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  Partner: UNT Libraries
 Department: Department of Physics
 Collection: UNT Theses and Dissertations
Charge State Distributions in Molecular Dissociation

Charge State Distributions in Molecular Dissociation

Date: December 1998
Creator: Renfrow, Steven N. (Steven Neal)
Description: The present work provides charge state fractions that may be used to generate TEAMS relative sensitivity factors for impurities in semiconductor materials.
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Magnetomorphic Oscillations in Zinc

Magnetomorphic Oscillations in Zinc

Date: August 1970
Creator: Waller, William Marvin
Description: In making this study it is important to search for ways to enhance and, if possible, make detection of MMO signals simpler in order that this technique for obtaining FS measurements may be extended to other materials. This attempt to improve measurement techniques has resulted in a significant discovery: the eddy-current techniques described in detail in a later section which should allow MMO to be observed and sensitively measured in many additional solids. The second major thrust of the study has been to use the newly discovered eddy-current technique in obtaining the first indisputable observation of MMO in zinc.
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Quantum-Confined CdS Nanoparticles on DNA Templates

Quantum-Confined CdS Nanoparticles on DNA Templates

Date: May 1998
Creator: Rho, Young Gyu
Description: As electronic devices became smaller, interest in quantum-confined semiconductor nanostructures increased. Self-assembled mesoscale semiconductor structures of II-VI nanocrystals are an especially exciting subject because of their controllable band gap and unique photophysical properties. Several preparative methods to synthesize and control the sizes of the individual nanocrystallites and the electronic and optical properties have been intensively studied. Fabrication of patterned nanostructures composed of quantum-confined nanoparticles is the next step toward practical applications. We have developed an innovative method to fabricate diverse nanostructures which relies on the size and a shape of a chosen deoxyribonucleic acid (DNA) template.
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Anisotropic Relaxation Time for Solids with Ellipsoidal Fermi Surfaces

Anisotropic Relaxation Time for Solids with Ellipsoidal Fermi Surfaces

Date: May 1971
Creator: Fuchser, Troy Denrich
Description: Many solids have Fermi surfaces which are approximated as ellipsoids. A comprehensive solution for the magnetoconductivity of an ellipsoid is obtained which proves the existence of a relaxation time tensor which can be anisotropic and which is a function of energy only.
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Fluorine Adsorption and Diffusion in Polycrystalline Silica

Fluorine Adsorption and Diffusion in Polycrystalline Silica

Date: December 1998
Creator: Jin, Jian-Yue
Description: The measurement of fluorine penetration into archeological flint artifacts using Nuclear Reaction Analysis (NRA) has been reported to be a potential dating method. However, the mechanism of how fluorine is incorporated into the flint surface, and finally transported into the bulk is not well understood. This research focuses on the study of the fluorine uptake phenomenon of flint mineral in aqueous fluoride solutions. Both theoretical and experimental approaches have been carried out. In a theoretical approach, a pipe-diffusion model was used to simulate the complicated fluorine transportation problem in flint, in which several diffusion mechanisms may be involved.
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Two-Fold Role of Randomness: A Source of Both Long-Range Correlations and Ordinary Statistical Mechanics

Two-Fold Role of Randomness: A Source of Both Long-Range Correlations and Ordinary Statistical Mechanics

Date: December 1998
Creator: Rocco, A. (Andrea)
Description: The role of randomness as a generator of long range correlations and ordinary statistical mechanics is investigated in this Dissertation. The difficulties about the derivation of thermodynamics from mechanics are pointed out and the connection between the ordinary fluctuation-dissipation process and possible anomalous properties of statistical systems is highlighted.
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Synthesis and Study of Engineered Heterogenous Polymer Gels

