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Oligonucleotide guanosine conjugated to gallium nitride nano-structures for photonics.

Description: In this work, I studied the hybrid system based on self-assembled guanosine crystal (SAGC) conjugated to wide-bandgap semiconductor gallium nitride (GaN). Guanosine is one of the four bases of DNA and has the lowest oxidation energy, which favors carrier transport. It also has large dipole moment. Guanosine molecules self-assemble to ribbon-like structure in confined space. GaN surface can have positive or negative polarity depending on whether the surface is Ga- or N-terminated. I studied… more
Date: August 2008
Creator: Li, Jianyou
Partner: UNT Libraries
open access

On Chaos and Anomalous Diffusion in Classical and Quantum Mechanical Systems

Description: The phenomenon of dynamically induced anomalous diffusion is both the classical and quantum kicked rotor is investigated in this dissertation. We discuss the capability of the quantum mechanical version of the system to reproduce for extended periods the corresponding classical chaotic behavior.
Date: August 1998
Creator: Stefancich, Marco
Partner: UNT Libraries
open access

On Delocalization Effects in Multidimensional Lattices

Description: A cubic lattice with random parameters is reduced to a linear chain by the means of the projection technique. The continued fraction expansion (c.f.e.) approach is herein applied to the density of states. Coefficients of the c.f.e. are obtained numerically by the recursion procedure. Properties of the non-stationary second moments (correlations and dispersions) of their distribution are studied in a connection with the other evidences of transport in a one-dimensional Mori chain. The second mom… more
Date: May 1998
Creator: Bystrik, Anna
Partner: UNT Libraries

Ongoing Developments on Continuum Solvation Models

Description: This work explores a continuum representation for diffuse layer models, thereby endowing continuum embedding models the ability to capture electrostatic phenomena in the environment such as the existence of electrolyte ions, and the nature of ionic liquids. It introduces a new field-aware continuum model that adjusts the size of the quantum regime per atom based on the distribution of charge in a system. The model accounts for the asymmetric nature of solvent distribution when applied to cation… more
Date: May 2022
Creator: Truscott, Matthew Anthony Si Ren
Partner: UNT Libraries
open access

Operator Gauge Transformations in Nonrelativistic Quantum Electrodynamics

Description: A system of nonrelativistic charged particles and radiation is canonically quantized in the Coulomb gauge and Maxwell's equations in quantum electrodynamics are derived. By requiring form invariance of the Schrodinger equation under a space and time dependent unitary transformation, operator gauge transformations on the quantized electromagnetic potentials and state vectors are introduced. These gauge transformed potentials have the same form as gauge transformations in non-Abelian gauge field … more
Date: December 1982
Creator: Gray, Raymond Dale
Partner: UNT Libraries
open access

Optical Control of Coherent Quantum Systems

Description: Optical control of coherent quantum systems has many methods and applications. In this defense we will discuss the effects of an electric field interacting with molecules with dipole moments. The theoretical study of such molecules will consist of two-level atom and a three-level atom in the λ configuration. The methods that will be discussed are population trapping using both bright and dark starts obtained by both STIRAP and CHIRAP pulses. The application to be discussed is how to create a ro… more
Date: December 2022
Creator: Roy, Colin Dean
Partner: UNT Libraries
open access

Optical Nonlinearities in Semiconductors for Limiting

Description: I have conducted detailed experimental and theoretical studies of the nonlinear optical properties of semiconductor materials useful for optical limiting. I have constructed optical limiters utilizing two-photon absorption along with photogenerated carrier defocusing as well as the bound electronic nonlinearity using the semiconducting material ZnSe. I have optimized the focusing geometry to achieve a large dynamic range while maintaining a low limiting energy for the device. The ZnSe monolithi… more
Date: May 1990
Creator: Wu, Yuan-Yen
Partner: UNT Libraries

Optical Property Study of 2D Graded Photonic Super-Crystals for Photon Management

