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  Partner: UNT Libraries Government Documents Department
 Serial/Series Title: Argonne National Laboratory Reports
Physics Division Annual Review: April 1, 1994-March 31, 1995

Physics Division Annual Review: April 1, 1994-March 31, 1995

Date: August 1995
Creator: Argonne National Laboratory. Physics Division.
Description: Annual report of activities of the Argonne National Laboratory Physics Division, including heavy-ion nuclear physics research, operation and development of ATLAS, medium-energy nuclear physics research, theoretical physics, atomic and molecular physics research.
Contributing Partner: UNT Libraries Government Documents Department
Validation of the Generic TRUEX Model Using Data from TRUEX Demonstrations with Actual High-Level Waste

Validation of the Generic TRUEX Model Using Data from TRUEX Demonstrations with Actual High-Level Waste

Date: August 1995
Creator: Regalbuto, M. C.; Aase, S. B. & Vandegrift, G. F.
Description: The Generic TRUEX Model (GTM) was used to simulate three different counter-current flowsheet tests performed using mixer-settlers that had been carried out prior to 1993 in the Chemical Processing Facility, Tokai-works, of the Power Reactor and Nuclear Fuel Development Corporation (PNC) of Japan. The feed for the PNC runs was the highly active raffinate from reprocessing of spent fuel from fast breeder reactors. The PNC demonstration runs were planned without using the GTM. Results predicted by the GTM and those obtained experimentally by PNC for the three demonstration runs are compared. Effects of stage efficiency, nitrate complexation, temperature, and equipment type are also included.
Contributing Partner: UNT Libraries Government Documents Department
Aqueous Biphasic Extraction of Uranium and Thorium from Contaminated Soils : Final Report

Aqueous Biphasic Extraction of Uranium and Thorium from Contaminated Soils : Final Report

Date: July 1995
Creator: Chaiko, David J.; Gartelmann, J.; Henriksen, J. L.; Krause, T. R.; Deepak; Vojta, Y. et al.
Description: The aqueous biphasic extraction (ABE) process for soil decontamination involves the selective partitioning of solutes and fine particulates between two immiscible aqueous phases. The biphase system is generated by the appropriate combination of a water-soluble polymer (e.g., polyethylene glycol) with an inorganic salt (e.g., sodium carbonate). Selective partitioning results in 99 to 99.5% of the soil being recovered in the cleaned-soil fraction, while only 0.5 to 1% is recovered in the contaminant concentrate. The ABE process is best suited to the recovery of ultrafine, refractory material from the silt and clay fractions of soils. During continuous countercurrent extraction tests with soil samples from the Fernald Environmental Management Project site (Fernald, OH), particulate thorium was extracted and concentrated between 6- and 16-fold, while the uranium concentration was reduced from about 500 mg/kg to about 77 mg/kg. Carbonate leaching alone was able to reduce the uranium concentration only to 146 mg/kg. Preliminary estimates for treatment costs are approximately $160 per ton of dry soil. A detailed flowsheet of the ABE process is provided.
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Extraction of Long-Lived Radionuclides from Caustic Hanford Tank Waste Supernatants

Extraction of Long-Lived Radionuclides from Caustic Hanford Tank Waste Supernatants

Date: July 1995
Creator: Chaiko, David J.; Mertz, C. J.; Vojta, Y.; Henriksen, J. L.; Neff, R. & Takeuchi, M.
Description: A series of polymer-based extraction systems, based on the use of polyethylene glycols (PEGs) or polypropylene glycols (PPGs), was demonstrated to be capable of selective extraction and recovery of long-lived radionuclides, such as Tc-99 and I-129, from Hanford SY-101 tank waste, neutralized current acid waste, and single-shell tank waste simulants. During the extraction process, anionic species like TcO₄⁻ and I⁻ are selectively transferred to the less dense PEG-rich aqueous phase. The partition coefficients for a wide range of inorganic cations and anions, such as sodium, potassium, aluminum, nitrate, nitrite, and carbonate, are all less than one. The partition coefficients for pertechnetate ranged from 12 to 50, depending on the choice of waste simulant and temperature. The partition coefficient for iodide was about 5, while that of iodate was about 0.25. Irradiation of the PEG phase with gamma-ray doses up to 20 Mrad had no detectable effect on the partition coefficients. The most selective extraction systems examined were those based on PPGs, which exhibited separation factors in excess of 3000 between TcO₄⁻ and NO₃⁻/NO₂⁻. An advantage of the PPG-based system is minimization of secondary waste production. These studies also highlighted the need for exercising great care in extrapolating the partitioning behavior ...
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Information Exchange within the U.S. Department of Energy Pollution Prevention Community