Synthesis and Study of Engineered Heterogenous Polymer Gels

Date: August 1998
Creator: Chen, Yuanye
Description: This dissertation studies physical properties and technological applications of engineered heterogenous polymer gels. Such gels are synthesized based on modulation of gel chemical nature in space. The shape memory gels have been developed in this study by using the modulated gel technology. At room temperature, they form a straight line. As the temperature is increased, they spontaneously bend or curl into a predetermined shape such as a letter of the alphabet, a numerical number, a spiral, a square, or a fish. The shape changes are reversible. The heterogenous structures have been also obtained on the gel surface. The central idea is to cover a dehydrated gel surface with a patterned mask, then to sputter-deposit a gold film onto it. After removing the mask, a gold pattern is left on the gel surface. Periodical surface array can serve as gratings to diffract light. The grating constant can be continuously changed by the external environmental stimuli such as temperature and electric field. Several applications of gels with periodic surface arrays as sensors for measuring gel swelling ratio, internal strain under an uniaxial stress, and shear modulus have been demonstrated. The porous NIPA gels have been synthesized by suspension technique. Microstructures of newly ...
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Structural and Photoelectron Emission Properties of Chemical Vapor Deposition Grown Diamond Films

Structural and Photoelectron Emission Properties of Chemical Vapor Deposition Grown Diamond Films

Date: August 1998
Creator: Akwani, Ikerionwu Asiegbu
Description: The effects of methane (CH4), diborone (B2H6) and nitrogen (N2) concentrations on the structure and photoelectron emission properties of chemical vapor deposition (CVD) polycrystalline diamond films were studied. The diamond films were grown on single-crystal Si substrates using the hot-tungsten filament CVD technique. Raman spectroscopy and x-ray photoelectron spectroscopy (XPS) were used to characterize the different forms of carbon in the films, and the fraction of sp3 carbon to sp3 plus sp2 carbon at the surface of the films, respectively. Scanning electron microscopy (SEM) was used to characterize the surface morphology of the films. The photoelectron emission properties were determined by measuring the energy distributions of photoemitted electrons using ultraviolet photoelectron spectroscopy (UPS), and by measuring the photoelectric current as a function of incident photon energy.
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On Delocalization Effects in Multidimensional Lattices

On Delocalization Effects in Multidimensional Lattices

Date: May 1998
Creator: Bystrik, Anna
Description: A cubic lattice with random parameters is reduced to a linear chain by the means of the projection technique. The continued fraction expansion (c.f.e.) approach is herein applied to the density of states. Coefficients of the c.f.e. are obtained numerically by the recursion procedure. Properties of the non-stationary second moments (correlations and dispersions) of their distribution are studied in a connection with the other evidences of transport in a one-dimensional Mori chain. The second moments and the spectral density are computed for the various degrees of disorder in the prototype lattice. The possible directions of the further development are outlined. The physical problem that is addressed in the dissertation is the possibility of the existence of a non-Anderson disorder of a specific type. More precisely, this type of a disorder in the one-dimensional case would result in a positive localization threshold. A specific type of such non-Anderson disorder was obtained by adopting a transformation procedure which assigns to the matrix expressing the physics of the multidimensional crystal a tridiagonal Hamiltonian. This Hamiltonian is then assigned to an equivalent one-dimensional tight-binding model. One of the benefits of this approach is that we are guaranteed to obtain a linear crystal with a ...
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Scanning Tunneling Microscopy of Epitaxial Diamond (110) and (111) Films and Field Emission Properties of Diamond Coated Molybdenum Microtips

Scanning Tunneling Microscopy of Epitaxial Diamond (110) and (111) Films and Field Emission Properties of Diamond Coated Molybdenum Microtips

Date: May 1998
Creator: Lim, Seong-Chu
Description: The growth mechanism of chemical vapor deposition (CVD) grown homo-epitaxial diamond (110) and (111) films was studied using ultrahigh vacuum (UHV) scanning tunneling microscopy (STM). In addition, the field emission properties of diamond coated molybdenum microtips were studied as a function of exposure to different gases.
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Microscopic Foundations of Thermodynamics and Generalized Statistical Ensembles

