Gas-Phase Radiolysis of Propane

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Abstract. the direct and inert-gas radiolysis, as well as the vacuum ultra-violet photolysis of CD3CH2CD3, CH3CD2CH3 and C3H2+C3D3 mixtures have been investigated in the presence of radical scavengers. The major conclusions are : (a) at atmospheric pressures, neutral propane decomposition contributes to the observed products although to a lesser extent than parent ion decompositions ; (b) a variation in pressure has a pronounced effect on the fragmentation of the parent ion ; (c) the hydrogen atoms in the ethyl ion are randomized in the direct as well as in the inert-gas sensitized radiolysis ; (d) rearrangement in the parent ion … continued below

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9 pages ; illustrations.

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Ausloos, Pierre J.; Lias, Sharon G., 1935- & Sandoval, L. B., (Mrs.) May 31, 1963.

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Description

Abstract. the direct and inert-gas radiolysis, as well as the vacuum ultra-violet photolysis of CD3CH2CD3, CH3CD2CH3 and C3H2+C3D3 mixtures have been investigated in the presence of radical scavengers. The major conclusions are : (a) at atmospheric pressures, neutral propane decomposition contributes to the observed products although to a lesser extent than parent ion decompositions ; (b) a variation in pressure has a pronounced effect on the fragmentation of the parent ion ; (c) the hydrogen atoms in the ethyl ion are randomized in the direct as well as in the inert-gas sensitized radiolysis ; (d) rearrangement in the parent ion is of minor importance in the radiolysis ; (e) although the formation of propylene is related to the propyl ion, it is not necessarily produced by the neutralization of this ion.

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9 pages ; illustrations.

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  • Accession or Local Control No: metadc1201750
  • Report No.: CONF-224-6
  • SuDoc Number: Y 3.At 7:22/CONF-224-6
  • Archival Resource Key: ark:/67531/metadc1201750

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Technical Report Archive and Image Library

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  • May 31, 1963

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  • Aug. 27, 2019, 3:53 p.m.

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  • April 1, 2020, 4:06 p.m.

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Ausloos, Pierre J.; Lias, Sharon G., 1935- & Sandoval, L. B., (Mrs.). Gas-Phase Radiolysis of Propane, report, May 31, 1963; Oak Ridge, Tennessee.. (https://digital.library.unt.edu/ark:/67531/metadc1201750/: accessed January 15, 2025), University of North Texas Libraries, UNT Digital Library, https://digital.library.unt.edu; crediting UNT Libraries Government Documents Department.

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