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Developing Ultra-Fast Plasmonic Spiking Neuron via Integrated Photonics

Description: This research provides a proof of concept and background theory for the physics behind the state-of-the-art ultra-fast plasmonic spiking neurons (PSN), which can serve as a primary synaptic device for developing a platform for fast neural computing. Such a plasmonic-powered computing system allows localized AI with ultra-fast operation speed. The designed architecture for a plasmonic spiking neuron (PSN) presented in this thesis is a photonic integrated nanodevice consisting of two electro-opti… more
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Date: August 2022
Creator: Goudarzi, Abbas, Sr.
Partner: UNT Libraries
open access

Nonreciprocal and Non-Spreading Transmission of Acoustic Beams through Periodic Dissipative Structures

Description: Propagation of a Gaussian beam in a layered periodic structure is studied analytically, numerically, and experimentally. It is demonstrated that for a special set of parameters the acoustic beam propagates without diffraction spreading. This propagation is also accompanied by negative refraction of the direction of phase velocity of the Bloch wave. In the study of two-dimensional viscous phononic crystals with asymmetrical solid inclusions, it was discovered that acoustic transmission is nonre… more
Date: May 2022
Creator: Zubov, Yurii
Partner: UNT Libraries
open access

Ionized Molecular Hydrogen Confinement Using Electron Space-Charge: A Plasma Trap

Description: An ion trap has been constructed that creates a potential well suitable for confining ions with the space charge of an electron cloud. The trap uses the concept of artificially structured boundaries, regions of overlapping electric and magnetic fields, to confine particles in a relatively field free volume. Measurements are presented from the build-up of ionized molecular hydrogen over time. Molecular hydrogen is introduced into the confinement volume by direct electron bombardment ionization o… more
Date: May 2022
Creator: Kiester, Allen Scott
Partner: UNT Libraries

Ongoing Developments on Continuum Solvation Models

Description: This work explores a continuum representation for diffuse layer models, thereby endowing continuum embedding models the ability to capture electrostatic phenomena in the environment such as the existence of electrolyte ions, and the nature of ionic liquids. It introduces a new field-aware continuum model that adjusts the size of the quantum regime per atom based on the distribution of charge in a system. The model accounts for the asymmetric nature of solvent distribution when applied to cation… more
Date: May 2022
Creator: Truscott, Matthew Anthony Si Ren
Partner: UNT Libraries
open access

Band Theory and Beyond: Applications of Quantum Algorithms for Quantum Chemistry

Description: In the past two decades, myriad algorithms to elucidate the characteristics and dynamics of molecular systems have been developed for quantum computers. In this dissertation, we explore how these algorithms can be adapted to other fields, both to closely related subjects such as materials science, and more surprising subjects such as information theory. Special emphasis is placed on the Variational Quantum Eigensolver algorithm adapted to solve band structures of a periodic system; three distin… more
Date: May 2022
Creator: Sherbert, Kyle Matthew
Partner: UNT Libraries
open access

Defect Modulated Properties of Molybdenum Disulfide Monolayer Films

Description: In this dissertation work, the study focuses on large areal growth of MoS2 monolayers and a study of the structural, optical and electrical properties of such monolayers before and after transfer using a polymer-lift off technique. This work will discuss the issue of contact resistance and the effect of defects (both intrinsic and extrinsic) on the overall quality of the monolayer films. The significance of this dissertation work is that a reproducible strategy for monolayer MoS2 film growth an… more
Date: May 2022
Creator: Jiang, Yan
Partner: UNT Libraries
open access

Relaxation Time Approximations in PAOFLOW 2.0

Description: Electronic transport properties have been used to classify and characterize materials and describe their functionality. Recent surge in computational power has enabled computational modelling and accelerated theoretical studies to complement and accelerate experimental discovery of novel materials. This work looks at methods for theoretical calculations of electronic transport properties and addresses the limitations of a common approximation in the calculation of these properties, namely, the … more
Date: May 2022
Creator: Jayaraj, Anooja
Partner: UNT Libraries
open access

Towards Increased Precision of the 4He:23P1→23P2 Transition Measurement Using Laser Spectroscopy

Description: Significant sub-systems were created and others enhanced providing a platform for an order of magnitude precision increase of the small 4He interval - 23P1→23P2 laser spectroscopy measurement, as well as other helium transitions. These measurements serve as tests of helium theory and quantum electro-dynamics in general. Many improvements to the original experiment are discussed and characterized. In particular, counting speed increased 10x, the signal level was doubled, a novel Doppler shift mi… more
Date: December 2021
Creator: Cameron, Garnet
Partner: UNT Libraries
open access