Microscopic Foundations of Thermodynamics and Generalized Statistical Ensembles

Date: May 2008
Creator: Campisi, Michele
Description: This dissertation aims at addressing two important theoretical questions which are still debated in the statistical mechanical community. The first question has to do with the outstanding problem of how to reconcile time-reversal asymmetric macroscopic laws with the time-reversal symmetric laws of microscopic dynamics. This problem is addressed by developing a novel mechanical approach inspired by the work of Helmholtz on monocyclic systems and the Heat Theorem, i.e., the Helmholtz Theorem. By following a line of investigation initiated by Boltzmann, a Generalized Helmholtz Theorem is stated and proved. This theorem provides us with a good microscopic analogue of thermodynamic entropy. This is the volume entropy, namely the logarithm of the volume of phase space enclosed by the constant energy hyper-surface. By using quantum mechanics only, it is shown that such entropy can only increase. This can be seen as a novel rigorous proof of the Second Law of Thermodynamics that sheds new light onto the arrow of time problem. The volume entropy behaves in a thermodynamic-like way independent of the number of degrees of freedom of the system, indicating that a whole thermodynamic-like world exists at the microscopic level. It is also shown that breaking of ergodicity leads to microcanonical ...
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Multifunctional Organic-Inorganic Hybrid Nanophotonic Devices

Multifunctional Organic-Inorganic Hybrid Nanophotonic Devices

Date: May 2008
Creator: Garner, Brett William
Description: The emergence of optical applications, such as lasers, fiber optics, and semiconductor based sources and detectors, has created a drive for smaller and more specialized devices. Nanophotonics is an emerging field of study that encompasses the disciplines of physics, engineering, chemistry, biology, applied sciences and biomedical technology. In particular, nanophotonics explores optical processes on a nanoscale. This dissertation presents nanophotonic applications that incorporate various forms of the organic polymer N-isopropylacrylamide (NIPA) with inorganic semiconductors. This includes the material characterization of NIPA, with such techniques as ellipsometry and dynamic light scattering. Two devices were constructed incorporating the NIPA hydrogel with semiconductors. The first device comprises a PNIPAM-CdTe hybrid material. The PNIPAM is a means for the control of distances between CdTe quantum dots encapsulated within the hydrogel. Controlling the distance between the quantum dots allows for the control of resonant energy transfer between neighboring quantum dots. Whereby, providing a means for controlling the temperature dependent red-shifts in photoluminescent peaks and FWHM. Further, enhancement of photoluminescent due to increased scattering in the medium is shown as a function of temperature. The second device incorporates NIPA into a 2D photonic crystal patterned on GaAs. The refractive index change of the NIPA hydrogel as ...
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Emergence of Complexity from Synchronization and Cooperation

Emergence of Complexity from Synchronization and Cooperation

Date: May 2008
Creator: Geneston, Elvis L.
Description: The dynamical origin of complexity is an object of intense debate and, up to moment of writing this manuscript, no unified approach exists as to how it should be properly addressed. This research work adopts the perspective of complexity as characterized by the emergence of non-Poisson renewal processes. In particular I introduce two new complex system models, namely the two-state stochastic clocks and the integrate-and-fire stochastic neurons, and investigate its coupled dynamics in different network topologies. Based on the foundations of renewal theory, I show how complexity, as manifested by the occurrence of non-exponential distribution of events, emerges from the interaction of the units of the system. Conclusion is made on the work's applicability to explaining the dynamics of blinking nanocrystals, neuron interaction in the human brain, and synchronization processes in complex networks.
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Perturbation of renewal processes