Description: In this dissertation, we study the optical property of 2D graded photonic super-crystals (GPSCs) for photon management. We focused primarily on manipulation and control of light by using the newly discovered GPSCs which present great opportunity for electromagnetic wave control in photonic devices. The GPSC has been used to explore the superior capability of improving the light extraction efficiency of OLEDs. The enhancement of extraction efficiency has been explained in term of destructive int… more
Date: May 2020
Creator: Hassan, Safaa
Partner: UNT Libraries

PAOFLOW-Aided Computational Materials Design

Description: Functional materials are essential to human welfare and to provide foundations for emerging industries. As an alternative route to experimental materials discovery, computational materials designs are playing an increasingly significant role in the whole discovery process. In this work, we use an in-house developed python utility: PAOFLOW, which generates finite basis Hamiltonians from the projection of first principles plane-wave pseudopotential wavefunctions on pseudo atomic orbitals(PAO) for… more
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Date: December 2019
Creator: Wang, Haihang
Partner: UNT Libraries
open access

Parametric Studies of Picosecond Laser-Induced Breakdown in Fused Quartz and NaCl

Description: Bulk laser-induced breakdown and self-focusing in single samples of fused quartz and NaCl were examined using picosecond optical pulses at 1.0 ym and 0.5 ym. The results of three separate but related experiments are reported. First the nonlinear index of refraction, n2, of each of the test materials is measured near the respective damage thresholds of the samples. The values of 1*2 were determined by detecting beam distortions in the far field, transmitted laser beam profile caused by the irrad… more
Date: December 1984
Creator: Williams, William Ely
Partner: UNT Libraries
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Perturbation of renewal processes

Description: Renewal theory began development in the early 1940s, as the need for it in the industrial engineering sub-discipline operations research had risen. In time, the theory found applications in many stochastic processes. In this thesis I investigated the effect of seasonal effects on Poisson and non-Poisson renewal processes in the form of perturbations. It was determined that the statistical analysis methods developed at UNT Center for Nonlinear Science can be used to detect the effects of seasona… more
Date: May 2008
Creator: Akin, Osman Caglar
Partner: UNT Libraries
open access

Phase Transition Studies in Polar and Nonpolar Liquids at Microwave Frequencies

Description: A resonant microwave cavity technique was employed to study the dielectric behavior of some polar and non-polar liquids near the phase transition temperatures at microwave frequencies of 7.2, 9.2 and 10.1 GHz. The Slater perturbation equations for a resonant microwave cavity are briefly discussed to show that the above technique can be used to determine both the real and imaginary parts of dielectric response. Abrupt changes in dielectric response were observed near the phase transition tempera… more
Date: August 1980
Creator: Dahiya, Jai N. (Jai Narain)
Partner: UNT Libraries
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Photoconductivity Investigation of Two-Photon Magneto-Absorption, PACRH, and Deep Levels in n-InSb

Description: A high resolution photoconductivity investigation of two 13 -3 photon magneto-absorption (TPMA) in n-InSb (n - 9 x 10 cm ) has been performed. This is the first time that two-photon absorption in a semiconductor has been studied with cw lasers only. With a stable cw CC>2 laser and a highly sensitive sampling and magnetic field modulation technique, a minimum of 4 2 transitions in the TPMA photoconductivity spectra can be observed. Most of these transitions are a result of the usual spherical ap… more
Date: May 1982
Creator: Goodwin, Mike Watson
Partner: UNT Libraries
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Photon Exchange Between a Pair of Nonidentical Atoms with Two Forms of Interactions

Description: A pair of nonidentical two-level atoms, separated by a fixed distance R, interact through photon exchange. The system is described by a state vector which is assumed to be a superposition of four "essential states": (1) the first atom is excited, the second one is in the ground state, and no photon is present, (2) the first atom is in its ground state, the second one is excited, and no photon is present, (3) both atoms are in their ground states and a photon is present, and (4) both atoms are e… more
Date: May 1987
Creator: Golshan, Shahram Mohammad-Mehdi
Partner: UNT Libraries
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Physical Boundary as a Source of Anomalies in Transport Processes in Acoustics and Electrodynamics

