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  Access Rights: Use restricted to UNT Community
 Decade: 2010-2019
 Collection: UNT Theses and Dissertations
Design, Synthesis and Screening of Homoleptic and Heteroleptic Platinum(ii) Pyridylazolate Complexes for N-type Semiconducting and Light-emitting Devices

Design, Synthesis and Screening of Homoleptic and Heteroleptic Platinum(ii) Pyridylazolate Complexes for N-type Semiconducting and Light-emitting Devices

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Date: August 2012
Creator: Oswald, Iain William Herbert
Description: A series of heteroleptic and homoleptic platinum(II) complexes has been synthesized and characterized towards their use in thin film devices such as organic light-emitting diodes (OLEDs) and organic thin film transistors (OTFTs). Pyridylpyrazolate- and pyridyltetrazolate-containing ligands were selected due to their structural rigidity and ease of functionalization. Single-crystal x-ray diffraction studies of two selected heteroleptic complexes show strong aggregation with preferential stacking into vertical columns with a varying degree of overlap of the neighboring square planar molecular units. It is shown that the close proximity of the molecules to one another in the stack increases semiconducting character, phosphorescence quantum yields, and shorter radiative lifetimes. The potential for these materials towards incorporation into high-efficiency doping free white OLEDs (DFW-OLEDs) for solid-state lighting and display applications has been realized and will be expanded upon by present and future embodiments of materials in this thesis.
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The Enemy of My Enemy Is What, Exactly? the British Flanders Expedition of 1793 and Coalition Diplomacy

The Enemy of My Enemy Is What, Exactly? the British Flanders Expedition of 1793 and Coalition Diplomacy

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Date: August 2012
Creator: Jarrett, Nathaniel W.
Description: The British entered the War of the First Coalition against Revolutionary France in 1793 diplomatically isolated and militarily unprepared for a major war. Nonetheless, a French attack on the Dutch Republic in February 1793 forced the British to dispatch a small expeditionary force to defend their ally. Throughout the Flanders campaign of 1793, the British expeditionary force served London as a tool to end British isolation and enlist Austrian commitment to securing British war objectives. The 1793 Flanders campaign and the Allied war effort in general have received little attention from historians, and they generally receive dismissive condemnation in general histories of the French Revolutionary Wars. This thesis examines the British participation in the 1793 Flanders campaign a broader diplomatic context through the published correspondence of relevant Allied military and political leaders. Traditional accounts of this campaign present a narrative of defeat and condemn the Allies for their failure to achieve in 1793 the accomplishments of the sixth coalition twenty years later. Such a perspective obscures a clear understanding of the reasons for Allied actions. This thesis seeks to correct this distortion by critically analyzing the relationship between British diplomacy within the Coalition and operations in Flanders. Unable to achieve ...
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José Antonio Gómez´s Versos Para Órgano (Section I): a Practical Guide for Performance

José Antonio Gómez´s Versos Para Órgano (Section I): a Practical Guide for Performance

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Date: August 2012
Creator: Carrasco Curíntzita, Laura A.
Description: José Antonio Gómez is an important figure in Mexican music history and his works are considered representative of the beginning of Mexico´s Independent era. Some musicians are familiar with Gómez´s choral output but his organ music is rarely considered. Due to the lack of an edition of Gómez´s Versets for Organ, a practical guide was found needed to aid its performance. This study is based on performance, analysis, and direct work on the only known source for it. The first chapter, Introduction, presents the argument for an edited version of the first part of the manuscript as a performance guide. The second provides biographical information on the composer. The third chapter discusses the background for the original performance of the Versets for Organ. Chapter 4 provides performance considerations for the works. The edition of the manuscript is included in chapter 5.
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The Useful Arts

The Useful Arts

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Date: August 2012
Creator: Hindman, Jessica
Description: This creative nonfiction dissertation is a series of braided narratives that chronicle the author's career as a trombonist in the John Smith Ensemble. As an amateur trombonist, the author is shocked to be hired as a professional musician for an orchestra that plays on PBS and at Carnegie Hall. She quickly realizes, however, that the job requires her to play the trombone quietly in front of an unplugged microphone while a CD recording of another, more talented trombonist is blasted out toward an unknowing audience. The job also requires the author to tour around America. The scenes of from this tour are braided with scenes wherein she reflects on her life as a professional fake musician and her past failed attempts at getting a job.
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Challenge the Silence

Challenge the Silence

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Date: August 2012
Creator: Peterson, Erica
Description: This collection of personal essays about incest, abuse, and depression explores the lasting effects of an invisible childhood. The essays follow the protagonist from the age of five to her early twenties. Her brother, at a young age, becomes sexually abusive of her and her sisters, and her parents fail to protect their daughters. The family is divided as the older girls strive to defend their little sisters, while their parents attempt to excuse their son. When her brother is finally sent away, the protagonist is left to salvage what remains of her relationships with her parents.
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Between Comancheros and Comanchería: a History of Fort Bascom, New Mexico

