ESC FY2002 Annual Report: Synchrotron-Radiation-Based Photoelectron Spectroscopy at the Advanced Light Source

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Despite recent intensive experimental effort, the electronic structure of Pu, particularly {delta}-Pu, remains ill defined. An evaluation of our previous synchrotron-radiation-based investigation of {alpha}-Pu and {delta}-Pu has lead to a new paradigm for the interpretation of photoemission spectra of U, Np, {alpha}-Pu, {delta}-Pu and Am. This approach is founded upon a model in which spin and spin-orbit splittings are included in the picture of the 5f states and upon the observation of chiral/spin-dependent effects in non-magnetic systems. By extending a quantitative model developed for the interpretation of core level spectroscopy in magnetic systems, it is possible to predict the contributions … continued below

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Tobin, J G; Chung, B W; Schulze, R K & Shuh, D K October 4, 2002.

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  • Main Title: ESC FY2002 Annual Report: Synchrotron-Radiation-Based Photoelectron Spectroscopy at the Advanced Light Source
  • Series Title: Fiscal Year 2002

Description

Despite recent intensive experimental effort, the electronic structure of Pu, particularly {delta}-Pu, remains ill defined. An evaluation of our previous synchrotron-radiation-based investigation of {alpha}-Pu and {delta}-Pu has lead to a new paradigm for the interpretation of photoemission spectra of U, Np, {alpha}-Pu, {delta}-Pu and Am. This approach is founded upon a model in which spin and spin-orbit splittings are included in the picture of the 5f states and upon the observation of chiral/spin-dependent effects in non-magnetic systems. By extending a quantitative model developed for the interpretation of core level spectroscopy in magnetic systems, it is possible to predict the contributions of the individual component states within the 5-f manifold. This has lead to a remarkable agreement between the results of the model and the previously collected spectra of U, Np, Pu and Am, particularly {delta}-Pu, and to a prediction of what we might expect to see in future spin-resolving experiments.

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PDF-FILE: 9 ; SIZE: 0.3 MBYTES pages

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  • Other Information: PBD: 4 Oct 2002

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  • October 4, 2002

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  • Jan. 23, 2019, 12:54 p.m.

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  • Feb. 6, 2019, 2:31 p.m.

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Tobin, J G; Chung, B W; Schulze, R K & Shuh, D K. ESC FY2002 Annual Report: Synchrotron-Radiation-Based Photoelectron Spectroscopy at the Advanced Light Source, report, October 4, 2002; California. (https://digital.library.unt.edu/ark:/67531/metadc1412666/: accessed April 16, 2024), University of North Texas Libraries, UNT Digital Library, https://digital.library.unt.edu; crediting UNT Libraries Government Documents Department.

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