Description: Various anomalous effects that emerge when the interfaces between media are involved in sound-matter or light-matter interactions are studied. The three specific systems examined are a fluid channel between elastic metal plates, a linear chain of metallic perforated cylindrical shells in air, and a metal-dielectric slab with the interfaces treated as finite regions of smoothly changing material properties. The scattering of acoustic signals on the first two is predicted to be accompanied by the… more
Date: December 2018
Creator: Bozhko, Andrii
Partner: UNT Libraries
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The Physics of Gaseous Exposures on Active Field Emission Microcathode Arrays

Description: The interaction of active molybdenum field emission microcathode arrays with oxygen, water, carbon dioxide, methane, hydrogen and helium gases was studied. Experiments were setup to measure the emission characteristics as a function of gas exposures. The resulting changes in the surface work function of the tips were determined from the Fowler-Nordheim plots. The kinetics of the FEA-gas interaction were studied by observing the ion species originating from the array during and after gas exposur… more
Date: September 1996
Creator: Chalamala, Babu Reddy
Partner: UNT Libraries
open access

Picosecond Dynamics of Free-Carrier Populations, Space-Charge Fields, and Photorefractive Nonlinearities in Zincblende Semiconductors

Description: Generally, nonlinear optics studies investigate optically-induced changes in refraction or absorption, and their application to spectroscopy or device fabrication. The photorefractive effect is a nonlinear optical effect that occurs in solids, where transport of an optically-induced free-carrier population results in an internal space-charge field, which produces an index change via the linear electrooptic effect. The photorefractive effect has been widely studied for a variety of materials and… more
Date: August 1999
Creator: Stark, Thomas S.
Partner: UNT Libraries
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Picosecond Laser-Induced Transient Gratings and Anisotropic State-Filling in Germanium

Description: We present a comparative theoretical study of the transient grating coherent effects in resonant picosecond excitation-probe experiments. Signals in both the probe and conjugate directions are discussed. The effects of recombination, non-radiative scattering and spatial and orientational diffusion are included. The analysis is applied to both a molecular and to a semiconductor model. Signal contributions from concentration and orientational gratings are distinguished and their temporal natures … more
Date: December 1982
Creator: Boggess, Thomas F. (Thomas Frederick)
Partner: UNT Libraries
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Picosecond Measurement of Interband Saturation, Intervalence Band Absorption, and Surface Recombination in Germanium

Description: The picosecond optical response of five thin germanium samples was measured following intense optical excitation using two variations of the excitation and probe technique. Seven-picosecond laser pulses of wavelength 1.054 um were used to measure the optical transmission of the samples for a variety of probe delays, excitation fluences, and sample temperatures. These parametric experiments were performed in an effort to determine if carrier cooling, carrier diffusion, or carrier recombination d… more
Date: August 1984
Creator: Perryman, Gary Paul
Partner: UNT Libraries
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Picosecond Measurement of Nonlinear Diffusion and Recombination Processes in Germanium

Description: A variation of the excite-and-probe technique is used to measure the picosecond evolution of laser-induced transient gratings that are produced in germanium by the direct absorption of 40 psec optical pulses at 1.06-μm. Grating lifetimes are determined for free carrier densities between 10¹⁸ cm⁻³ and 10²¹ cm⁻³ . For carrier densities less than 10¹⁹ cm⁻³ , a linear diffusion-recombination model for the grating provides a good fit to the experimental data and allows the extraction of the diffusio… more
Date: May 1981
Creator: Moss, Steven Charles
Partner: UNT Libraries
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Placing High-Redshift Quasars in Perspective: Unifying Distant Quasars with Their Lower Redshift Counterparts through Near-Infrared Spectroscopy

Description: I present spectroscopic measurements for 260 sources from the Gemini Near Infrared Spectrograph–Distant Quasar Survey (GNIRS-DQS). Being the largest uniform, homogeneous survey of its kind, it represents a flux-limited sample of Sloan Digital Sky Survey (SDSS) quasars at 1.5 < z < 3.5. A combination of the GNIRS and SDSS spectra covers principal quasar diagnostic features, chiefly the C IV λ1549, Mg II λλ2798, 2803, Hβ λ4861, and [O III] λλ4959, 5007 emission lines, in each source. The spectral… more
Date: May 2023
Creator: Matthews, Brandon M.
Partner: UNT Libraries
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