Computational Techniques for Accelerated Materials Discovery

Description: Increasing ubiquity of computational resources has enabled simulation of complex electronic systems and modern materials. The PAOFLOW software package is a tool designed to construct and analyze tight binding Hamiltonians from the solutions of DFT calculations. PAOFLOW leverages localized basis sets to greatly reduce computational costs of post-processing QE simulation results, enabling efficient determination of properties such as electronic density, band structures in the presence of electric… more
Date: December 2021
Creator: Cerasoli, Franklin
Partner: UNT Libraries
open access

Information and Self-Organization in Complex Networks

Description: Networks that self-organize in response to information are one of the most central studies in complex systems theory. A new time series analysis tool for studying self-organizing systems is developed and demonstrated. This method is applied to interacting complex swarms to explore the connection between information transport and group size, providing evidence for Dunbar's numbers having a foundation in network dynamics. A complex network model of information spread is developed. This network in… more
Date: December 2021
Creator: Culbreth, Garland
Partner: UNT Libraries

Low-Energy Electron Irradiation of 2D Graphene and Stability Investigations of 2D MoS2

Description: In this work, we demonstrate the mechanism for etching exfoliated graphene on SiO2 and other technological important substrates (Si, SiC and ITO), using low-energy electron sources. Our mechanism is based on helium ion sputtering and vacancy formation. Helium ions instead of incident electrons cause the defects that oxygen reacts with and etches graphene. We found that etching does not occur on low-resistivity Si and ITO. Etching occurs on higher resistivity Si and SiC, although much less than … more
Date: August 2021
Creator: Femi Oyetoro, John Dideoluwa
Partner: UNT Libraries
open access

A Study of Anomalous Conduction in n-Type Amorphous Silicon and Correlations in Conductivity and Noise in Gold Nanoparticle-Ligand Arrays

Description: This work explores two very different structural systems: n-type hydrogenated amorphous silicon (a-Si:H) and gold nanoparticles (AuNPs) suspended in a matrix of organic ligands. For a-Si:H, examination of the gas-phase concentration of dopant (1-6% PH3/SiH4) and argon diluent effects includes the temperature dependent conductivity, low-frequency electronic noise, and Raman spectroscopy to examine structure. It is found that a-Si:H samples grown with high dopant concentration or with argon dilut… more
Date: August 2021
Creator: Western, Brianna J
Partner: UNT Libraries
open access

Classical Simulations of the Drift of Magnetobound States of Positronium

Description: The production and control of antihydrogen at very low temperatures provided a key tool to test the validity for the antimaterial of the fundamental principles of the interactions of nature such as the weak principle of equivalence (WEP), and CPT symmetry (Charge, Parity, and Time reversal). The work presented in this dissertation studies the collisions of electrons and positrons in strong magnetic fields that generate magnetobound positronium (positron-electron system temporarily bound due to … more
Date: August 2021
Creator: Aguirre Farro, Franz
Partner: UNT Libraries
open access

The Electrochemical Etching Process of a Tungsten Wire

Description: This study produced and analyzed shaped tungsten wire tips formed through electrochemical etching. Specifically, the cone length and the radius of curvature of the tip were analyzed. Having the tips move dynamically through an electrolytic solution, such as potassium hydroxide, and tuning the initial starting depth of the tungsten wire along with the dynamic speed of the tungsten wire as it passed throughout the solution allowed various types of tip profiles to be produced. The tip's radius of … more
Date: August 2021
Creator: Richardson, Aaron Michael
Partner: UNT Libraries
open access

Deep Minima and Vortices for Positronium Formation in Positron-Hydrogen and Positron-Helium Collisions

Description: This dissertation work is a study of positronium formation for positron-hydrogen and positron-helium collisions in the Ore gap (the energy region between the threshold for ground-state positronium formation and the first excitation level of the target atom) using variational K-matrices. We have fitted the K-matrices using multichannel effective range theories and using polynomials. Using the variational K-matrices and their fits, we have located zeros in the positronium-formation scattering amp… more
Date: May 2021
Creator: Alrowaily, Albandari Wanes
Partner: UNT Libraries

Modeling, Characterization, and Magnetic Behavior of Transition Metal Nanosystems Synthesized in Silicon Using Low Energy Ion Implantation

Description: Magnetic nano-clusters in silicon involving iron and cobalt were synthesized using low energy (50 keV) ion implantation technique and post-implantation thermal annealing. Before the irradiation, multiple ion-solid interaction simulations were carried out to estimate optimal ion energy and fluence for each experiment. For high-fluence low-energy irradiation of heavy ions in a relatively lighter substrate, modeling the ion irradiation process using dynamic code SDTrimSP showed better agreement w… more
Date: May 2021
Creator: Singh, Satyabrata
Partner: UNT Libraries

Investigation of Room Temperature Soft Ferromagnetism in Indium Phosphide Substrate Synthesized via Low Energy Nickel Ion Implantation

