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open access

Analysis of Biological Materials Using a Nuclear Microprobe

Description: The use of nuclear microprobe techniques including: Particle induced x-ray emission (PIXE) and Rutherford backscattering spectrometry (RBS) for elemental analysis and quantitative elemental imaging of biological samples is especially useful in biological and biomedical research because of its high sensitivity for physiologically important trace elements or toxic heavy metals. The nuclear microprobe of the Ion Beam Modification and Analysis Laboratory (IBMAL) has been used to study the enhanceme… more
Date: December 2014
Creator: Mulware, Stephen Juma
Partner: UNT Libraries
open access

Broad-band Light Emission From Ion Implanted Silicon Nanocrystals Via Plasmonic and Non-plasmonic Effects for Optoelectronics

Description: Broad band light emission ranging from the ultraviolet (UV) to the near infrared (NIR) has been observed from silicon nanoparticles fabricated using low energy (30-45 keV) metal and non-metal ion implantation with a fluence of 5*1015 ions/cm2 in crystalline Si(100). It is found from a systematic study of the annealing carried out at certain temperatures that the spectral characteristics remains unchanged except for the enhancement of light emission intensity due to annealing. The annealing resu… more
Date: December 2012
Creator: Singh, Akhilesh K.
Partner: UNT Libraries
open access

Core-Shell Based Metamaterials: Fabrication Protocol and Optical Properties

Description: The objective of this study is to examine core-shell type plasmonic metamaterials aimed at the development of materials with unique electromagnetic properties. The building blocks of metamaterials under study consist of gold as a metal component, and silica and precipitated calcium carbonate (PCC) as the dielectric media. The results of this study demonstrate important applications of the core-shells including scattering suppression, airborne obscurants made of fractal gold shells, photomodific… more
Date: December 2017
Creator: De Silva, Vashista C
Partner: UNT Libraries
open access

Design, Construction, and Application of an Electrostatic Quadrupole Doublet for Heavy Ion Nuclear Microprobe Research

Description: A nuclear microprobe, typically consisting of 2 - 4 quadrupole magnetic lenses and apertures serving as objective and a collimating divergence slits, focuses MeV ions to approximately 1 x 1 μm for modification and analysis of materials. Although far less utilized, electrostatic quadrupole fields similarly afford strong focusing of ions and have the added benefit of doing so independent of ion mass. Instead, electrostatic quadrupole focusing exhibits energy dependence on focusing ions. A heav… more
Date: December 2017
Creator: Manuel, Jack Elliot
Partner: UNT Libraries
open access

Electrical Conduction Mechanisms in the Disordered Material System P-type Hydrogenated Amorphous Silicon

Description: The electrical and optical properties of boron doped hydrogenated amorphous silicon thin films (a-Si) were investigated to determine the effect of boron and hydrogen incorporation on carrier transport. The a-Si thin films were grown by plasma enhanced chemical vapor deposition (PECVD) at various boron concentrations, hydrogen dilutions, and at differing growth temperatures. The temperature dependent conductivity generally follows the hopping conduction model. Above a critical temperature, the d… more
Date: December 2014
Creator: Shrestha, Kiran (Engineer)
Partner: UNT Libraries
open access

Electrically Tunable Absorption and Perfect Absorption Using Aluminum-Doped Zinc Oxide and Graphene Sandwiched in Oxides

Description: Understanding the fundamental physics in light absorption and perfect light absorption is vital for device applications in detector, sensor, solar energy harvesting and imaging. In this research study, a large area fabrication of Al-doped ZnO/Al2O3/graphene/Al2O3/gold/silicon device was enabled by a spin-processable hydrophilic mono-layer graphene oxide. In contrast to the optical properties of noble metals, which cannot be tuned or changed, the permittivity of transparent metal oxides, such a… more
Date: December 2018
Creator: Adewole, Murthada Oladele
Partner: UNT Libraries
open access

Exploring Growth Kinematics and Tuning Optical and Electronic Properties of Indium Antimonide Nanowires

Description: This dissertation work is a study of the growth kinematics, synthesis strategies and intrinsic properties of InSb nanowires (NWs). The highlights of this work include a study of the effect of the growth parameters on the composition and crystallinity of NWs. A change in the temperature ramp-up rate as the substrate was heated to reach the NW growth temperature resulted in NWs that were either crystalline or amorphous. The as-grown NWs were found to have very different optical and electrical pro… more
Date: December 2018
Creator: Algarni, Zaina Sluman
Partner: UNT Libraries
open access

Fabrication and Study of the Optical Properties of 3D Photonic Crystals and 2D Graded Photonic Super-Crystals

Description: In this dissertation, I am presenting my research on the fabrication and simulation of the optical properties of 3D photonic crystals and 2D graded photonic super-crystals. The 3D photonic crystals were fabricated using holographic lithography with a single, custom-built reflective optical element (ROE) and single exposure from a visible light laser. Fully 3D photonic crystals with 4-fold, 5- fold, and 6-fold symmetries were fabricated using the flexible, 3D printed ROE. In addition, novel 2D g… more
Date: December 2018
Creator: Lowell, David
Partner: UNT Libraries
open access