Perturbation of renewal processes

Date: May 2008
Creator: Akin, Osman Caglar
Description: Renewal theory began development in the early 1940s, as the need for it in the industrial engineering sub-discipline operations research had risen. In time, the theory found applications in many stochastic processes. In this thesis I investigated the effect of seasonal effects on Poisson and non-Poisson renewal processes in the form of perturbations. It was determined that the statistical analysis methods developed at UNT Center for Nonlinear Science can be used to detect the effects of seasonality on the data obtained from Poisson/non-Poisson renewal systems. It is proved that a perturbed Poisson process can serve as a paradigmatic model for a case where seasonality is correlated to the noise and that diffusion entropy method can be utilized in revealing this relation. A renewal model making a connection with the stochastic resonance phenomena is used to analyze a previous neurological experiment, and it was shown that under the effect of a nonlinear perturbation, a non-Poisson system statistics may make a transition and end up in the of Poisson basin of statistics. I determine that nonlinear perturbation of the power index for a complex system will lead to a change in the complexity characteristics of the system, i.e., the system will reach ...
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The Use of Mossbauer Effect for the Study of Recoilless Rayleigh Scattering of Low-Energy Gamma Rays from Sodium Chloride

The Use of Mossbauer Effect for the Study of Recoilless Rayleigh Scattering of Low-Energy Gamma Rays from Sodium Chloride

Date: August 1963
Creator: Fowler, Eugene Franklin
Description: Evidence that recoilless emission and absorption exist may be shown by an experiment in which the source gamma rays are allowed to pass through a suitable absorber to a detector.
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Extinguishment of a Low-pressure Argon Discharge by a Magnetic Field

Extinguishment of a Low-pressure Argon Discharge by a Magnetic Field

Date: January 1964
Creator: Criswell, David Russell
Description: The experiment in this study involves the extinguishment of a low-pressure argon discharge by a magnetic field.
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Thermomagnetic Phenomena in Antimony at Liquid Helium Temperatures

Thermomagnetic Phenomena in Antimony at Liquid Helium Temperatures

Date: January 1964
Creator: Haywood, Charles Thomas
Description: The purpose of this investigation was to study head-transport phenomena in a single crystal of antimony at liquid helium temperatures. In particular, the longitudinal and transverse components of the thermal resistivity tensor were measured as a function of magnetic field up to eighteen kilogauss.
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Magnetically Driven Instabilities in Gas Discharges

Magnetically Driven Instabilities in Gas Discharges

Date: August 1963
Creator: Choate, Jimmie W.
Description: In the present experiment a gas discharge plasma generator was designed and constructed and a search was made for evidence of a plasma instability due to the influence of an externally applied magnetic field. The evidence for such an unstable mode of operation is too indirect to make a possible conclusion, but an approach to more certain identification will be indicated.
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Thermal Properties of a Single Crystal of Bismuth at Liquid-helium Temperatures

Thermal Properties of a Single Crystal of Bismuth at Liquid-helium Temperatures

Date: January 1964
Creator: Alsup, Dale Lynn
Description: The purpose of this investigation was the determination of the thermal conduction properties of a single crystal of bismuth at liquid-helium temperatures in magnetic fields up to eighteen kilogauss.
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A Vacuum Tube for an Electrostatic Accelerator

A Vacuum Tube for an Electrostatic Accelerator

Date: June 1963
Creator: Wiley, Ralph
Description: The purpose of this study has been to design a prototype accelerating tube, to determine the correct point shape and spacing needed to produce corona current along the tube for the case of negative-point-to-positive-plane discharge, and to study the voltage-gradient characteristics of short sections of the tube when they were evacuated to a low internal pressure.
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High Efficiency High Power Blue Laser by Resonant Doubling in PPKTP

High Efficiency High Power Blue Laser by Resonant Doubling in PPKTP

Date: August 2011
Creator: Danekar, Koustubh
Description: I developed a high power blue laser for use in scientific and technical applications (eg. precision spectroscopy, semiconductor inspection, flow cytometry, etc). It is linearly polarized, single longitudinal and single transverse mode, and a convenient fiber coupled continuous wave (cw) laser source. My technique employs external cavity frequency doubling and provides better power and beam quality than commercially available blue diode lasers. I use a fiber Bragg grating (FBG) stabilized infrared (IR) semiconductor laser source with a polarization maintaining (PM) fiber coupled output. Using a custom made optical and mechanical design this output is coupled with a mode matching efficiency of 96% into the doubling cavity. With this carefully designed and optimized cavity, measurements were carried out at various fundamental input powers. A net efficie ncy of 81 % with an output power of 680 mW at 486 nm was obtained using 840 mW of IR input. Also I report an 87.5 % net efficiency in coupling of blue light from servo locked cavity into a single mode PM fiber. Thus I have demonstrated a total fiber to fiber efficiency of 71% can be achieved in our approach using periodically poled potassium titanyl phosphate (PPKTP). To obtain these results, all ...
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Complexity as Aging Non-Poisson Renewal Processes

