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Coherent Resonant Interaction and Harmonic Generation in Atomic Vapors

Description: This work examines the use of higher order multiphoton resonances in higher harmonic generation together with judicious exploitation of coherent interaction properties to achieve efficient harmonic generation. A detailed experimental study on third harmonic generation in two photon resonant coherent interaction and a theoretical study on four photon resonant coherent interaction have been conducted. Two photon resonant coheren propagation in lithium vapor (2S-4S and 2S-3D interaction) has been … more
Date: August 1987
Creator: Mukherjee, Nandini
Partner: UNT Libraries
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Collision Broadening in the Microwave Rotational Spectrum of Gaseous Monomeric Formaldehyde

Description: A source-modulation microwave spectrograph was utilized to measure line width parameters for several spectral lines in the pure rotational spectrum of formaldehyde (H₂CO). The spectrograph featured high-gain ac amplification and phase-sensitive detection, and was capable of measuring microwave lines having absorption coefficients as small as 10⁻⁷ cm⁻¹ with a frequency resolution on the order of 30 kHz. Center frequencies of the measured lines varied from 4,830 MHz to 72,838 MHz; hence, most of … more
Date: December 1973
Creator: Rogers, David Valmore
Partner: UNT Libraries
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Collision Broadening of Microwave Spectral Lines of Monomeric Formaldehyde and Formic Acid

Description: Line width parameters for a number of spectral lines in the pure rotational spectrum of formaldehyde (CH20) and formic acid (HCOOH) have been measured using a sourcemodulated microwave spectrograph. All transitions studied in this investigation were of the type ΔJ=O (i.e. Q-branch transitions), with ΔK-1=0 and ΔK+1 =+l. The center frequencies of the measured lines varied from 8662.0 MHz to 48612.70 MHz. The experimentally determined collision diameters for self broadening interactions involving… more
Date: August 1975
Creator: Venkatachar, Arun C.
Partner: UNT Libraries
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Complex Numbers in Quantum Theory

Description: In 1927, Nobel prize winning physicist, E. Schrodinger, in correspondence with Ehrenfest, wrote the following about the new theory: “What is unpleasant here, and indeed directly to be objected to, is the use of complex numbers. Psi is surely fundamentally a real function.” This seemingly simple issue remains unexplained almost ninety years later. In this dissertation I elucidate the physical and theoretical origins of the complex requirement. I identify a freedom/constraint situation encoun… more
Date: August 2015
Creator: Maynard, Glenn
Partner: UNT Libraries
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Complexity as a Form of Transition From Dynamics to Thermodynamics: Application to Sociological and Biological Processes.

Description: This dissertation addresses the delicate problem of establishing the statistical mechanical foundation of complex processes. These processes are characterized by a delicate balance of randomness and order, and a correct paradigm for them seems to be the concept of sporadic randomness. First of all, we have studied if it is possible to establish a foundation of these processes on the basis of a generalized version of thermodynamics, of non-extensive nature. A detailed account of this attempt is … more
Date: May 2003
Creator: Ignaccolo, Massimiliano
Partner: UNT Libraries
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Complexity as Aging Non-Poisson Renewal Processes

Description: The search for a satisfactory model for complexity, meant as an intermediate condition between total order and total disorder, is still subject of debate in the scientific community. In this dissertation the emergence of non-Poisson renewal processes in several complex systems is investigated. After reviewing the basics of renewal theory, another popular approach to complexity, called modulation, is introduced. I show how these two different approaches, given a suitable choice of the parameter … more
Date: May 2007
Creator: Bianco, Simone
Partner: UNT Libraries
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A Comprehensive Model for the Rotational Spectra of Propyne CH₃CCH in the Ground and V₁₀=1,2,3,4,5 Vibrational States

Description: The energy states of C₃ᵥ symmetric top polyatomic molecules were studied. Both classical and quantum mechanical methods have been used to introduce the energy states of polyatomic molecules. Also, it is shown that the vibration-rotation spectra of polyatomic molecules in the ground and excited vibrational states can be predicted by group theory. A comprehensive model for predicting rotational frequency components in various v₁₀ vibrational levels of propyne was developed by using perturbation t… more
Date: December 1986
Creator: Rhee, Won Myung
Partner: UNT Libraries
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Computational Studies of Selected Ruthenium Catalysis Reactions.