Fractional Calculus and Dynamic Approach to Complexity

Description: Fractional calculus enables the possibility of using real number powers or complex number powers of the differentiation operator. The fundamental connection between fractional calculus and subordination processes is explored and affords a physical interpretation for a fractional trajectory, that being an average over an ensemble of stochastic trajectories. With an ensemble average perspective, the explanation of the behavior of fractional chaotic systems changes dramatically. Before now what ha… more
Date: December 2015
Creator: Beig, Mirza Tanweer Ahmad
Partner: UNT Libraries
open access

Interaction of Plasmons and Excitons for Low-Dimension Semiconductors

Description: The effects of surface plasmon for InGaN/GaN multi-quantum wells and ZnO nanoparticles optical linear and nonlinear emission efficiency had been experimentally studied. Due to the critical design for InGaN MQWs with inverted hexagonal pits based on GaN, both contribution of surface plasmon effect and image charge effect at resonant and off resonant frequencies were experimentally and theoretically investigated. With off- resonant condition, the InGaN MQWs emission significantly enhanced by meta… more
Date: December 2014
Creator: Lin, Jie (physicist)
Partner: UNT Libraries
open access

Ion Beam Synthesis of Binary and Ternary Transition Metal Silicide Thin Films

Description: Among the well-known methods to form or modify the composition and physical properties of thin films, ion implantation has shown to be a very powerful technique. In particular, ion beam syntheses of binary iron silicide have been studied by several groups. Further, the interests in transition metal silicide systems are triggered by their potential use in advanced silicon based opto-electronic devices. In addition, ternary silicides have been by far less studied than their binary counterparts de… more
Date: December 2016
Creator: Lakshantha, Wickramaarachchige Jayampath
Partner: UNT Libraries
open access

Local Phase Manipulation for Multi-Beam Interference Lithography for the Fabrication of Two and Three Dimensional Photonic Crystal Templates

Description: In this work, we study the use of a spatial light modulator (SLM) for local manipulation of phase in interfering laser beams to fabricate photonic crystal templates with embedded, engineered defects. A SLM displaying geometric phase patterns was used as a digitally programmable phase mask to fabricate 4-fold and 6-fold symmetric photonic crystal templates. Through pixel-by-pixel phase engineering, digital control of the phases of one or more of the interfering beams was demonstrated, thus allo… more
Date: December 2016
Creator: Lutkenhaus, Jeffrey Ryan
Partner: UNT Libraries
open access

Low-Energy Electron Irradiation of Preheated and Gas-Exposed Single-Wall Carbon Nanotubes

Description: We investigate the conditions under which electron irradiation of single-walled carbon nanotube (SWCNT) bundles with 2 keV electrons produces an increase in the Raman D peak. We find that an increase in the D peak does not occur when SWCNTs are preheated in situ at 600 C for 1 h in ultrahigh vacuum (UHV) before irradiation is performed. Exposing SWCNTs to air or other gases after preheating in UHV and before irradiation results in an increase in the D peak. Small diameter SWCNTs that are not pr… more
Date: December 2016
Creator: Ecton, Philip
Partner: UNT Libraries

Manipulation of Light-Matter Interactions in Molybdenum Disulfide (MoS2) Monolayer through Dressed Phonons (DP) and Plasmons

Description: The performance of electrical and optical devices based on two-dimensional semiconductors (2D) such as molybdenum disulfide is critically influenced due to very poor light absorption in the atomically thin layers. In this study, the phonon mediated optical absorption and emission properties in single atomic layers of MoS2 have been investigated. The electronic transitions in MoS2 due to near-field optical interaction and the influence of interface phonons due to the dielectric substrate GaN on … more
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Date: December 2019
Creator: Poudel, Yuba R
Partner: UNT Libraries
open access

Nonlinear and Quantum Optics Near Nanoparticles

Description: We study the behavior of electric fields in and around dielectric and metal nanoparticles, and prepare the ground for their applications to a variety of systems viz. photovoltaics, imaging and detection techniques, and molecular spectroscopy. We exploit the property of nanoparticles being able to focus the radiation field into small regions and study some of the interesting nonlinear, and quantum coherence and interference phenomena near them. The traditional approach to study the nonlinear lig… more
Date: December 2015
Creator: Dhayal, Suman
Partner: UNT Libraries
open access

Novel Semi-Conductor Material Systems: Molecular Beam Epitaxial Growth and Characterization

Description: Semi-conductor industry relies heavily on silicon (Si). However, Si is not a direct-band gap semi-conductor. Consequently, Si does not possess great versatility for multi-functional applications in comparison with the direct band-gap III-V semi-conductors such as GaAs. To bridge this gap, what is ideally required is a semi-conductor material system that is based on silicon, but has significantly greater versatility. While sparsely studied, the semi-conducting silicides material systems offer gr… more
Date: December 2013
Creator: Elmarhoumi, Nader M.
Partner: UNT Libraries

