Three small samples of zircalloy-2, obtained from a KER tube, were irradiated in the Quickie Facility in F Reactor for one, four, and nine months, respectively. Each sample weighed approximately two grams. One day after discharge from the reactor, the specific activity of each of the samples was essentially the same (about 150 mr/hr/gram at one foot in air). Attenuation measurements taken one day after discharge using lead plates yielded a ten-fold reduction in gamma intensity for each 0.95 inches of lead. This indicates that an enclosure for kilogram samples of zircalloy which have been irradiated for long periods of …
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Publisher Info:
General Electric Co., Richland, WA (United States). Hanford Atomic Products Operation
Place of Publication:
Richland, Washington
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Description
Three small samples of zircalloy-2, obtained from a KER tube, were irradiated in the Quickie Facility in F Reactor for one, four, and nine months, respectively. Each sample weighed approximately two grams. One day after discharge from the reactor, the specific activity of each of the samples was essentially the same (about 150 mr/hr/gram at one foot in air). Attenuation measurements taken one day after discharge using lead plates yielded a ten-fold reduction in gamma intensity for each 0.95 inches of lead. This indicates that an enclosure for kilogram samples of zircalloy which have been irradiated for long periods of time at fluxes up to 10{sup 14} neutrons per square centimeter per second should have six inch thick lead walls or the equivalent for gamma shielding. Based on the effective gamma energy and the half-life for the first day, it appears that Zr-89 may be the predominant isotope initially. After a few days, the half-life become long and gamma spectrometer measurements indicate the gamma softens revealing that Zr-95 might become the predominant isotope. However, isotopes were not determined specifically; impurities, other isotopes, or combination of isotopes could yield the same results.
Physical Description
6 p.
Notes
OSTI as DE94017101; Paper copy available at OSTI: phone, 865-576-8401, or email, reports@adonis.osti.gov
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