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Department:
Ion Beam Modification and Analysis Laboratory
Decade:
1990-1999
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UNT Scholarly Works
Charge-state dependence of K-shell x-ray production in aluminum by 2-12-MeV carbon ions
Date: June 1996
Creator: Sun, H. L.; Yu, Y. C.; Lin, E. K.; Wang, C. W.; Duggan, Jerome L.; Azordegan, A. R. et al
Description: This article discusses charge-state dependence of K-shell x-ray production in aluminum by 2-12-MeV carbon ions. Abstract: Charge-state dependence for K-shell x-ray production cross sections in 13Al bombarded by 2-12-MeV 6C ions with charge states from 2+ to 6+ was measured using a Si(Li) detector. A thin Al target was used to ensure single collision conditions. Contributions of the electron capture as well as direct ionization to the inner-shell ionization were determined by an analysis of the charge-state dependence of the target x-ray production. The measurements are compared with the prediction of the ECPSSR theory using a single-hole fluorescence yield. The ECPSSR theory is based on the perturbed stationary state (PSS) formalism and relativistic efforts (R) for the target electrons, and energy loss (E) and Coulomb deflection (C) of the projectile. In general, this theory gives reasonable agreement with the data for carbon ions without K vacancies while it overpredicts the data for carbon ions with K vacancies. The significant underprediction of the data at the lowest energy is likely associated with the molecular-orbital effect that is not accounted for in the ECPSSR theory.
Contributing Partner: UNT College of Arts and Sciences
Permallink:digital.library.unt.edu/ark:/67531/metadc139497/
Charge-state dependence of M-shell x-ray production in 67Ho by 2-12-MeV carbon ions
Date: November 1995
Creator: Yu, Y. C.; Sun, H. L.; Duggan, Jerome L.; McDaniel, Floyd Del. (Floyd Delbert), 1942-; Yin, J. Y. & Lapicki, G.
Description: This article discusses charge-state dependence of M-shell x-ray production in 67Ho by 2-12-MeV carbon ions. Abstract: Charge-state dependence of M-shell x-ray production cross sections of 67Ho bombarded by 2-12-MeV carbon ions, with and without K-shell vacancies, were measured using a windowless Si(Li) x-ray detector with a full-width-at-half-maximum resolution of 135 eV at 5.9 keV. Carbon ions of different charge states were produced using a postacceleration, nitrogen gas stripping cell. The carbon ions were then magnetically analyzed to select the desired charge state and energy before entering the target chamber. The total M-shell and Mζ, Mα,β, and Mγ x-ray cross sections were measured. The electron-capture (EC) contributions as well as the direct-ionization (DI) contributions can be determined by making a comprehensive study of the projectile-charge-state dependence of the target x-ray production cross sections for targets in which the single-collision realm is maintained. In this paper, both EC and DI contributions and the total M-shell x-ray production cross sections are compared to both the first Born theory and to the perturbed-stationary-state theory with energy-loss, Coulomb-deflection, and relativistic corrections.
Contributing Partner: UNT College of Arts and Sciences
Permallink:digital.library.unt.edu/ark:/67531/metadc139496/
Experimental evidence for a discrete transition to channeling for 1.0-MeV protons in Si〈100〉
Date: April 1998
Creator: Zhao, Z. Y.; Arrale, A. M.; Li, S. L.; Marble, D. K.; Weathers, Duncan L.; Matteson, Samuel E. et al
Description: This article discusses experimental evidence for a discrete transition to channeling for 1.0-MeV protons in Si〈100〉. Abstract: The present work reports the experimental evidence of anomalies exhibited by the energy loss and energy straggling of channeled protons in silicon in transmission measurements versus the incident angle. Results are presented for 1.0-MeV protons channeled along the 〈100〉 axis for a silicon foil of 3.8 μm thickness. It is shown that the transition from random to a channeling condition is discrete. The energy spectra of transmitted ions show a random peak (lower energy) and a channeled peak (higher energy). The random peak has a fixed energy, while the energy of the channeled peak increases as the target crystal's axis approaches alignment with the direction of the incident ion beam. The results support a model suggesting that the channeled ions lose energy only to valence electrons and are concentrated in a narrow cone about the direction of incidence when they emerge from the crystal. The energy straggling of channeled particles reaches a minimum in the hyper-channeled condition. Both the energy loss and the energy straggling of channeled protons show a dependence on the local electron density.
Contributing Partner: UNT College of Arts and Sciences
Permallink:digital.library.unt.edu/ark:/67531/metadc139489/
Fabrication of silicon-based optical components for an ultraclean accelerator mass spectronomy negative ion source
Date: May 1994
Creator: Kirchhoff, J. F.; Marble, D. K.; Weathers, Duncan L.; McDaniel, Floyd Del. (Floyd Delbert), 1942-; Matteson, Samuel E.; Anthony, J. M. et al
Description: This article discusses fabrication of silicon-based optical components for an ultraclean accelerator mass spectronomy negative ion source. Abstract: An ultraclean accelerator mass spectronomy negative ion source for semiconductor material mass analysis has been built and is in operation at the University of North Texas' Ion Beam Modification and Analysis Laboratory (IBMAL). The source is unique in that the active surfaces and apertures of the optical components in the ion source have been fabricated from high-purity single crystal silicon. This prevents both the 133Cs+ beam incident on the semiconductor samples and the negative ions from the sample surfaces from "seeing" and sputtering any metal surfaces (mostly stainless steel) in the beamline. The Cs+ beam can be rastered across the sample surface and the impact energy is adjustable to control depth-profiling rates. An ultraclean ion source of this type is necessary to prevent the injection of Fe and other beamline elements onto the sample or into the tandem accelerator, which is equivalent to putting an impurity signal into the mass analysis of the semiconductor sample. Suppression of these elements increases the sensitivity of the analysis to one part in 10¹² for many masses. The fabrication and alignment of the optical components-einzel lenses, ...