Complexity as Aging Non-Poisson Renewal Processes

Date: May 2007
Creator: Bianco, Simone
Description: The search for a satisfactory model for complexity, meant as an intermediate condition between total order and total disorder, is still subject of debate in the scientific community. In this dissertation the emergence of non-Poisson renewal processes in several complex systems is investigated. After reviewing the basics of renewal theory, another popular approach to complexity, called modulation, is introduced. I show how these two different approaches, given a suitable choice of the parameter involved, can generate the same macroscopic outcome, namely an inverse power law distribution density of events occurrence. To solve this ambiguity, a numerical instrument, based on the theoretical analysis of the aging properties of renewal systems, is introduced. The application of this method, called renewal aging experiment, allows us to distinguish if a time series has been generated by a renewal or a modulation process. This method of analysis is then applied to several physical systems, from blinking quantum dots, to the human brain activity, to seismic fluctuations. Theoretical conclusions about the underlying nature of the considered complex systems are drawn.
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Nanoscale Materials Applications: Thermoelectrical, Biological, and Optical Applications with Nanomanipulation Technology

Nanoscale Materials Applications: Thermoelectrical, Biological, and Optical Applications with Nanomanipulation Technology

Date: August 2011
Creator: Lee, Kyung-Min
Description: In a sub-wavelength scale, even approaching to the atomic scale, nanoscale physics shows various novel phenomena. Since it has been named, nanoscience and nanotechnology has been employed to explore and exploit this small scale world. For example, with various functionalized features, nanowire (NW) has been making its leading position in the researches of physics, chemistry, biology, and engineering as a miniaturized building block. Its individual characteristic shows superior and unique features compared with its bulk counterpart. As one part of these research efforts and progresses, and with a part of the fulfillment of degree study, novel methodologies and device structures in nanoscale were devised and developed to show the abilities of high performing thermoelectrical, biological, and optical applications. A single β-SiC NW was characterized for its thermoelectric properties (thermal conductivity, Seebeck coefficient, and figure of merit) to compare with its bulk counterpart. The combined structure of Ag NW and ND was made to exhibit its ability of clear imaging of a fluorescent cell. And a plasmonic nanosture of silver (Ag) nanodot array and a β-SiC NW was fabricated to show a high efficient light harvesting device that allows us to make a better efficient solar cell. Novel nanomanipulation techniques were ...
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Non-Poissonian statistics, aging and "blinking'" quantum dots.

Non-Poissonian statistics, aging and "blinking'" quantum dots.

Date: August 2004
Creator: Aquino, Gerardo
Description: This dissertation addresses the delicate problem of aging in complex systems characterized by non-Poissonian statistics. With reference to a generic two-states system interacting with a bath it is shown that to properly describe the evolution of such a system within the formalism of the continuous time random walk (CTRW), it has to be taken into account that, if the system is prepared at time t=0 and the observation of the system starts at a later time ta>0, the distribution of the first sojourn times in each of the two states depends on ta, the age of the system. It is shown that this aging property in the fractional derivative formalism forces to introduce a fractional index depending on time. It is shown also that, when a stationary condition exists, the Onsager regression principle is fulfilled only if the system is aged and consequently if an infinitely aged distribution for the first sojourn times is adopted in the CTRW formalism used to describe the system itself. This dissertation, as final result, shows how to extend to the non-Poisson case the Kubo Anderson (KA) lineshape theory, so as to turn it into a theoretical tool adequate to describe the time evolution of ...
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