Information Exchange within the U.S. Department of Energy Pollution Prevention Community

Date: July 1995
Creator: Thuot, James R.
Description: Improving Pollution Prevention and Waste Minimization Program (PP/WMIN) technologies, actions, and culture could be an important cost-cutting step for the US Department of Energy (DOE). Communicating ideas, concepts, process changes, and achievements is essential for the success of this program. The need to openly communicate ideas and concepts in a cost-effective manner is essential in an organization that has such diverse components as research and development, weapons production, and power generation. This approach is in contrast to the historic DOE culture developed within the cold war period in which compartmentalization, independence, and secrecy were stressed. DOE has now recognized that for any pollution prevention program to be successful, the many diverse elements of the organization must share information. Avenues for such information exchange are examined in this report.
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Nonlinear Dynamics of a Stack/Cable System

Nonlinear Dynamics of a Stack/Cable System

Date: July 1995
Creator: Cai, Y. & Chen, Shoei-Sheng
Description: In this study, we developed a coupled model of wind-induced vibration of a stack, based on an unsteady-flow theory and nonlinear dynamics of the stack's heavy elastic suspended cables. Numerical analysis was performed to identify excitation mechanisms. The stack was found to be excited by vortex shedding. Once lock-in resonance occurred, the cables were excited by the transverse motion of the stack. Large-amplitude oscillations of the cables were due to parametric resonance. Appropriate techniques have been proposed to alleviate the vibration problem.
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Technology Development Goals for Automotive Fuel Cell Power Systems

Technology Development Goals for Automotive Fuel Cell Power Systems

Date: July 1995
Creator: Thomas, C. E. & James, Brian D.
Description: Directed Technologies, Inc. has previously submitted a detailed technical assessment and concept design for a mid-size, five-passenger fuel cell electric vehicle (FCEV), under contract to Argonne National Laboratory. As a supplement to that contract, DTI has reviewed the literature and conducted a preliminary evaluation of two energy carriers for the FCEV: hydrogen and methanol. This report compares the estimated fuel efficiency, cost of producing and delivering the fuel, and the resultant life cycle costs of the FCEV when fueled directly by hydrogen and when fueled by methanol with on-board reforming to produce the required hydrogen-rich gas for the fuel cell. This work will be supplemented and expanded under the Ford contract with the Department of Energy to develop the FCEV and its fuel infrastructure.
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ANL Technical Support Program for DOE Environmental Restoration and Waste Management Annual Report October 1993 - September 1994

ANL Technical Support Program for DOE Environmental Restoration and Waste Management Annual Report October 1993 - September 1994

Date: June 1995
Creator: Bates, John K.
Description: A program was established for DOE Environmental Restoration and Waste Management (EM) to evaluate factors that are anticipated to affect waste glass reaction during repository disposal, especially in an unsaturated environment typical of what may be expected for the proposed Yucca Mountain repository site.
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Chemical Technology Division Annual Technical Report: 1994

Chemical Technology Division Annual Technical Report: 1994

Date: June 1995
Creator: Argonne National Laboratory. Chemical Technology Division.
Description: Annual report of the Argonne National Laboratory Chemical Technology Division (CMT) discussing the group's activities during 1994. These included electrochemical technology; fossil energy research; hazardous waste research; nuclear waste programs; separation science and technology; electrometallurgical technology; actinide recovery; applied physical chemistry; basic chemistry research; analytical chemistry.
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Argonne National Laboratory-East Site Environmental Report for Calendar Year 1994

Argonne National Laboratory-East Site Environmental Report for Calendar Year 1994

Date: May 1995
Creator: Golchert, N. W. & Kolzow, R. G.
Description: This report discusses the results of the environmental protection program at Argonne National Laboratory-East (ANL) for 1994. To evaluate the effects of ANL operations on the environment, samples of environmental media collected on the site, at the site boundary, and off the ANL site were analyzed and compared to applicable guidelines and standards. A variety of radionuclides was measured in air, surface water, groundwater, soil, grass, and bottom sediment samples. In addition, chemical constituents in surface water, groundwater, and ANL effluent water were analyzed.
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