Description: Computational techniques were employed to investigate pathways that would improve the properties and characteristics of transition metal (i.e., ruthenium) catalysts, and to explore their mechanisms. The studied catalytic pathways are particularly relevant to catalytic hydroarylation of olefins. These processes involved the +2 to +3 oxidation of ruthenium and its effect on ruthenium-carbon bond strengths, carbon-hydrogen bond activation by 1,2-addition/reductive elimination pathways appropriate … more
Date: December 2007
Creator: Barakat, Khaldoon A.
Partner: UNT Libraries
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Computational Techniques for Accelerated Materials Discovery

Description: Increasing ubiquity of computational resources has enabled simulation of complex electronic systems and modern materials. The PAOFLOW software package is a tool designed to construct and analyze tight binding Hamiltonians from the solutions of DFT calculations. PAOFLOW leverages localized basis sets to greatly reduce computational costs of post-processing QE simulation results, enabling efficient determination of properties such as electronic density, band structures in the presence of electric… more
Date: December 2021
Creator: Cerasoli, Franklin
Partner: UNT Libraries
open access

The Concept of Collision Strength and Its Applications

Description: Collision strength, the measure of strength for a binary collision, hasn't been defined clearly. In practice, many physical arguments have been employed for the purpose and taken for granted. A scattering angle has been widely and intensively used as a measure of collision strength in plasma physics for years. The result of this is complication and unnecessary approximation in deriving some of the basic kinetic equations and in calculating some of the basic physical terms. The Boltzmann equatio… more
Date: May 2004
Creator: Chang, Yongbin
Partner: UNT Libraries
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Cooperation-induced Criticality in Neural Networks

Description: The human brain is considered to be the most complex and powerful information-processing device in the known universe. The fundamental concepts behind the physics of complex systems motivate scientists to investigate the human brain as a collective property emerging from the interaction of thousand agents. In this dissertation, I investigate the emergence of cooperation-induced properties in a system of interacting units. I demonstrate that the neural network of my research generates a series o… more
Date: August 2013
Creator: Zare, Marzieh
Partner: UNT Libraries
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Core-Shell Based Metamaterials: Fabrication Protocol and Optical Properties

Description: The objective of this study is to examine core-shell type plasmonic metamaterials aimed at the development of materials with unique electromagnetic properties. The building blocks of metamaterials under study consist of gold as a metal component, and silica and precipitated calcium carbonate (PCC) as the dielectric media. The results of this study demonstrate important applications of the core-shells including scattering suppression, airborne obscurants made of fractal gold shells, photomodific… more
Date: December 2017
Creator: De Silva, Vashista C
Partner: UNT Libraries
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Criticality in Cooperative Systems

Description: Cooperative behavior arises from the interactions of single units that globally produce a complex dynamics in which the system acts as a whole. As an archetype I refer to a flock of birds. As a result of cooperation the whole flock gets special abilities that the single individuals would not have if they were alone. This research work led to the discovery that the function of a flock, and more in general, that of cooperative systems, surprisingly rests on the occurrence of organizational collap… more
Date: May 2012
Creator: Vanni, Fabio
Partner: UNT Libraries
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Decoherence, Master Equation for Open Quantum Systems, and the Subordination Theory

Description: This thesis addresses the problem of a form of anomalous decoherence that sheds light into the spectroscopy of blinking quantum dots. The system studied is a two-state system, interacting with an external environment that has the effect of establishing an interaction between the two states, via a coherence generating coupling, called inphasing. The collisions with the environment produce also decoherence, named dephasing. Decoherence is interpreted as the entanglement of the coherent superposit… more
Date: August 2005
Creator: Giraldi, Filippo
Partner: UNT Libraries
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Deep Minima and Vortices for Positronium Formation in Positron-Hydrogen and Positron-Helium Collisions

Description: This dissertation work is a study of positronium formation for positron-hydrogen and positron-helium collisions in the Ore gap (the energy region between the threshold for ground-state positronium formation and the first excitation level of the target atom) using variational K-matrices. We have fitted the K-matrices using multichannel effective range theories and using polynomials. Using the variational K-matrices and their fits, we have located zeros in the positronium-formation scattering amp… more
Date: May 2021
Creator: Alrowaily, Albandari Wanes
Partner: UNT Libraries
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Defect Modulated Properties of Molybdenum Disulfide Monolayer Films

Description: In this dissertation work, the study focuses on large areal growth of MoS2 monolayers and a study of the structural, optical and electrical properties of such monolayers before and after transfer using a polymer-lift off technique. This work will discuss the issue of contact resistance and the effect of defects (both intrinsic and extrinsic) on the overall quality of the monolayer films. The significance of this dissertation work is that a reproducible strategy for monolayer MoS2 film growth an… more
Date: May 2022
Creator: Jiang, Yan
Partner: UNT Libraries
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Degenerate Four Wave Mixing of Short and Ultrashort Light Pulses