Description: In this work, we have utilized an ion beam process known as gettering to migrate implanted Ni ions much deeper into the bulk substrate than their initial projected end of the range. The projected mean depth is known as Rp. The gettering effect is the most crucial part of the fabrication and we have found that for an H fluence of 3x 1016 cm-2 there is a threshold fluence of approximately 7.5 x 1015 cm-2 that cannot be surpassed if the gettering process is to be completed along with the substrat… more
Date: May 2021
Creator: Jones, Daniel C.
Partner: UNT Libraries

Synthesis, Modification, and Analysis of Silicate Cosmic Dust Analogues Using Ion-Beam Techniques

Description: Silicates analogous to cosmic dust were synthesized, modified, and analyzed utilizing ion-beam techniques with Rutherford backscattering spectrometry (RBS) and x-ray diffraction (XRD). Silicate dust is a common constituent in interstellar space, with an estimated 50% of dust produced in the stellar winds of M class Asymptotic Giant Branch (AGB) stars. Silicate dust acts as a surface upon which other chemicals may form (water ice for example), increasing significance in the cosmochemistry field,… more
Date: August 2020
Creator: Young, Joshua Michael
Partner: UNT Libraries

Fabrication of Nano-Channel Templates and a Study of the Electrical and Magnetic Properties of Nanowires Grown in Template Pores

Description: This thesis is a study of the structural, electrical and magnetic properties of indium antimonide (InSb) nanowires (NWs), that were synthesized by a template-assisted ordered growth technique via electrochemical deposition. InSb was chosen for this study because of its intrinsic properties that make it a material of choice for applications in high channel mobility, infrared (IR) sensing, thermoelectrics, and magnetoresistive sensing martials. This work has four main components: (i) Growth in co… more
Date: May 2020
Creator: Singh, Abhay Pratap
Partner: UNT Libraries

Optical Property Study of 2D Graded Photonic Super-Crystals for Photon Management

Description: In this dissertation, we study the optical property of 2D graded photonic super-crystals (GPSCs) for photon management. We focused primarily on manipulation and control of light by using the newly discovered GPSCs which present great opportunity for electromagnetic wave control in photonic devices. The GPSC has been used to explore the superior capability of improving the light extraction efficiency of OLEDs. The enhancement of extraction efficiency has been explained in term of destructive int… more
Date: May 2020
Creator: Hassan, Safaa
Partner: UNT Libraries
open access

Investigation of Specialized Laser and Optical Techniques to Improve Precision Atomic Spectroscopy of Helium

Description: The aim of this thesis is to develop both Yb and Tm fiber laser sources with all fiber cavities. Both wavelength ranges provide useful laser sources for optical pumping of helium. The goal is to develop Tm laser sources operating at 2058 nm to optically quench 3He (2058.63 nm) and 4He (2058.69 nm) singlets (21S0). We also have developed Yb laser sources at 1083 nm to optical pump the triplet states of helium and laser cool an atomic beam of helium.
Date: May 2020
Creator: Currey, Ronnie
Partner: UNT Libraries

Manipulation of Light-Matter Interactions in Molybdenum Disulfide (MoS2) Monolayer through Dressed Phonons (DP) and Plasmons

Description: The performance of electrical and optical devices based on two-dimensional semiconductors (2D) such as molybdenum disulfide is critically influenced due to very poor light absorption in the atomically thin layers. In this study, the phonon mediated optical absorption and emission properties in single atomic layers of MoS2 have been investigated. The electronic transitions in MoS2 due to near-field optical interaction and the influence of interface phonons due to the dielectric substrate GaN on … more
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Date: December 2019
Creator: Poudel, Yuba R
Partner: UNT Libraries

PAOFLOW-Aided Computational Materials Design

Description: Functional materials are essential to human welfare and to provide foundations for emerging industries. As an alternative route to experimental materials discovery, computational materials designs are playing an increasingly significant role in the whole discovery process. In this work, we use an in-house developed python utility: PAOFLOW, which generates finite basis Hamiltonians from the projection of first principles plane-wave pseudopotential wavefunctions on pseudo atomic orbitals(PAO) for… more
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Date: December 2019
Creator: Wang, Haihang
Partner: UNT Libraries
open access

Renewal and Memory Approaches to Study Biological and Physiological Processes

Description: In nature we find many instances of complex behavior for example the dynamics of stock markets, power grids, internet networks, highway traffic, social networks, heartbeat dynamics, neural dynamics, dynamics of living organisms, etc. The study of these complex systems involves the use of tools of non-linear dynamics and non-equilibrium statistical physics. This dissertation is devoted to understanding two different sources of complex behavior – non-poissonian renewal events also called crucial… more
Date: May 2019
Creator: Tuladhar, Rohisha
Partner: UNT Libraries
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