Between Comancheros and Comanchería: a History of Fort Bascom, New Mexico

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Date: August 2012
Creator: Blackshear, James Bailey
Description: In 1863, Fort Bascom was built along the Canadian River in the Eroded Plains of Territorial New Mexico. Its unique location placed it between the Comanches of Texas and the Comancheros of the Sangre de Cristo Mountains. This post was situated within Comanchería during the height of the United States Army's war against the Southern Plains Indians, yet it has garnered little attention. This study broadens the scholarly understanding of how the United States Army gained control of the Southwest by examining the role Fort Bascom played in this mission. This includes an exploration of the Canadian River Valley environment, an examination of the economic relationship that existed between the Southern Plains Indians and the mountain people of New Mexico, and an account of the daily life of soldiers posted to Fort Bascom. This dissertation thus provides an environmental and cultural history of the Canadian River Valley in New Mexico, a social history of the men stationed at Fort Bascom, and proof that the post played a key role in the Army's efforts to gain control of the Southern Plains Indians. This study argues that Fort Bascom should be recognized as Texas' northern-most frontier fort. Its men were closer to ...
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Southern Roots, Western Foundations: the Peculiar Institution and the Livestock Industry on the Northwestern Frontier of Texas, 1846-1864

Southern Roots, Western Foundations: the Peculiar Institution and the Livestock Industry on the Northwestern Frontier of Texas, 1846-1864

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Date: August 2012
Creator: Liles, Deborah Marie
Description: This dissertation challenges Charles W. Ramsdell's needless war theory, which argued that profitable slavery would not have existed west of the 98th meridian and that slavery would have died a natural death. It uses statistical information that is mined from the county tax records to show how slave-owners on the northwestern frontier of Texas raised livestock rather than market crops, before and during the Civil War. This enterprise was so strong that it not only continued to expand throughout this period, but it also became the foundation for the recovery of the Texas economy after the war.
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Expression of G-protein Coupled Receptors in Young and Mature Thrombocytes and Knockdown of Gpr18 in Zebrafish

Expression of G-protein Coupled Receptors in Young and Mature Thrombocytes and Knockdown of Gpr18 in Zebrafish

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Date: May 2013
Creator: Potbhare, Vrinda Nikhil
Description: In this study, a novel method based on biotinylated antibodies and streptavidin coated magnetic beads was used to separate the thrombocyte subpopulations from zebrafish whole blood. DiI-C18, a lipophilic dye, labels only young thrombocytes when used at low concentrations. Commercially available biotinylated anti-Cy3 antibody was used to label the chromophore of DiI-C18 on the young thrombocytes and streptavidin coated magnetic beads were added subsequently, to separate young thrombocytes. The remaining blood cells were probed with custom-made biotinylated anti-GPIIb antibody and streptavidin magnetic beads to separate them from other cells. Further, thrombocytes are equivalents of mammalian platelets. Platelets play a crucial role in thrombus formation. The G-protein coupled receptors (GPCRs) present on the platelet surface are involved during platelet activation and aggregation processes. So, thrombocytes were studied for the presence of GPCRs. The GPCR mRNA transcripts expressed in the young and mature thrombocytes were subjected to densitometry analysis and pixel intensities of the bands were compared using one way ANOVA. This analysis did not show significant differences between the young and mature GPCR mRNA transcripts but identified a novel GPCR, GPR18 that was not reported in platelets earlier. To study the function of this GPCR, it was knocked down using GPR18 ...
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Interspecimen Study of Bone to Relate Macromechanical, Nanomechanical and Compositional Changes Across the Femoral Cortex of Bone

Interspecimen Study of Bone to Relate Macromechanical, Nanomechanical and Compositional Changes Across the Femoral Cortex of Bone

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Date: May 2013
Creator: Nar, Mangesh
Description: Mechanics of bone is widely studied and researched, mainly for the study of fracture. This has been done mostly on a macro scale. In this work hierarchical nature of bone has been explored to investigate bone mechanics in more detail. Flexural test were done to classify the bones according to their strength and deflection. Raman spectroscopy analysis was done to map the mineralization, collagen crosslinking changes across the thickness of the bone. Nanoindentation was done to map indentation hardness and indentation modulus across femoral cortex of the bone. The results indicate that the composition of the bone changes across the thickness of the femoral cortex. The hypothesis is confirmed as increase in mineralization, carbonate to phosphate ratio and collagen crosslinking shows the effect as increased indentation hardness and modulus and decreased deflection.
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Investigating Postpartum Depression in Southern Rural Egypt and Effects of Sertraline on Fsh and Lh Gene Expression on Fathead Minnows Using Rt-pcr

Investigating Postpartum Depression in Southern Rural Egypt and Effects of Sertraline on Fsh and Lh Gene Expression on Fathead Minnows Using Rt-pcr

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Date: May 2013
Creator: Mohamed, Hagar Abdo
Description: Postpartum depression (PPD) is a major health problem that affects many women worldwide. In Egypt, PPD is neglected despite the expected high prevalence rate among women during the transition period after the Egyptian revolution. This research investigated the prevalence, risk factors, and interventions of postpartum depression in southern rural Egypt. Interviews were conducted with 57 participants recruited from public and private hospitals. Questionnaires and the Arabic version of the Edinburgh Postnatal Depression Scale were administered. The prevalence of PPD is 73.7%. PPD is associated with low income and age at childbirth. Most participants regarded screening mothers after childbirth for PPD as effective; in comparison to, antidepressants that were regarded by most participants as ineffective. Women in southern rural Egypt prefer high number of pregnancies, so investigating the influence of sertraline, an antidepressant medication, on female hormones becomes important. In this research, fathead minnows were exposed to 3 and 10 ppb sertraline for 7 days. Real-time Polymerase Chain Reaction was used to detect the change in gene expression of the Follicle-stimulating hormone (FSH) and luteinizing hormone (LH). Results showed that a down regulation at the 10 ppb was evident on the LH and to a lesser extent on FSH. Our results ...
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