Description: This dissertation presents experimental and theoretical studies of transient degenerate four wave mixing (DFWM) in organic dyes. Chapter 1 is an introduction to DFWM. Chapter 2 describes DFWM experiments that were performed in the gain medium of a dye laser. Chapter 3 presents the theory of DFWM of short pulses in three level saturable media. Chapter 4 presents DFWM experiments of femtosecond pulses in the saturable absorber of a passively modelocked ring dye laser. Chapter 5 presents the theor… more
Date: August 1984
Creator: McMichael, Ian C. (Ian Charles)
Partner: UNT Libraries
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Degradation Mechanisms and Dynamics of Silicon Telluride: A Guide to the Effective Fabrication and Characterization of Silicon Telluride-Based Devices

Description: Silicon telluride (Si2Te3) and many other tellurium containing compounds show emergent Raman peaks located at ~120 cm-1 and ~140 cm-1 as they age. The origin of these two emergent peaks is controversial in the literature and has been attributed to myriad causes such as the intrinsic Raman modes of the telluride materials, surface oxidation, defects, double resonances, and tellurium precipitates. The controversial nature of these peaks has led to the misidentification of highly degraded materia… more
Date: December 2023
Creator: Hathaway, Evan Allen
Partner: UNT Libraries
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Design, Construction, and Application of an Electrostatic Quadrupole Doublet for Heavy Ion Nuclear Microprobe Research

Description: A nuclear microprobe, typically consisting of 2 - 4 quadrupole magnetic lenses and apertures serving as objective and a collimating divergence slits, focuses MeV ions to approximately 1 x 1 μm for modification and analysis of materials. Although far less utilized, electrostatic quadrupole fields similarly afford strong focusing of ions and have the added benefit of doing so independent of ion mass. Instead, electrostatic quadrupole focusing exhibits energy dependence on focusing ions. A heav… more
Date: December 2017
Creator: Manuel, Jack Elliot
Partner: UNT Libraries
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Detection of the Resonant Vibration of the Cellular Membrane Using Femtosecond Laser Pulses

Description: An optical detection technique is developed to detect and measure the resonant vibration of the cellular membrane. Biological membranes are active components of living cells and play a complex and dynamic role in life processes. They are believed to have oscillation modes of frequencies in the range of 1 to 1000 GHz. To measure such a high-frequency vibration, a linear laser cavity is designed to produce a train of femtosecond pulses of adjustable repetition rate. The method is then directly ap… more
Date: December 1989
Creator: Jamasbi, Nooshin
Partner: UNT Libraries
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A Determination of the Fine Structure Constant Using Precision Measurements of Helium Fine Structure

Description: Spectroscopic measurements of the helium atom are performed to high precision using an atomic beam apparatus and electro-optic laser techniques. These measurements, in addition to serving as a test of helium theory, also provide a new determination of the fine structure constant α. An apparatus was designed and built to overcome limitations encountered in a previous experiment. Not only did this allow an improved level of precision but also enabled new consistency checks, including an extr… more
Date: August 2010
Creator: Smiciklas, Marc
Partner: UNT Libraries
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Deterministic Brownian Motion

Description: The goal of this thesis is to contribute to the ambitious program of the foundation of developing statistical physics using chaos. We build a deterministic model of Brownian motion and provide a microscpoic derivation of the Fokker-Planck equation. Since the Brownian motion of a particle is the result of the competing processes of diffusion and dissipation, we create a model where both diffusion and dissipation originate from the same deterministic mechanism - the deterministic interaction of t… more
Date: August 1993
Creator: Trefán, György
Partner: UNT Libraries

Developing Ultra-Fast Plasmonic Spiking Neuron via Integrated Photonics

Description: This research provides a proof of concept and background theory for the physics behind the state-of-the-art ultra-fast plasmonic spiking neurons (PSN), which can serve as a primary synaptic device for developing a platform for fast neural computing. Such a plasmonic-powered computing system allows localized AI with ultra-fast operation speed. The designed architecture for a plasmonic spiking neuron (PSN) presented in this thesis is a photonic integrated nanodevice consisting of two electro-opti… more
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Date: August 2022
Creator: Goudarzi, Abbas, Sr.
Partner: UNT Libraries
open access

Dielectric Relaxation of Aqueous Solutions at Microwave Frequencies for 335 GHz. Using a Loaded Microwave Cavity Operating in the TM010 Mode

Description: The frequency dependence and temperature dependence of the complex dielectric constant of water is of great interest. The temperature dependence of the physical properties of water given in the literature, specific heat, thermal conductivity, electric conductivity, pH, etc. are compared to the a. c. (microwave) and d. c. conductivity of water with a variety of concentration of different substances such as HC1, NaCl, HaS04, etc. When each of these properties is plotted versus inverse absolute te… more
Date: August 1994
Creator: Wang, Henry F. S. (Henry Fu-Sen)
Partner: UNT Libraries
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