR22464
  • Office of Scientific & Technical Information Report Number: 380269
  • Archival Resource Key: ark:/67531/metadc685715

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Office of Scientific & Technical Information Technical Reports

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  • January 1, 1996

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  • July 25, 2015, 2:20 a.m.

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  • Jan. 25, 2016, 3:53 p.m.

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Mesmer, R.E.; Palmer, D.A.; Simonson, J.M.; Holmes, H.F.; Ho, P.C.; Wesolowski, D.J. et al. Experimental studies in high temperature aqueous chemistry at Oak Ridge National Laboratory, article, January 1, 1996; Tennessee. (digital.library.unt.edu/ark:/67531/metadc685715/: accessed December 16, 2017), University of North Texas Libraries, Digital Library, digital.library.unt.edu; crediting UNT Libraries Government Documents Department.