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  Partner: UNT College of Arts and Sciences
 Department: Physics
 Language: English
Charge transfer equilibria in ambient-exposed epitaxial graphene on (0001) 6 H-SiC

Charge transfer equilibria in ambient-exposed epitaxial graphene on (0001) 6 H-SiC

Date: June 5, 2012
Creator: Sidorov, Anton N.; Gaskill, D. Kurt.; Buongiorno Nardelli, Marco; Tedesco, Joseph L.; Myers-Ward, Rachel L.; Eddy, Charles R. et al
Description: This article discusses charge transfer equilibria in ambient-exposed epitaxial graphene on (0001) 6 H-SiC. Abstract: The transport properties of electronic materials have been long interpreted independently from both the underlying bulk-like behavior of the substrate or the influence of ambient gases. This is no longer the case for ultra-thin graphene whose properties are dominated by the interfaces between the active material and its surroundings. Here, the authors show that the graphene interactions with its environments are critical for the electrostatic and electrochemical equilibrium of the active device layers and their transport properties. Based on the prototypical case of epitaxial graphene on (0001) 6 H-SiC and using a combination of 'in-situ' thermoelectric power and resistance measurements and simulations from first principles, the authors demonstrate that the cooperative occurrence of an electrochemically mediated charge transfer from the graphene to air, combined with the peculiar electronic structure of the graphene/SiC interface, explains the wide variation of measured conductivity and charge carrier type found in prior reports.
Contributing Partner: UNT College of Arts and Sciences
Coherent control of atomic excitation using off-resonant strong few-cycle pulses

Coherent control of atomic excitation using off-resonant strong few-cycle pulses

Date: October 20, 2010
Creator: Jha, Pankaj K.; Eleuch, Hichem & Rostovtsev, Yuri V.
Description: This article discusses coherent control of atomic excitation using off-resonant strong few-cycle pulses. Abstract: We study the dynamics of a two-level system driven by an off-resonance few-cycle pulse which has a phase jump ø at t = t₀, in contrast to many-cycle pulses, under the nonrotating-wave approximation (NRWA). We give a closed form analytical solution for the evolution of the probability amplitude |Cₐ(t)| for the upper level. Using the appropriate pulse parameters like the phase jump ø, jump time t₀, pulse width Շ, frequency ν, and Rabi frequency Ώ₀ the population transfer after the pulse is gone can be optimized and, for the pulse considered here, an enhancement factor of 10⁶-10⁸ was obtained.
Contributing Partner: UNT College of Arts and Sciences
Coherent control of refractive index in far-detuned Λ systems

Coherent control of refractive index in far-detuned Λ systems

Date: December 15, 2011
Creator: O'Brien, Chris; Anisimov, Petr M.; Rostovtsev, Yuri V. & Kocharovskaya, Olga
Description: This article discusses the coherent control of refraction index in far-detuned Λ systems. Abstract: Enhancement and control of the index of refraction in a mixture of two three-level atomic species that form a pair of far-detuned Λ schemes under two-photon resonance and has been studied. We employ the density-matrix approach to properly take population relaxation into account and to describe the interaction of each Λ system with the electromagnetic fields. Both Λ systems are driven by a corresponding far-detuned coherent field at one atomic transition and are probed by the same weak field. In the dressed-state basis, it represents a superposition of effective two-level subsystems with the positions, widths, and amplitudes of the resonances controlled by the driving fields and allows for efficient control of the susceptibility of the total system; leading to refractive index (RI) enhancement with vanishing absorption in the absence of amplification. We analyze the experimental implementation of such a system in a cell of Rb atoms with a natural abundance of isotopes. An upper limit estimate of the RI enhancement is obtained.
Contributing Partner: UNT College of Arts and Sciences
Coherent excitation of a two-level atom driven by a far-off-resonant classical field: Analytical solutions

Coherent excitation of a two-level atom driven by a far-off-resonant classical field: Analytical solutions

Date: March 15, 2010
Creator: Jha, Pankaj K. & Rostovtsev, Yuri V.
Description: This article discusses the coherent excitation of a two-level atom driven by a far-off-resonant classical field. Abstract: We present an analytical treatment of coherent excitation of a two-level atom driven by a far-off-resonant classical field. A class of pulse envelope is obtained for which this problem is exactly solvable. The solutions are given in terms of the Heun function, which is a generalization of the hypergeometric function. Degeneracy of the Heun to a hypergeometric equation can give all the exactly solvable pulse shapes of Gauss hypergeometric form from the generalized pulse shape obtained here. We discuss the application of the results obtained to the generation of soft x-ray and ultraviolet radiations.
Contributing Partner: UNT College of Arts and Sciences
Comment on "Modification of graphene properties due to electron-beam irradiation"

Comment on "Modification of graphene properties due to electron-beam irradiation"

Date: December 17, 2009
Creator: Jones, Jason D.; Ecton, Philip A.; Mo, Yudong & Pérez, José M.
Description: This article is a comment on another article titled 'Modification of graphene properties due to electron-beam irradiation'. These articles discuss the modification of graphene properties due to electron-beam irradiation.
Contributing Partner: UNT College of Arts and Sciences
Complex Materials for Molecular Spintronics Applications: Cobalt Bis(dioxolene) Valence Tautomers, from Molecules to Polymers