Contributing Partner: UNT College of Arts and Sciences
Permallink:digital.library.unt.edu/ark:/67531/metadc146573/
Low-level copper concentration measurements in silicon wafers using trace-element accelerator mass spectrometry
Date: June 8, 1998
Creator: McDaniel, Floyd Del. (Floyd Delbert), 1942-; Datar, Sameer A.; Guo, Baonian N.; Renfrow, Steve N.; Anthony, J. M. & Zhao, Z. Y.
Description: This article discusses low-level copper concentration measurements in silicon wafers using trace-element accelerator mass spectrometry. Abstract: Accelerator mass spectrometry (AMS) is now widely used in over 30 laboratories throughout the world to measure ratios of the abundances of long-lived radioisotopes such as ¹⁰Be, ¹⁴C, ³⁶Cl, and ¹²⁷I to their stable isotopes at levels as low as 10(-16). Trace-element AMS (TEAMS) is an application of AMS to the measurement of very low levels of stable isotope impurities. Copper concentrations as low as 1 part per billion have been measured in silicon wafers. In this letter, the authors demonstrate the use of TEAMS to measure previously unknown copper concentration depth profiles in As-implanted Si wafers at a few parts per billion. To verify the TEAMS technique, the samples from the same wafer were measured with secondary ion mass spectrometry, which showed the same profiles, albeit plateauing out at a concentration level six times higher than the TEAMS measurement. The ability to measure at these levels is especially significant in light of the recent moves towards the use of copper interconnects in place of aluminum in integrated circuits.
Contributing Partner: UNT College of Arts and Sciences
Permallink:digital.library.unt.edu/ark:/67531/metadc146577/
Simultaneous measurement of the average ion-induced electron emission yield and the mean charge for isotachic ions in carbon foils
Date: February 1997
Creator: Arrale, A.M.; Zhao, Z.Y.; Kirchhoff, J.F.; Weathers, Duncan L.; McDaniel, Floyd Del & Matteson, Samuel E.
Description: This article discusses simultaneous measurement of the average ion-induced electron emission yield and the mean charge for isotachic ions in carbon foils. Knowledge of the incident ion's atomic number (Z₁) dependence of ion-induced electron emission yields can be the basis for a general understanding of ion-atom interaction phenomena and, in particular, for the design of Z₁-sensitive detectors that could be useful, for example, in the separation of isobars in accelerator mass spectrometry. The Z₁ dependence of ion-induced electron emission yields, y, has been investigating using heavy ions C³⁺, O³⁺, F³⁺, Na³⁺, Al³⁺, Si³⁺, P³⁺, S³⁺, Cl³⁺, K³⁺, Ti³⁺, Cr³⁺, Mn⁴⁺, Fe⁴⁺, Co⁴⁺, Ni⁴⁺, Cu⁴⁺, Ga⁴⁺, As⁵⁺, Br⁵⁺, Ru⁷⁺, Ag⁷⁺, Sn⁷⁺, and I⁸⁺ of identical velocity (v = 2v₀, where v₀ is the Bohr velocity) normally incident on 50 μg/cm² sputter-cleaned carbon foils. Measured yields as a function of Z₁ reveal an oscillatory behavior with pronounced maxima and minima. Contrary to previously reported yields that assumed to monotonically increasing empirical mean charge state for the exiting ion, the present work indicates the Z₁ oscillations in the experimentally measured yields, a fact masked in previous work. The strong Z₁ oscillations can only be observed by simultaneous measurement of the yield and the ...
Contributing Partner: UNT College of Arts and Sciences
Permallink:digital.library.unt.edu/ark:/67531/metadc146596/
Z1 oscillations of the mean charge for isotachic ions in carbon foils
Date: April 1995
Creator: Arrale, A.M.; Jin, Jianyue; Zhao, Z.Y.; Weathers, Duncan L.; McDaniel, Floyd Del & Matteson, Samuel E.
Description: This article discusses Z1 oscillations of the mean charge for isotachic ions in carbon foils. Oscillations in the mean-charge state of swift ions as a function of the atomic number Z1 are reported for a wide range of ions of identical velocity (isotachic ions). A previously suggested mechanism for the enhancement of the mean charge for certain ion-charge combinations that involves closed shells is shown to be an inadequate explanation. Post-foil-Auger processes, however, are demonstrated to be a more plausible explanation for the observed behavior of the mean charge of the ions.
Contributing Partner: UNT College of Arts and Sciences
Permallink:digital.library.unt.edu/ark:/67531/metadc139492/