PAOFLOW-Aided Computational Materials Design

Description: Functional materials are essential to human welfare and to provide foundations for emerging industries. As an alternative route to experimental materials discovery, computational materials designs are playing an increasingly significant role in the whole discovery process. In this work, we use an in-house developed python utility: PAOFLOW, which generates finite basis Hamiltonians from the projection of first principles plane-wave pseudopotential wavefunctions on pseudo atomic orbitals(PAO) for… more
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Date: December 2019
Creator: Wang, Haihang
Partner: UNT Libraries
open access

Physical Boundary as a Source of Anomalies in Transport Processes in Acoustics and Electrodynamics

Description: Various anomalous effects that emerge when the interfaces between media are involved in sound-matter or light-matter interactions are studied. The three specific systems examined are a fluid channel between elastic metal plates, a linear chain of metallic perforated cylindrical shells in air, and a metal-dielectric slab with the interfaces treated as finite regions of smoothly changing material properties. The scattering of acoustic signals on the first two is predicted to be accompanied by the… more
Date: December 2018
Creator: Bozhko, Andrii
Partner: UNT Libraries
open access

Quantum Coherence Effects Coupled via Plasmons

Description: This thesis is an attempt at studying quantum coherence effects coupled via plasmons. After introducing the quantum coherence in atomic systems in Chapter 1, we utilize it in Chapter 2 to demonstrate a new technique of detection of motion of single atoms or irons inside an optical cavity. By taking into account the interaction of coherences with surface plasmonic waves excited in metal nanoparticles, we provide a theoretical model along with experimental data in Chapter 3 to describe the modifi… more
Date: December 2018
Creator: Moazzezi, Mojtaba
Partner: UNT Libraries
open access

Sputtering of Bi and Preferential Sputtering of an Inhomogeneous Alloy

Description: Angular distributions and total yields of atoms sputtered from bismuth targets by normally incident 10 keV -50 keV Ne+ and Ar+ ions have been measured both experimentally and by computer simulation. Polycrystalline Bi targets were used for experimental measurements. The sputtered atoms were collected on high purity aluminum foils under ultra-high vacuum conditions, and were subsequently analyzed using Rutherford backscattering spectroscopy. The Monte-Carlo based SRIM code was employed to simula… more
Date: December 2014
Creator: Deoli, Naresh T.
Partner: UNT Libraries
open access

Studies of Charged Particle Dynamics for Antihydrogen Synthesis

Description: Synthesis and capture of antihydrogen in controlled laboratory conditions will enable precise studies of neutral antimatter. The work presented deals with some of the physics pertinent to manipulating charged antiparticles in order to create neutral antimatter, and may be applicable to other scenarios of plasma confinement and charged particle interaction. The topics covered include the electrostatic confinement of a reflecting ion beam and the transverse confinement of an ion beam in a purely … more
Date: December 2014
Creator: Correa, Jose Ricardo
Partner: UNT Libraries
open access

Temporal Properties Of Dynamic Processes On Complex Networks

Description: Many social, biological and technological systems can be viewed as complex networks with a large number of interacting components. However despite recent advancements in network theory, a satisfactory description of dynamic processes arising in such cooperative systems is a subject of ongoing research. In this dissertation the emergence of dynamical complexity in networks of interacting stochastic oscillators is investigated. In particular I demonstrate that networks of two and three state stoc… more
Date: December 2011
Creator: Turalska, Malgorzata A.
Partner: UNT Libraries
open access

Theoretical and Experimental Investigations of Peg Based Thermo Sensitive Hydro Microgel

Description: Poly ethylene glycol (PEG) based microgels were synthesized and investigated. The PEG microgel has the same phase transition as the traditional poly N-isopropylacrylamide (PNIPAM). As a good substitute of PNIPAM, PEG microgel exhibits many advantages: it is easier to control the lower critical solution temperature (LCST) of the microgel by changing the component of copolymers; it has a more solid spherical core-shell structure to have a double thermo sensitivity; it is straightforward to add ot… more
Date: December 2012
Creator: Chi, Chenglin
Partner: UNT Libraries
open access

Variational Calculations of Positronium Scattering with Hydrogen

Description: Positronium-hydrogen (Ps-H) scattering is of interest, as it is a fundamental four-body Coulomb problem. We have investigated low-energy Ps-H scattering below the Ps(n=2) excitation threshold using the Kohn variational method and variants of the method with a trial wavefunction that includes highly correlated Hylleraas-type short-range terms. We give an elegant formalism that combines all Kohn-type variational methods into a single form. Along with this, we have also developed a general formali… more
Date: December 2015
Creator: Woods, Denton
Partner: UNT Libraries
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