Complex Materials for Molecular Spintronics Applications: Cobalt Bis(dioxolene) Valence Tautomers, from Molecules to Polymers

Date: October 16, 2012
Creator: Calzolari, Arrigo; Chen, Yifeng; Lewis, Geoffrey F.; Dougherty, Daniel B.; Shultz, David A. & Buongiorno Nardelli, Marco
Description: This article discusses complex materials for molecular spintronics applications. Abstract: Using first principles calculations, the authors predict a complex multifunctional behavior in cobalt bis(dioxolene) valence tautomeric compounds. Molecular spin-state switching is shown to dramatically alter electronic properties and corresponding transport properties. This spin state dependence has been demonstrated for technologically relevant coordination polymers of valence tautomers as well as for novel conjugated polymers with valence tautomeric functionalization. As a result, these materials are proposed as promising candidates for spintronic devices that can couple magnetic bistability with novel electrical and spin conduction properties. The authors' findings pave the way to the fundamental understanding and future design of active multifunctional organic materials for spintronics applications.
Contributing Partner: UNT College of Arts and Sciences
Complexity and Synchronization

Complexity and Synchronization

Date: August 14, 2009
Creator: Turalska, Malgorzata; Lukovic, Mirko; West, Bruce J. & Grigolini, Paolo
Description: This article discusses complexity and synchronization. Abstract: We study a fully connected network (cluster) of interacting two-state units as a model of cooperative decision making. Each unit in isolation generates a Poisson process with rate g. We show that when the number of nodes is finite, the decision-making process becomes intermittent. The decision-time distribution density is characterized by inverse power-law behavior with index μ=1.5 and is exponentially truncated. We find that the condition of perfect consensus is recovered by means of a fat tail that becomes more and more extended with increasing numbers of nodes N. The intermittent dynamics of the global variable are described by the motion of a particle in a double well potential. The particle spends a portion of the total time τs at the top of the potential barrier. Using theoretical and numerical arguments it is proved that τs ∝ (1/g)1n(const X N). The second portion of its time, τk, is spent by the particle at the bottom of the potential well and it is given by τk=(1/g)exp(const X N). We show that the time τk is responsible for the Kramers fat tail. This generates a stronger ergodicity breakdown than that generated by the inverse power ...
Contributing Partner: UNT College of Arts and Sciences
Compression and Diffusion: A Joint Approach to Detect Complexity

Compression and Diffusion: A Joint Approach to Detect Complexity

Date: February 2003
Creator: Allegrini, Paolo; Benci, V. (Vieri); Grigolini, Paolo; Hamilton, P.; Ignaccolo, Massimiliano; Menconi, G. et al
Description: This article discusses a joint approach to detect complexity. Abstract: The adoption of the Kolmogorov-Sinai (KS) entropy is becoming a popular research tool among physicists, especially when applied to a dynamical system fitting the conditions of validity of the Pesin theorem. The study of time series that are a manifestation of system dynamics whose rules are either unknown or too complex for a mathematical treatment, is still a challenge since the KS entropy is not computable, in general, in that case. Here the authors present a plan of action based on the joint action of two procedures, both related to the KS entropy, but compatible with computer implementation through fast and efficient programs. The former procedure, called Compression Algorithm Sensitive To Regularity (CASToRe), establishes the amount of order by the numerical evaluation of algorithmic compressibility. The latter, called Complex Analysis of Sequences via Scaling AND Randomness Assessment (CASSANDRA), establishes the complexity degree through the numerical evaluation of the strength of an anomalous effect. This is the departure, of the diffusion process generated by the observed fluctuations, from ordinary Brownian motion. The CASSANDRA algorithm shares with CASToRe a connection with the Kolmogorov complexity. This makes both algorithms especially suitable to study ...
Contributing Partner: UNT College of Arts and Sciences
Control of chaos in a CO2 laser

Control of chaos in a CO2 laser

Date: September 5, 1994
Creator: Pérez, José M.; Steinshnider, J.; Stallcup, Richard E. & Aviles, A. F.
Description: This article discusses the control of chaos in a CO2 laser. Abstract: We report the experimental control of chaos in an optically modulated CO2 laser. The CO2 laser was driven into chaos by injecting a feedback beam modulated by an electro-optical modulator. Control of chaos was achieved using a modified proportional feedback technique in which the control pulses were delayed by approximately one relaxation period. Using this technique, it was possible to control unstable periodic orbits up to period 6.
Contributing Partner: UNT College of Arts and Sciences
Controllable enhanced dragging of light in ultradispersive media

Controllable enhanced dragging of light in ultradispersive media

Date: July 5, 2012
Creator: Rostovtsev, Yuri V. & Davuluri, Sankar
Description: This article discusses controllable enhanced dragging of light in ultradispersive media. Abstract: We have theoretically demonstrated an enhanced Fizeau effect due to dragging the light that occurs when the group velocity of light is ultraslow. The proposed experiment can be done in a cell of atomic Rb vapor under conditions such that the group velocity of light is of the order of a few hundred meters per second. We show theoretically that higher-order dispersion can influence the Fizeau effect and can be observed experimentally. It has been shown that the change of phase is sensitive to the motion of the cell with the speed of the order of 10⁻³ cm/s and for possible displacements as small as 10 Å. The enhanced dragging effect can be applied for position control, detection of slow mechanical motion, and efficient modulators of light.
Contributing Partner: UNT College of Arts and Sciences